Most of the plutonium in the world resides inside spent nuclear reactor fuel rods. This high-level radioactive waste is commonly held in long-term storage within large, heavily shielded casks. Currently, international nuclear safeguards inspectors have no stand-alone method of verifying the amount of reactor fuel stored within a sealed cask. Here we demonstrate experimentally that measurements of the scattering angles of cosmic-ray muons, which pass through a storage cask, can be used to determine if spent fuel assemblies are missing without opening the cask. This application of technology and methods commonly used in high-energy particle physics provides a potential solution to this long-standing problem in international nuclear safeguards.

We demonstrate the efficacy of wave-interference-based light trapping and carrier transport in parabolic-pore photonic-crystal, thin-crystalline silicon ($c$-Si) solar cells to achieve above 29% power conversion efficiencies. Using a rigorous solution of Maxwell’s equations through a standard finite-difference time domain scheme, we optimize the design of the vertical-parabolic-pore photonic crystal (PhC) on a $10\text{−}\mu \mathrm{m}$-thick $c$-Si solar cell to obtain a maximum achievable photocurrent density (MAPD) of $40.6\mathrm{mA}/{\mathrm{cm}}^2$ beyond the ray-optical, Lambertian light-trapping limit. For a slanted-parabolic-pore PhC that breaks $x\text{−}y$ symmetry, improved light trapping occurs due to better coupling into parallel-to-interface refraction modes. We achieve the optimum MAPD of $41.6\mathrm{mA}/{\mathrm{cm}}^2$ for a tilt angle of 10° with respect to the vertical axis of the pores. This MAPD is further improved to $41.72\mathrm{mA}/{\mathrm{cm}}^2$ by introducing a 75-nm ${\mathrm{SiO}}_2$ antireflective coating on top of the solar cell. We use this MAPD and the associated charge-carrier generation profile as input for a numerical solution of Poisson’s equation coupled with semiconductor drift-diffusion equations using a Shockley-Read-Hall and Auger recombination model. Using experimentally achieved surface recombination velocities of $10\mathrm{cm}/\mathrm{s}$, we identify semiconductor doping profiles that yield power conversion efficiencies over 29%. Practical considerations of additional upper-contact losses suggest efficiencies close to 28%. This improvement beyond the current world record is largely due to an open-circuit voltage approaching 0.8 V enabled by reduced bulk recombination in our thin silicon architecture while maintaining a high short-circuit current through wave-interference-based light trapping.

The generation of true optical time standards will require the conversion of the highly stable optical-frequency output of an optical atomic clock to a high-fidelity time output. We demonstrate a comb-based clockwork that phase-coherently integrates $\sim 7\times {10}^{20}$ optical cycles of an input optical frequency to create a coherent time output. We verify the underlying stability of the optical timing system by comparing two comb-based clockworks with a common input optical frequency and show $<20\mathrm{fs}$ total time drift over the 37-day measurement period. Both clockworks also generate traditional timing signals including an optical pulse per second and a 10-MHz rf reference. The optical pulse-per-second time outputs remain synchronized to 240 attoseconds (240 as) at 1000 s. The phase-coherent 10-MHz rf outputs are stable to near a part in ${10}^{19}$. Fault-free timekeeping from an optical clock to femtosecond level over months is an important step in replacing the current microwave time standard by an optical standard.

A bipedal DNA nanowalker was recently reported to convert chemical energy into directional motion autonomously and efficiently. To elucidate its chemomechanical coupling mechanisms, three-dimensional molecular modeling is used to obtain coarse-grained foot-track binding potentials of the DNA nanowalker via unbiased and biased sampling techniques (for the potentials’ basin and high-energy edges, respectively). The binding state that is protected against fuel-induced dissociation responds asymmetrically to forward versus backward forces, unlike the unprotected state, demonstrating a mechanosensing capability to gate fuel binding. Despite complex DNA mechanics, the foot-track potential exhibits a surprisingly neat three-part profile, offering some general guidelines to rationally design efficient nanowalkers. Subsequent modeling of the bipedal walker attached to the track gives estimates of the free energy for each bipedal state, showing how the mechanosensing foot-track binding breaks the symmetry between the rear and front feet, enabling the rear foot to be selectively dissociated by fuel and generating efficient chemomechanical coupling.

