Export citation

Export citation

Choose format for download:

Download Citation
  • Access by Xinjiang University

Near-Threshold Photoemission from Graphene-Coated Cu(110)

Christopher J. Knill1,*, Hisato Yamaguchi2, Kenji Kawahara3, Gaoxue Wang2, Enrique Batista2, Ping Yang2, Hiroki Ago3, Nathan Moody2, and Siddharth Karkare1,†

  • 1Department of Physics, Arizona State University, Tempe, Arizona 85287, USA
  • 2Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
  • 3Global Innovation Center, Kyushu University, Kasuga, Fukuoka 816-8580, Japan

  • *Authors to whom correspondence should be addressed: cknill2@asu.edu
  • Authors to whom correspondence should be addressed: karkare@asu.edu

Phys. Rev. Applied 19, 014015 – Published 5 January, 2023

DOI: https://doi.org/10.1103/PhysRevApplied.19.014015

Abstract

The brightness of electron beams emitted from photocathode sources plays a critical role in determining the performance of x-ray free-electron lasers and ultrafast electron-diffraction applications. In order to achieve the maximum brightness, the electrons need to be emitted from a photocathode with the lowest-possible mean transverse energy (MTE). Recent investigations have shown that capping a Cu(110) photocathode with a monolayer of graphene can protect the quantum efficiency (QE) from long-term exposure to varying vacuum conditions. However, there have been no studies that investigate the effects that a monolayer of graphene has on the MTE. Here, we report on measurements of a graphene-coated Cu(110) single crystal near the photoemission threshold for room and liquid-nitrogen temperatures. At room temperature, a minimum MTE of 25 meV is measured at 295 nm. At liquid-nitrogen temperatures, a minimum MTE of 9 meV is measured at the photoemission threshold of 290 nm.

Physics Subject Headings (PhySH)

Corrections

20 January, 2023

Correction: Two support statements were missing from the Acknowledgment section and have been inserted.

Article Text

References (34)

