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Inelastic light scattering from correlated electrons

Thomas P. Devereaux* and Rudi Hackl†

Thomas P. Devereaux*

  • Department of Physics, University of Waterloo, Waterloo, ON, Canada N2L 3G1

Rudi Hackl†

  • Walther Meissner Institute, Bavarian Academy of Sciences, D-85748 Garching, Germany

  • *Electronic address: tpd@uwaterloo.ca
  • †Electronic address: hackl@wmi.badw.de
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Rev. Mod. Phys. 79, 175 – Published 31 January, 2007

DOI: https://doi.org/10.1103/RevModPhys.79.175

Abstract

Inelastic light scattering is an intensively used tool in the study of electronic properties of solids. Triggered by the discovery of high-temperature superconductivity in the cuprates and by new developments in instrumentation, light scattering in both the visible (Raman effect) and x-ray part of the electromagnetic spectrum has become a method complementary to optical (infrared) spectroscopy while providing additional and relevant information. The main purpose of the review is to position Raman scattering with regard to single-particle methods like angle-resolved photoemission spectroscopy, and other transport and thermodynamic measurements in correlated materials. Particular focus will be placed on photon polarizations and the role of symmetry to elucidate the dynamics of electrons in different regions of the Brillouin zone. This advantage over conventional transport (usually measuring averaged properties) provides new insights into anisotropic and complex many-body behavior of electrons in various systems. Recent developments in the theory of electronic Raman scattering in correlated systems and experimental results in paradigmatic materials such as the A15 superconductors, magnetic and paramagnetic insulators, compounds with competing orders, as well as the cuprates with high superconducting transition temperatures are reviewed. An overview of the manifestations of complexity in the Raman response due to the impact of correlations and developing competing orders is presented. In a variety of materials, observations which may be understood and a summary of important open questions that pave the way to a detailed understanding of correlated electron systems, are discussed.

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Rev. Mod. Phys. 79, 175– Published 31 January, 2007

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