Single photon detection is a key resource for sensing at the quantum limit and the enabling technology for measurement-based quantum computing. Photon detection at optical frequencies relies on irreversible photoassisted ionization of various natural materials. However, microwave photons have energies 5 orders of magnitude lower than optical photons, and are therefore ineffective at triggering measurable phenomena at macroscopic scales. Here, we report the observation of a new type of interaction between a single two-level system (qubit) and a microwave resonator. These two quantum systems do not interact coherently; instead, they share a common dissipative mechanism to a cold bath: the qubit irreversibly switches to its excited state if and only if a photon enters the resonator. We have used this highly correlated dissipation mechanism to detect itinerant photons impinging on the resonator. This scheme does not require any prior knowledge of the photon waveform nor its arrival time, and dominant decoherence mechanisms do not trigger spurious detection events (dark counts). We demonstrate a detection efficiency of 58% and a record low dark count rate of 1.4 per millisecond. This work establishes engineered nonlinear dissipation as a key enabling resource for a new class of low-noise nonlinear microwave detectors.

Black-hole solutions to general relativity carry a thermodynamic entropy, discovered by Bekenstein and Hawking to be proportional to the area of the event horizon, at leading order in the semiclassical expansion. In a theory of quantum gravity, black holes must constitute ensembles of quantum microstates whose large number accounts for the entropy. We study this issue in the context of gravity with a negative cosmological constant. We exploit the most basic example of the holographic description of gravity ($\mathrm{AdS}/\mathrm{CFT}$): type IIB string theory on ${\mathrm{AdS}}_5\times S^5$, equivalent to maximally supersymmetric Yang-Mills theory in four dimensions. We thus resolve a long-standing question: Does the four-dimensional $\mathcal{N}=4$ $\mathrm{SU}(N)$ Super-Yang-Mills theory on $S^3$ at large $N$ contain enough states to account for the entropy of rotating electrically charged supersymmetric black holes in 5D anti–de Sitter space? Our answer is positive. By reconsidering the large $N$ limit of the superconformal index, using the so-called Bethe-ansatz formulation, we find an exponentially large contribution which exactly reproduces the Bekenstein-Hawking entropy of the black holes. Besides, the large $N$ limit exhibits a complicated structure, with many competing exponential contributions and Stokes lines, hinting at new physics. Our method opens the way toward a quantitative study of quantum properties of black holes in anti–de Sitter space.

Phonon polaritons localized in polar nanoresonators and superlattices are being actively investigated as promising platforms for midinfrared nanophotonics. Here we show that the nonlocal nature of the phonon response can strongly modify their nanoscale physics. Using a nonlocal dielectric approach, we study dielectric nanospheres and thin dielectric films taking into account optical phonons dispersion. We discover a rich nonlocal phenomenology, qualitatively different from the one of plasmonic systems. Our theory allows us to explain the recently reported discrepancy between theory and experiments in atomic-scale superlattices, and it provides a practical tool for the design of phonon-polariton nanodevices.

Far-from-equilibrium dynamics that lead to self-organization are highly relevant to complex dynamical systems not only in physics but also in life, earth, and social sciences. However, it is challenging to find systems with sufficiently controllable parameters that allow quantitatively modeling of emergent properties. Here, we study a nonequilibrium phase transition and observe signatures of self-organized criticality in a dilute thermal vapor of atoms optically excited to strongly interacting Rydberg states. Electromagnetically induced transparency provides excellent control over the population dynamics and enables high-resolution probing of the driven-dissipative dynamics, which also exhibits phase bistability. Increased sensitivity compared to previous work allows us to reconstruct the complete phase diagram, including in the vicinity of the critical point. We observe that interaction-induced energy shifts and enhanced decay only occur in one of the phases above a critical Rydberg population. This case limits the application of generic mean-field models; however, a modified, threshold-dependent approach is in qualitative agreement with experimental data. Near threshold, we observe self-organized dynamics in the form of population jumps that return the density to a critical value.