  1. A. A. Ischenko, P. M. Weber, and R. J. D. Miller, Capturing chemistry in action with electrons: Realization of atomically resolved reaction dynamics, Chem. Rev. 117, 11066 (2017).
  2. B. J. Siwick, J. R. Dwyer, R. E. Jordan, and R. J. D. Miller, Ultrafast electron optics: Propagation dynamics of femtosecond electron packets, J. Appl. Phys. 92, 1643 (2002).
  3. M. Ferrario, Overview of FEL injectors, Proceedings of EPAC, Edinburgh, Scotland (2015).
  4. J. B. Rosenzweig, et al., An ultra-compact x-ray free electron laser, New J. Phys. 22, 093067 (2020).
  5. P. Musumeci, J. T. Moody, C. Scoby, M. S. Gutierrez, H. A. Bender, and N. S. Wilcox, High quality single shot diffraction patterns using ultrashort mega-electron volt electron beams from a radio frequency photoinjector, Rev. Sci. Instrum. 81, 013306 (2010).
  6. F. Ji, D. Durham, A. Minor, P. Musumeci, J. Navarro, and D. Filippetto, Ultrafast relativistic electron nanoprobes, Nat. Comm. Phys. 2, 54 (2019).
  7. A. R. Bainbridge, C. W. B. Myers, and W. A. Bryan, Femtosecond few-to single-electron point-projection microscopy for nanoscale dynamic imaging, Struct. Dyn. 3, 023612 (2016).
  8. I. V. Bazarov, B. M. Dunham, and C. K. Sinclair, Maximum Achievable Brightness from Photoinjectors, Phys. Rev. Lett. 102, 104801 (2009).
  9. S. A. Aseyev, E. A. Ryabov, B. N. Mironov, and A. A. Ischenko, The development of ultrafast electron microscopy, Crystals 10, 452 (2020).
  10. N. R. da Silva, M. Moller, A. Feist, H. Ulrichs, C. Ropers, and S. Schafer, Nanoscale Mapping of Ultrafast Magnetization Dynamics with Femtosecond Lorentz Microscopy, Phys. Rev. X 8, 031052 (2018).
  11. F. Carbone, O. Kwon, and A. H. Zewail, Dynamics of chemical bonding mapped by energy-resolved 4D electron microscopy, Science 325, 181 (2009).
  12. B. Barwick, H. Park, O. Kwon, J. Baskin, and A. H. Zewail, 4D imaging of transient structures and morphologies in ultrafast electron microscopy, Science 322, 1227 (2008).
  13. P. Musumeci, J. Navarro, J. B. Rosenzweig, L. Cultrera, I. Bazarov, J. Maxson, S. Karkare, and H. Padmore, Advances in bright electron sources, Nucl. Instrum. Meth. A 907, 208 (2018).
  14. D. H. Dowell and J. Schmerge, Quantum efficiency and thermal emittance of metal photocathodes, Phys. Rev. ST Accel. Beams 12, 074201 (2009).
  15. T. Vecchione, D. Dowell, W. Wan, J. Feng, and H. A. Padmore, Quantum efficiency and transverse momentum from metals, Proceedings of FEL2013, Geneva, Switzerland, 4242013.
  16. J. Feng, S. Karkare, J. Nasiatka, S. Schubert, J. Smedley, and H. A. Padmore, Near atomically smooth alkali antimonide photocathode thin films, J. Appl. Phys. 121, 044904 (2017).
  17. S. Karkare, G. Adhikari, W. A. Schroeder, J. K. Nangoi, T. Arias, J. M. Maxson, and H. A. Padmore, Ultracold Electrons via Near-Threshold Photoemission from Single-Crystal Cu(100), Phys. Rev. Lett. 125, 054801 (2020).
  18. L. Cultrera, S. Karkare, H. Lee, X. Liu, I. Bazarov, and B. Dunham, Cold electron beams from cryocooled, alkali antimonide photocathodes, Phys. Rev. ST Accel. Beams 18, 113401 (2015).
  19. W. A. Schroeder and G. Adhikari, Evaluation of photocathode emission properties in an electron gun: One-step photoemission from bulk band to vacuum states, New J. Phys. 21, 033040 (2019).
  20. S. Karkare and I. Bazarov, Effects of Surface Nonuniformities on the Mean Transverse Energy from Photocathodes, Phys. Rev. Appl. 4, 024015 (2015).
  21. G. Gevorkyan, S. Karkare, S. Emamian, I. V. Bazarov, and H. A. Padmore, Effects of physical and chemical surface roughness on the brightness of electron beams from photocathodes, Phys. Rev. Accel. Beams 21, 093401 (2018).
  22. S. Karkare, J. Feng, X. Chen, W. Wan, F. J. Palomares, T.-C. Chiang, and H. A. Padmore, Reduction of Intrinsic Electron Emittance from Photocathodes Using Ordered Crystalline Surfaces, Phys. Rev. Lett. 118, 164802 (2017).
  23. C. J. Knill, H. A. Padmore, and S. S. Karkare, Near-threshold nonlinear photoemission from Cu(100), Proceedings of the 12th International Particle Accelerator Conference, Sao Paulo, Brazil, WEPAB099 (2021).
  24. J. Bae, L. Cultrera, I. V. Bazarov, J. M. Maxson, S. Karkare, and H. A. Padmore, Multi-photon photoemission and ultrafast electron heating in Cu photocathodes, Proceedings of the 9th International Particle Accelerator Conference, Vancouver, Canada, TUPML0262018.
  25. J. M. Maxson, P. Musumeci, L. Cultrera, S. Karkare, and H. A. Padmore, Ultrafast laser pulse heating of metallic photocathodes and its contribution to intrinsic emittance, Nucl. Instrum. Meth. A 865, 99 (2017).
  26. B. Dunham, et al., Record high average current from a high-brightness photoinjector, Appl. Phys. Lett. 102, 034105 (2013).
  27. H. Yamaguchi, F. Liu, J. DeFazio, C. W. N. Villarrubia, D. Finkenstadt, A. Shabaev, K. L. Jensen, V. Pavlenko, M. Mehl, S. Lambrakos, G. Gupta, A. D. Mohite, and N. A. Moody, Active bialkali photocathodes on free-standing graphene substrates, npj 2D Mater. Appl. 1, 12 (2017).
  28. H. Yamaguchi, F. Liu, J. DeFazio, M. Gaowei, C. W. N. Villarrubia, J. Xie, V. Pavlenko, K. L. Jensen, J. Smedley, A. D. Mohite, and N. A. Moody, Free-standing bialkali photocathodes using atomically thin substrates, Adv. Mater. Inter. 5, 1800249 (2018).
  29. F. Liu, L. Guo, J. DeFazio, V. Pavlenko, M. Yamamoto, N. A. Moody, and H. Yamaguchi, Photoemission from bialkali photocathodes through an atomically thin protection layer, ACS Appl. Mater. Inter. 14, 1710 (2022).
  30. F. Liu, N. A. Moody, K. L. Jensen, V. Pavlenko, C. W. N. Villarrubia, A. D. Mohite, and G. Gupta, Single layer graphene protective gas barrier for copper photocathodes, Appl. Phys. Lett. 110, 041607 (2017).
  31. C. J. Knill, H. Yamaguchi, K. Kawahara, G. Wang, E. Batista, P. Yang, H. Ago, N. A. Moody, and S. S. Karkare, Near threshold photoemission from graphene coated Cu single crystals, Proceedings of the 3rd North American Particle Accelerator Conference, Albuquerque, NM, USA, WEPA66 (2022).
  32. H. Ago, K. Kawahara, Y. Ogawa, S. Tanoue, M. A. Bissett, M. Tsuji, H. Sakaguchi, R. J. Koch, F. Fromm, T. Seyller, K. Komatsu, and K. Tsukagoshi, Epitaxial growth and electronic properties of large hexagonal graphene domains on Cu(111) thin film, Appl. Phys. Exp. 6, 075101 (2013).
  33. N. R. Wilson, A. J. Marsden, M. Saghir, C. J. Bromley, R. Schaub, G. Costantini, T. W. White, C. Partridge, A. Barinov, P. Dudin, A. M. Sanchez, J. J. Mudd, M. Walker, and G. R. Bell, Weak mismatch epitaxy and structural feedback in graphne growth on copper foil, Nano Res. 6, 99 (2013).
  34. S. Karkare, J. Feng, J. Maxson, and H. A. Padmore, Development of a 3-D energy-momentum analyzer for meV-scale energy electrons, Rev. Sci. Instrum. 90, 053902 (2019).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation