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Spectroscopy and Ground-State Transfer of Ultracold Bosonic Molecules
Phys. Rev. Lett. 135, 203401 – Published 12 November, 2025Erratum Phys. Rev. Lett. 136, 249902 (2026)
DOI: https://doi.org/10.1103/gjzh-8dsb
Abstract
We report the creation of ultracold samples of molecules in their rovibrational ground state. By investigating potentially suitable excited states using one- and two-photon spectroscopy, we have identified a pathway to the ground state via an exceptionally narrow intermediate state. Using stimulated Raman adiabatic passage, we create trapped samples of up to 3500 molecules at temperatures of with one-way efficiencies of 71%. The lifetime of these samples is limited by a near-universal two-body loss process, which could shed new light on similar loss mechanisms in other molecular species. Our results are a step toward establishing an alternative molecular species as a platform for the study of bosonic and fermionic quantum matter with strong dipolar interactions.
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Erratum
Erratum: Spectroscopy and Ground-State Transfer of Ultracold Bosonic Molecules [Phys. Rev. Lett. 135, 203401 (2025)]
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References (71)
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