Recently, it was suggested that the polarization dependence of light absorption to a single-walled carbon nanotube is altered by carrier doping. We specify theoretically the doping level at which the polarization anisotropy is reversed by plasmon excitation. The plasmon energy is mainly determined by the diameter of a nanotube because pseudospin makes the energy independent of the details of the band structure. We find that the effect of doping on the Coulomb interaction appears through the screened exchange energy, which can be observed as changes in the absorption peak positions. Our results strongly suggest the possibility that oriented nanotubes function as a polarization switch.

We present a technique for the precision synthesis of arbitrary polarization states of light with a high modulation bandwidth. Our approach consists of superimposing two laser light fields with the same wavelength, but with opposite circular polarizations, where the phase and the amplitude of each light field are individually controlled. We find that the polarization-synthesized beam reaches a degree of polarization of 99.99%, which is mainly limited by static spatial variations of the polarization state over the beam profile. We also find that the depolarization caused by temporal fluctuations of the polarization state is about 2 orders of magnitude smaller. In a recent work, Robens et al. [Low-Entropy States of Neutral Atoms in Polarization-Synthesized Optical Lattices, Phys. Rev. Lett. 118, 065302 (2017)] demonstrated an application of the polarization synthesizer to create two independently controllable optical lattices which trap atoms depending on their internal spin state. We use ultracold atoms in polarization-synthesized optical lattices to give an independent, in situ demonstration of the performance of the polarization synthesizer.

Removing particles from fibrous materials involves loosening via surfactants followed by particle transfer in a flow. While flow advection is commonly believed to be the major driver for pore-scale transport, small pores within the fabric do not allow any significant fluid flow inside them, thus significantly reducing the role of advection. However, rinsing the fabric with fresh water naturally establishes a surfactant gradient within the pore space, providing a suitable environment for particles to undergo diffusiophoresis. We demonstrate that this mechanism can remove particles from deep within fabric pores at an accelerated rate. The nonlinear aspect of diffusiophoresis significantly prolongs the lifetime of the phoretic motion beyond the naive solute diffusion time scale during rinsing, allowing long-lasting, continuous removal of particles. Moreover, owing to the fine balance between chemiphoresis and electrophoresis for particles in anionic surfactant concentration gradients, we show that the particle removal is sensitive to the counterion mobility, suggesting a simple route to control the effect. We thus claim to have resolved the “stagnant core problem”—a long-standing mystery in laundry detergency—and have identified a physicochemical approach to particle transport in fibrous media with broad applicability.

Quantum computing architectures rely on classical electronics for control and readout. Employing classical electronics in a feedback loop with the quantum system allows us to stabilize states, correct errors, and realize specific feedforward-based quantum computing and communication schemes such as deterministic quantum teleportation. These feedback and feedforward operations are required to be fast compared to the coherence time of the quantum system to minimize the probability of errors. We present a field-programmable-gate-array-based digital signal processing system capable of real-time quadrature demodulation, a determination of the qubit state, and a generation of state-dependent feedback trigger signals. The feedback trigger is generated with a latency of 110 ns with respect to the timing of the analog input signal. We characterize the performance of the system for an active qubit initialization protocol based on the dispersive readout of a superconducting qubit and discuss potential applications in feedback and feedforward algorithms.

Autonomous wireless body-implanted devices for biotelemetry, telemedicine, and neural interfacing constitute an emerging technology providing powerful capabilities for medicine and clinical research. We study the through-tissue electromagnetic propagation mechanisms, derive the optimal frequency range, and obtain the maximum achievable efficiency for radiative energy transfer from inside a body to free space. We analyze how polarization affects the efficiency by exciting TM and TE modes using a magnetic dipole and a magnetic current source, respectively. Four problem formulations are considered with increasing complexity and realism of anatomy. The results indicate that the optimal operating frequency $f$ for deep implantation (with a depth $d\gtrsim 3\mathrm{cm}$) lies in the (${10}^8–{10}^9$)-Hz range and can be approximated as $f=2.2\times {10}^7/d$. For a subcutaneous case ($d\lesssim 3\mathrm{cm}$), the surface-wave-induced interference is significant: within the range of peak radiation efficiency (about $2\times {10}^8$ to $3\times {10}^9\mathrm{Hz}$), the max-to-min ratio can reach a value of 6.5. For the studied frequency range, 80%–99% of radiation efficiency is lost due to the tissue-air wave-impedance mismatch. Parallel polarization reduces the losses by a few percent; this effect is inversely proportional to the frequency and depth. Considering the implantation depth, the operating frequency, the polarization, and the directivity, we show that about an order-of-magnitude efficiency improvement is achievable compared to existing devices.