A microwave amplifier combining noise performances as close as possible to the quantum limit with large bandwidth and high saturation power is highly desirable for many solid-state quantum technologies. Here, we introduce a new traveling-wave parametric amplifier based on superconducting quantum interference devices. It displays a 3-GHz bandwidth, a $-100$-dBm saturation (1-dB compression) point and added noise near the quantum limit. Compared to the previous state of the art, it is an order of magnitude more compact, its characteristic impedance is in situ tunable, and its fabrication process requires only two lithography steps. The key is the engineering of a gap in the dispersion relation of the transmission line. This is obtained using a periodic modulation of the SQUID size, similarly to what is done with photonic crystals. Moreover, we provide a new theoretical treatment to describe the nontrivial interplay between nonlinearity and such periodicity. Our approach provides a path to cointegration with other quantum devices such as qubits given the low footprint and easy fabrication of our amplifier.

Two-dimensional semiconductors provide an ideal platform for exploration of linear exciton and polariton physics, primarily due to large exciton binding energy and strong light-matter coupling. These features, however, generically imply reduced exciton-exciton interactions, hindering the realization of active optical devices such as lasers or parametric oscillators. Here, we show that electrical injection of itinerant electrons into monolayer molybdenum diselenide allows us to overcome this limitation: dynamical screening of exciton-polaritons by electrons leads to the formation of new quasiparticles termed polaron-polaritons that exhibit unexpectedly strong interactions as well as optical amplification by Bose-enhanced polaron-electron scattering. To measure the nonlinear optical response, we carry out time-resolved pump-probe measurements and observe polaron-polariton interaction enhancement by a factor of 50 ($0.5\mu \mathrm{eV}\mu {\mathrm{m}}^2$) as compared to exciton-polaritons. Concurrently, we measure a spectrally integrated transmission gain of the probe field of $\gtrsim 2$ stemming from stimulated scattering of polaron-polaritons. We show theoretically that the nonequilibrium nature of optically excited quasiparticles favors a previously unexplored interaction mechanism stemming from a phase-space filling in the screening cloud, which provides an accurate explanation of the strong repulsive interactions observed experimentally. Our findings show that itinerant electron-exciton interactions provide an invaluable tool for electronic manipulation of optical properties, demonstrate a new mechanism for dramatically enhancing polariton-polariton interactions, and pave the way for realization of nonequilibrium polariton condensates.

Thin elastic solids are easily deformed into a myriad of three-dimensional shapes, which may contain sharp localized structures as in a crumpled candy wrapper or have smooth and diffuse features like the undulating edge of a flower. Anticipating and controlling these morphologies is crucial to a variety of applications involving textiles, synthetic skins, and inflatable structures. Here, we show that a “wrinkle-to-crumple” transition, previously observed in specific settings, is a ubiquitous response for confined sheets. This unified picture is borne out of a suite of model experiments on polymer films confined to liquid interfaces with spherical, hyperbolic, and cylindrical geometries, which are complemented by experiments on macroscopic membranes inflated with gas. We use measurements across this wide range of geometries, boundary conditions, and length scales to quantify several robust morphological features of the crumpled phase, and we build an empirical phase diagram for crumple formation that disentangles the competing effects of curvature and compression. Our results suggest that crumples are a generic microstructure that emerge at large curvatures due to a competition of elastic and substrate energies.

Both helium and ammonia are main components of icy giant planets. While ammonia is very reactive, helium is the most inert element in the universe. It is of great interest whether ammonia and helium can react with each other under planetary conditions, and if so, what kinds of structures and states of matter can form. Here, using crystal structure prediction methods and first-principles calculations, we report three new stable stoichiometries and eight new stable phases of $\mathrm{He}\text{−}{\mathrm{NH}}_3$ compounds under pressures up to 500 GPa. These structures may exhibit perovskitelike structures for ${\mathrm{HeNH}}_3$ and ${\mathrm{He}}_2{\mathrm{NH}}_3$, and a host-guest crystal structure for $\mathrm{He}{({\mathrm{NH}}_3)}_2$. Superionic states are found in all these $\mathrm{He}\text{−}{\mathrm{NH}}_3$ compounds under high pressures and temperatures in which the hydrogen atoms are diffusive while the nitrogen and helium atoms remain fixed. Such dynamical behavior in helium ammonia compounds is quite different from that in helium water compounds, where weakly interacting helium is more diffusive than stronger bound hydrogen. The low-density host-guest phase of space group $I4cm$ is found to be stable at very low pressures (about 3 GPa) and it enters into a plastic state, characterized by freely rotating ammonia molecules. The present results suggest that plastic or superionic helium ammonia compounds may exist under planetary conditions, and helium contributes crucially to the exotic physics and chemistry observed under extreme conditions.

Unraveling the structure and function of the brain requires a detailed knowledge about the neuronal connections, i.e., the spatial architecture of the nerve fibers. One of the most powerful histological methods to reconstruct the three-dimensional nerve fiber pathways is 3D-polarized light imaging (3D-PLI). The technique measures the birefringence of histological brain sections and derives the spatial fiber orientations of whole human brain sections with micrometer resolution. However, the technique yields only a single fiber orientation for each measured tissue voxel even if it is composed of fibers with different orientations, so that in-plane crossing fibers are misinterpreted as out-of-plane fibers. When generating a detailed model of the three-dimensional nerve fiber architecture in the brain, a correct detection and interpretation of nerve fiber crossings is crucial. Here, we show how light scattering in transmission microscopy measurements can be leveraged to identify nerve fiber crossings in 3D-PLI data and demonstrate that measurements of the scattering pattern can resolve the substructure of brain tissue like the crossing angles of the nerve fibers. For this purpose, we develop a simulation framework that permits the study of transmission microscopy measurements—in particular, light scattering—on large-scale complex fiber structures like brain tissue, using finite-difference time-domain (FDTD) simulations and high-performance computing. The simulations are used not only to model and explain experimental observations, but also to develop new analysis methods and measurement techniques. We demonstrate in various experimental studies on brain sections from different species (rodent, monkey, and human) and in FDTD simulations that the polarization-independent transmitted light intensity (transmittance) decreases significantly (by more than 50%) with an increasing out-of-plane angle of the nerve fibers and that it is mostly independent of the in-plane crossing angle. Hence, the transmittance can be used to distinguish regions with low fiber density and in-plane crossing fibers from regions with out-of-plane fibers, solving a major problem in 3D-PLI and allowing for a much better reconstruction of the complex nerve fiber architecture in the brain. Finally, we show that light scattering (oblique illumination) in the visible spectrum reveals the underlying structure of brain tissue like the crossing angle of the nerve fibers with micrometer resolution, enabling an even more detailed reconstruction of nerve fiber crossings in the brain and opening up new fields of research.

Exploring new parameter regimes to realize and control novel phases of matter has been a main theme in modern condensed matter physics research. The recent discovery of two-dimensional (2D) magnetism in nearly freestanding monolayer atomic crystals has already led to observations of a number of novel magnetic phenomena absent in bulk counterparts. Such intricate interplays between magnetism and crystalline structures provide ample opportunities for exploring quantum phase transitions in this new 2D parameter regime. Here, using magnetic field- and temperature-dependent circularly polarized Raman spectroscopy of phonons and magnons, we map out the phase diagram of chromium triiodide (${\mathrm{CrI}}_3$) that has been known to be a layered antiferromagnet (AFM) in its 2D films and a ferromagnet (FM) in its three-dimensional (3D) bulk. However, we reveal a novel mixed state of layered AFM and FM in 3D ${\mathrm{CrI}}_3$ bulk crystals where the layered AFM survives in the surface layers, and the FM appears in deeper bulk layers. We then show that the surface-layered AFM transits into the FM at a critical magnetic field of 2 T, similar to what was found in the few-layer case. Interestingly, concurrent with this magnetic phase transition, we discover a first-order structural phase transition that alters the crystallographic point group from $C_{3i}$ (rhombohedral) to $C_{2h}$ (monoclinic). Our result not only unveils the complex single-magnon behavior in 3D ${\mathrm{CrI}}_3$, but it also settles the puzzle of how ${\mathrm{CrI}}_3$ transits from a bulk FM to a thin-layered AFM semiconductor, despite recent efforts in understanding the origin of layered AFM in ${\mathrm{CrI}}_3$ thin layers, and reveals the intimate relationship between the layered AFM-to-FM and the crystalline rhombohedral-to-monoclinic phase transitions. These findings further open opportunities for future 2D magnet-based magnetomechanical devices.

