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Force-induced breakdown of flexible polymerized membrane
Phys. Rev. E 85, 021805 – Published 21 February, 2012
DOI: https://doi.org/10.1103/PhysRevE.85.021805
Abstract
We consider the fracture of a free-standing two-dimensional (2D) elastic-brittle network to be used as protective coating subject to constant tensile stress applied on its rim. Using a molecular-dynamics simulation with a Langevin thermostat, we investigate the scission and recombination of bonds, and the formation of cracks in the 2D graphenelike hexagonal sheet for different pulling force and temperature . We find that bond rupture occurs almost always at the sheet periphery, and the first mean breakage time of bonds decays with membrane size as , where and denotes the number of atoms in the membrane. The probability distribution of bond scission times is given by a Poisson function . The mean failure time necessary to rip off the sheet declines with growing size as a power law . We also find , where the nucleation barrier for crack formation , in agreement with Griffith's theory. displays an Arrhenian dependence of on temperature . Our results indicate a rapid increase in crack spreading velocity with growing external tension .
Article Text
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