We present a method to design an initial state in a quantum antenna in order to shape the emitted field higher-order correlation functions at will. This method is based on quantum state reconstruction techniques and relies on an entanglement of the emitters. We show that even the simplest antenna arrangements such as linear dipole arrays can exhibit a large variability in the emitted field-correlation function patterns, including, e.g., the generation of highly codirectional and contradirectional correlated twin photons, as well as multiphoton entangled states. Moreover, we identify a class of initial states that lead to a complete suppression of the field in the far-field zone. We also demonstrate the possibility to use a modified semiclassical approach for designing quantum antennas, simplifying the antenna state inference task. Our approach can find applications in the development of future quantum optics devices and methods, such as quantum sources for superresolution quantum imaging, high-precision sensing, as well as emitter-field interfaces for quantum information processing systems.

We experimentally investigate the decoherence of single surface-plasmon polaritons in metal stripe waveguides. We use a Mach-Zehnder configuration previously considered for measuring decoherence in atomic, electronic, and photonic systems. By placing waveguides of different lengths in one arm, we are able to measure the amplitude damping time $T_1=1.90\pm 0.01\times {10}^{-14}\mathrm{s}$, pure phase damping time $T_2^{*}=11.19\pm 4.89\times {10}^{-14}\mathrm{s}$ and total phase damping time $T_2=2.83\pm 0.32\times {10}^{-14}\mathrm{s}$. We find that decoherence is mainly due to amplitude damping, and thus loss arising from inelastic electron and photon scattering plays the most important role in the decoherence of plasmonic waveguides in the quantum regime. However, pure phase damping is not completely negligible. The results will be useful in the design of plasmonic waveguide systems for carrying out phase-sensitive quantum applications, such as quantum sensing. The probing techniques developed may also be applied to other plasmonic nanostructures, such as those used as nanoantennas, as unit cells in metamaterials, and as nanotraps for cold atoms.

We use microwave radiation generated by a semiconductor double-quantum-dot (DQD) micromaser for charge-state detection. A cavity is populated with $n_c\sim 6000$ photons by driving a current through an emitter DQD. These photons are used to sense the charge state of a target DQD that is located at the opposite end of the cavity. The charge dynamics in the target DQD influences the output power and emission frequency of the maser. Three different readout mechanisms are compared. The detection scheme requires no cavity input field and may potentially be used to improve the scalability of semiconductor and superconducting qubit readout technologies.

Voltage-induced magnetization dynamics in a conically magnetized free layer with an elliptic cylinder shape is theoretically studied on the basis of the macrospin model. It is found that an application of voltage pulse can induce the precessional switching of magnetization even at zero-bias magnetic field, which is of substantial importance for device applications such as voltage-controlled nonvolatile memory. Analytical expressions of the conditions for precessional switching are derived.

Focusing is a ubiquitous way to transform waves. Recently, a new type of shock wave has been observed experimentally with high-frame-rate ultrasound: shear shock waves in soft solids. These strongly nonlinear waves are characterized by a high Mach number, because the shear wave velocity is much slower, by 3 orders of magnitude, than the longitudinal wave velocity. Furthermore, these waves have a unique cubic nonlinearity which generates only odd harmonics. Unlike longitudinal waves for which only compressional shocks are possible, shear waves exhibit cubic nonlinearities which can generate positive and negative shocks. Here we present the experimental observation of shear shock wave focusing, generated by the vertical motion of a solid cylinder section embedded in a soft gelatin-graphite phantom to induce linearly vertically polarized motion. Raw ultrasound data from high-frame-rate (7692 images per second) acquisitions in combination with algorithms that are tuned to detect small displacements (approximately $1\mu \mathrm{m}$) are used to generate quantitative movies of gel motion. The features of shear shock wave focusing are analyzed by comparing experimental observations with numerical simulations of a retarded-time elastodynamic equation with cubic nonlinearities and empirical attenuation laws for soft solids.

Transient negative differential capacitance, the dynamic reversal of transient capacitance in an electrical circuit, is of highly technological and scientific interest since it probes the foundation of ferroelectricity. We study a resistor-ferroelectric capacitor ($R$-FEC) network through a series of coupled equations based on Kirchhoff’s law, electrostatics, and Landau theory. We show that transient negative capacitance (NC) in a $R$-FEC circuit originates from the mismatch in switching rate between the free charge on the metal plate and the bound charge in a ferroelectric (FE) capacitor during the polarization switching. This transient free charge–polarization mismatch is driven by the negative curvature of the FE free-energy landscape, and it is also analytically shown that a free-energy profile with a negative curvature is the only physical system that can describe transient NC in a $R$-FEC circuit. Furthermore, transient NC induced by the free charge–polarization mismatch is justified by its dependence on both external resistance and the intrinsic FE viscosity coefficient. The depolarization effect on FE capacitors emphasizes the importance of negative curvature to transient NC and also implies that transient and steady-state NC cannot be observed in a FE capacitor simultaneously. Finally, using the transient NC measurements, a procedure to experimentally determine the viscosity coefficient is presented to provide more insight into the relation between transient NC and the FE free-energy profile.