We employ machine learning techniques to provide accurate variational wave functions for matrix quantum mechanics, with multiple bosonic and fermionic matrices. The variational quantum Monte Carlo method is implemented with deep generative flows to search for gauge-invariant low-energy states. The ground state (and also long-lived metastable states) of an $\mathrm{SU}(N)$ matrix quantum mechanics with three bosonic matrices, and also its supersymmetric “mini-BMN” extension, are studied as a function of coupling and $N$. Known semiclassical fuzzy sphere states are recovered, and the collapse of these geometries in more strongly quantum regimes is probed using the variational wave function. We then describe a factorization of the quantum mechanical Hilbert space that corresponds to a spatial partition of the emergent geometry. Under this partition, the fuzzy sphere states show a boundary-law entanglement entropy in the large $N$ limit.

Measuring the magnetic response of matter relies acutely on the degree to which a magnetic field source’s amplitude, spatial, and temporal character can be tailored. Magnetic fields are inseparable from light-matter interaction, yet due to the dominance of electric-field-induced effects in many systems, laser pulses have heretofore provided comparatively limited insight into the high-frequency magnetic response of matter. Conductors or superconductors arranged in a solenoidal configuration embody the state-of-the-art apparatus for generating spatially isolated magnetic fields, but the reliance on electrical circuitry limits the field amplitude, pulse brevity, and absolute timing of the generated fields. We transfer the concept of solenoidal currents commonly leveraged in electromagnets to photo-ionized electrons driven by moderately intense vector laser beams, in a scheme that does not require the laser mode to carry orbital angular momentum. We predict that this all-optical approach will enable magnetic fields exceeding 8 Tesla to be turned on within 50 femtoseconds using moderate laser intensities, an unprecedented combination of parameters that will open the possibility for ultrafast metrological techniques to be combined with intense, spatially isolated, magnetic fields.

Betatron x-ray sources from laser-plasma accelerators reproduce the principle of a synchrotron at the millimeter scale. They combine compactness, femtosecond pulse duration, broadband spectrum, and micron source size. However, when produced with terawatt class femtosecond lasers, their energy and flux are not sufficient to compete with synchrotron sources, thus limiting their dissemination and its possible applications. Here we present a simple method to enhance the energy and the flux of betatron sources without increasing the laser energy. The orbits of the relativistic electrons emitting the radiation were controlled using density tailored plasmas so that the energetic efficiency of the betatron source is increased by more than one order of magnitude.

It is widely assumed that photons cannot be manipulated using electric or magnetic fields. Even though hybridization of photons with electronic polarization to form exciton-polaritons has paved the way to a number of groundbreaking experiments in semiconductor microcavities, the neutral bosonic nature of these quasiparticles has severely limited their response to external gauge fields. Here, we demonstrate polariton acceleration by external electric and magnetic fields in the presence of nonperturbative coupling between polaritons and itinerant electrons, leading to formation of new quasiparticles termed polaron-polaritons. We identify the generation of electron density gradients by the applied fields to be primarily responsible for inducing a gradient in polariton energy, which in turn leads to acceleration along a direction determined by the applied fields. Remarkably, we also observe that different polarization components of the polaritons can be accelerated in opposite directions when the electrons are in $\nu =1$ integer quantum Hall state.

There is much interest in employing terahertz (THz) radiation across a range of imaging applications, but so far, technologies have struggled to achieve the necessary frame rates. Here, we demonstrate a THz imaging system based upon efficient THz-to-optical conversion in atomic vapor, where full-field images can be collected at ultrahigh speeds using conventional optical camera technology. For a 0.55-THz field, we show an effective $1\text{−}{\mathrm{cm}}^2$ sensor with near diffraction-limited spatial resolution and a minimum detectable power of $(190\pm 30)\mathrm{fW}{\mathrm{s}}^{-1/2}$ per $(40\times 40)\mu {\mathrm{m}}^2$ pixel capable of video capture at 3000 frames per second. This combination of speed and sensitivity represents a step change in the state of the art of THz imaging and will likely lead to its uptake in wider industrial settings.

