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Synchrotron radiation techniques and their application to actinide materials

R. Caciuffo*, G. H. Lander, and G. van der Laan

R. Caciuffo*

  • European Commission, Joint Research Centre (JRC), Postfach 2340, DE-76125 Karlsruhe, Germany and Istituto Nazionale di Fisica Nucleare, Via Dodecaneso 33, IT-16146 Genova, Italy

G. H. Lander

  • European Commission, Joint Research Centre (JRC), Postfach 2340, DE-76125 Karlsruhe, Germany and Interface Analysis Centre, School of Physics, University of Bristol, Tyndall Avenue, Bristol BS8 1TL, United Kingdom

G. van der Laan

  • Diamond Light Source, Harwell Science and Innovation Campus, Didcot OX11 0DE, United Kingdom

  • *Corresponding author. roberto.caciuffo@ge.infn.it, rgm.caciuffo@gmail.com
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Rev. Mod. Phys. 95, 015001 – Published 3 March, 2023

DOI: https://doi.org/10.1103/RevModPhys.95.015001

Abstract

Research on actinide materials, both basic and applied, has been greatly advanced by the general techniques available from high-intensity photon beams from x-ray synchrotron sources. The most important single reason is that such x-ray sources can work with minute (e.g., microgram) samples, and at this level the radioactive hazards of actinides are significantly reduced. The form and encapsulation procedures used for different techniques are discussed, followed by the basic theory for interpreting the results. To demonstrate the potential of synchrotron radiation techniques for the study of lattice and electronic structure, hybridization effects, multipolar order, and lattice dynamics in actinide materials, a selection of x-ray diffraction, resonant elastic x-ray scattering, x-ray magnetic circular dichroism, resonant and nonresonant inelastic scattering, dispersive inelastic x-ray scattering, and conventional and resonant photoemission experiments are reviewed.

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Rev. Mod. Phys. 95, 015001– Published 3 March, 2023
  • Received 23 June 2022
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