Current thermometry techniques lack the spatial resolution required to see the temperature gradients in typical, highly scaled modern transistors. As a step toward addressing this problem, we measure the temperature dependence of the volume plasmon energy in silicon nanoparticles from room temperature to $1250°\mathrm{C}$, using a chip-style heating sample holder in a scanning transmission electron microscope (STEM) equipped with electron energy loss spectroscopy (EELS). The plasmon energy changes as expected for an electron gas subject to the thermal expansion of silicon. Reversing this reasoning, we find that measurements of the plasmon energy provide an independent measure of the nanoparticle temperature consistent with that of the heater chip’s macroscopic, dual-function heater-and-thermometer to within the 5% accuracy of the thermometer’s calibration. Thus, silicon has the potential to provide its own high-spatial-resolution thermometric readout signal via measurements of its volume plasmon energy. Furthermore, nanoparticles can, in general, serve as convenient nanothermometers for in situ electron-microscopy experiments.

Wave-front shaping has emerged over the past decade as a powerful tool to control wave propagation through complex media, initially in optics and more recently also in the microwave domain with important applications in telecommunication, imaging, and energy transfer. The crux of implementing wave-front shaping concepts in real life is often its need for (direct) feedback, requiring access to the target to focus on. Here, we present the shaping of a microwave field based on indirect, unsolicited, and blind feedback which may be the pivotal step towards practical implementations. With the example of a radio-frequency harvester in a metallic cavity, we demonstrate tenfold enhancement of the harvested power by wave-front shaping based on nonlinear signals detected at an arbitrary position away from the harvesting device.

We demonstrate that small quantum memories, realized via quantum error correction in multiqubit devices, can benefit substantially by choosing a quantum code that is tailored to the relevant error model of the system. For a biased noise model, with independent bit and phase flips occurring at different rates, we show that a single code greatly outperforms the well-studied Steane code across the full range of parameters of the noise model, including for unbiased noise. In fact, this tailored code performs almost optimally when compared with 10 000 randomly selected stabilizer codes of comparable experimental complexity. Tailored codes can even outperform the Steane code with realistic experimental noise, and without any increase in the experimental complexity, as we demonstrate by comparison in the observed error model in a recent seven-qubit trapped ion experiment.

Porpoises are small-toothed whales, and they can produce directional acoustic waves to detect and track prey with high resolution and a wide field of view. Their sound-source sizes are rather small in comparison with the wavelength so that beam control should be difficult according to textbook sonar theories. Here, we demonstrate that the multiphase material structure in a porpoise’s forehead is the key to manipulating the directional acoustic field. Computed tomography (CT) derives the multiphase (bone-air-tissue) complex, tissue experiments obtain the density and sound-velocity multiphase gradient distributions, and acoustic fields and beam formation are numerically simulated. The results suggest the control of wave propagations and sound-beam formations is realized by cooperation of the whole forehead’s tissues and structures. The melon size significantly impacts the side lobes of the beam and slightly influences the main beams, while the orientation of the vestibular sac mainly adjusts the main beams. By compressing the forehead complex, the sound beam can be expanded for near view. The porpoise’s biosonar allows effective wave manipulations for its omnidirectional sound source, which can help the future development of miniaturized biomimetic projectors in underwater sonar, medical ultrasonography, and other ultrasonic imaging applications.

We propose two transistor concepts based on lateral heterostructures of monolayer ${\mathrm{MoS}}_2$, composed of adjacent regions of $1T$ (metallic) and $2H$ (semiconducting) phases, inspired by recent research showing the possibility to obtain such heterostructures by electron-beam irradiation. The first concept, the lateral heterostructure field-effect transistor, exhibits the potential of better performance with respect to the foreseen evolution of CMOS technology, both for high-performance and low-power applications. Performance potential is evaluated by means of detailed multiscale materials and device simulations. The second concept, the planar barristor, also exhibits potential competitive performance with CMOS, and an improvement of orders of magnitude in terms of the main figures of merit with respect to the recently proposed vertical barristor.