Quantum field theory is a powerful tool to describe the relevant physics governing complex quantum many-body systems. Here, we develop a general pathway to extract the irreducible building blocks of quantum field theoretical descriptions and its parameters purely from experimental data. This determination is accomplished by extracting the one-particle irreducible (1PI) correlation functions from which one can construct all physical observables. To match the capabilities of experimental techniques, our approach employs a formulation of quantum field theory based on equal-time correlation functions only. We illustrate the theoretical foundations of our procedure by applying it to the sine-Gordon model in thermal equilibrium and then demonstrate explicitly how to extract these quantities from an experiment where we quantum simulate the sine-Gordon model by two tunnel-coupled superfluids. We extract all 1PI correlation functions up to the 1PI four-point function (interaction vertex) and their variation with momentum, encoding the “running” of the couplings. The measured 1PI correlation functions are compared to the theoretical estimates, verifying our procedure. Our work opens new ways of addressing complex many-body questions emerging in a large variety of settings from fundamental science to practical quantum technology.

Quantum probes are atomic sized devices mapping information of their environment to quantum-mechanical states. By improving measurements and at the same time minimizing perturbation of the environment, they form a central asset for quantum technologies. We realize spin-based quantum probes by immersing individual Cs atoms into an ultracold Rb bath. Controlling inelastic spin-exchange processes between the probe and bath allows us to map motional and thermal information onto quantum-spin states. We show that the steady-state spin population is well suited for absolute thermometry, reducing temperature measurements to detection of quantum-spin distributions. Moreover, we find that the information gain per inelastic collision can be maximized by accessing the nonequilibrium spin dynamic. Keeping the motional degree of freedom thermalized, individual spin-exchange collisions yield information about the gas quantum by quantum. We find that the sensitivity of this nonequilibrium quantum probing effectively beats the steady-state Cramér-Rao limit by almost an order of magnitude, while reducing the perturbation of the bath to only three quanta of angular momentum. Our work paves the way for local probing of quantum systems at the Heisenberg limit, and moreover, for optimizing measurement strategies via control of nonequilibrium dynamics.

Evaluating the nonlinear dynamics of human descending thoracic aortas is essential for building the next generation of vascular prostheses. This study characterizes the nonlinear dynamics, viscoelastic material properties, and fluid-structure interaction of 11 ex-vivo human descending thoracic aortas the full range of physiological heart rates. The aortic segments are harvested from heart-beating donors screened for transplants. A mock circulatory loop is developed to reproduce physiological pulsatile pressure and flow. The results show cyclic axisymmetric diameter changes, which are satisfactorily compared to in-vivo measurements at a resting pulse rate of 60 bpm, with an additional bending vibration. An increase of the dynamic stiffness (i.e., storage modulus) with age is also observed. This increase is accompanied by a strong reduction with age of the cyclic diameter change during the heart pulsation at 60 bpm and by a significant reduction of the loss factor (i.e., damping). Large dissipation is observed at higher pulse rates due to the combined effects of fluid-structure interaction and viscoelasticity of the aortic wall. This study presents data necessary for developing innovative grafts that better mimic the dynamics of the aorta.

Proposals for experiments in quantum chemistry on quantum computers leverage the ability to target a subset of degrees of freedom containing the essential quantum behavior, sometimes called the active space. This approximation allows one to treat more difficult problems using fewer qubits and lower gate depths than would otherwise be possible. However, while this approximation captures many important qualitative features, it may leave the results wanting in terms of absolute accuracy (basis error) of the representation. In traditional approaches, increasing this accuracy requires increasing the number of qubits and an appropriate increase in circuit depth as well. Here we explore two techniques requiring no additional qubits or circuit depth that are able to remove much of this approximation in favor of additional measurements. The techniques are constructed and analyzed theoretically, and some numerical proof-of-concept calculations are shown. As an example, we show how to achieve the accuracy of a 20-qubit representation using only four qubits and a modest number of additional measurements for a hydrogen molecule. We close with an outlook on the impact such techniques may have on both near-term and fault-tolerant quantum simulations.

A statistical theory of rogue waves is proposed and tested against experimental data collected in a long water tank where random waves with different degrees of nonlinearity are mechanically generated and free to propagate along the flume. Strong evidence is given that the rogue waves observed in the tank are hydrodynamic instantons, that is, saddle point configurations of the action associated with the stochastic model of the wave system. As shown here, these hydrodynamic instantons are complex spatiotemporal wave field configurations which can be defined using the mathematical framework of large deviation theory and calculated via tailored numerical methods. These results indicate that the instantons describe equally well rogue waves created by simple linear superposition (in weakly nonlinear conditions) or by nonlinear focusing (in strongly nonlinear conditions), paving the way for the development of a unified explanation to rogue wave formation.