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Probing the helium-graphite interaction

Milton W. Cole, D. R. Frankl, and David L. Goodstein

Milton W. Cole and D. R. Frankl

  • Physics Department, The Pennsylvania State University, University Park, Pennsylvania 16802

David L. Goodstein

  • California Institute of Technology, Pasadena, California 91125

Rev. Mod. Phys. 53, 199 – Published 1 April, 1981

DOI: https://doi.org/10.1103/RevModPhys.53.199

Abstract

Two separate lines of investigation have recently converged to produce a highly detailed picture of the behavior of helium atoms physisorbed on graphite basal plane surfaces. Atomic beam scattering experiments on single crystals have yielded accurate values for the binding energies of several states for both He4 and He3, as well as matrix elements of the largest Fourier component of the periodic part of the interaction potential. From these data, a complete three-dimensional description of the potential has been constructed, and the energy band structure of a helium atom moving in this potential calculated. At the same time, accurate thermodynamic measurements were made on submonolayer helium films adsorbed on Grafoil. The binding energy and low-coverage specific heat deduced from these measurements are in excellent agreement with those calculated from the band structures.

References (72)

  1. Ahlrichs, R., R. Penco, and G. Scoles, 1977, Chem. Phys. 19, 119
  2. Bennett, A. J., 1974, Phys. Rev. B 9, 741
  3. Bienfait, M., J. G. Dash, and J. Stoltenberg, 1980, Phys. Rev. B 21, 2765
  4. Boato, G., P. Cantini, and R. Tatarek, 1978, Phys. Rev. Lett. 40, 887
  5. Boato, G. P., P. Cantini, C. Guidi, R. Tatarek, and G. P. Felcher, 1979, Phys. Rev. B 20, 3957
  6. Boato, G. P., P. Cantini, R. Tatarek, and G. P. Felcher, 1979, Surf. Sci. 80, 518
  7. Bonino, G., C. Pisani, F. Ricca, and C. Roetti, 1975, Surf. Sci. 50, 379
  8. Bretz, M., 1977, Phys. Rev. Lett. 38, 501
  9. Bretz, M., and J. G. Dash, 1971, Phys. Rev. Lett. 26, 963
  10. Bretz, M., J. G. Dash, D. C. Hickernell, E. O. McLean, and O. E. Vilches, 1973, Phys. Rev. A 8, 1589
  11. Bruch, L. W., 1981, unpublished
  12. Bruch, L. W., and H. Watanabe, 1977, Surf. Sci. 65, 619
  13. Carlos, W. E., and M. W. Cole, 1978, Surf. Sci. 77, L173
  14. Carlos, W. E., and M. W. Cole, 1980a, Surf. Sci. 91, 339
  15. Carlos, W. E., and M. W. Cole, 1980b, Phys. Rev. B 21, 3713
  16. Carneiro, K., L. Passell, W. Thomlinson, and H. Taub, 1980, Phys. Rev. B (in press)
  17. Celli, V., N. Garcia, and J. Hutchison, 1979, Surf. Sci. 87, 112
  18. Chow, H., 1979, Surf. Sci. 79, 157
  19. Chow, H., and E. D. Thompson, 1976, Surf. Sci. 59, 225
  20. Chow, H., and E. D. Thompson, 1979, Surf. Sci. 82, 1
  21. Cole, M. W., and D. R. Frankl, 1978, Surf. Sci. 70, 585
  22. Cole, M. W., B. Garrison, and W. A. Steele, 1980, (unpublished)
  23. Cole, M. W., and F. Toigo, 1980, submitted to Phys. Rev. B
  24. Dash, J. G., 1968, J. Chem. Phys. 48, 2820
  25. Dash, J. G., and M. Schick, 1979, in The Physics of Liquid and Solid Helium, edited by K. H. Bennemann and J. B. Ketterson (Wiley, New York), Part 2
  26. den Boer, M. L., T. L. Einstein, W. T. Elam, R. L. Park, L. D. Roelofs, and G. E. Laramore, 1980, Phys. Rev. Lett. 44, 496
  27. Derry, G. D., D. Wesner, W. E. Carlos, and D. R. Frankl, 1979, Surf. Sci. 87, 629
  28. Derry, G. N., D. Wesner, G. Vidali, T. Thwaites, and D. R. Frankl, 1980, Surf. Sci. 94, 221
  29. Elgin, R. L., and L. Goodstein, 1974, Phys. Rev. A 9, 2657
  30. Elgin, R. L., J. M. Greif, and D. L. Goodstein, 1978, Phys. Rev. Lett. 41, 1723
  31. Estermann, I., and O. Stern, 1930, Z. Phys. 61, 95
  32. Frankl, D. R., 1980, Crit. Rev. Solid State and Mater. Sci. (to be published)
  33. Frankl, D. R., D. Wesner, S. V. Krishnaswamy, G. Derry, and T. O'Gorman, 1978, Phys. Rev. Lett. 41, 60
  34. Freeman, D. L., 1975, J. Chem. Phys. 62, 941
  35. Frisch, R., and O. Stern, 1933, Z. Phys. 84, 430
  36. Garcia, N., W. E. Carlos, M. W. Cole, and V. Celli, 1980, Phys. Rev. B 21, 1636
  37. Garcia, N., V. Celli, and F. O. Goodman, 1979, Phys. Rev. B 19, 634
  38. Goodman, F. O., 1977, Crit. Rev. Solid State and Mater. Sci. 7, 33
  39. Gordon, R. G., and Y. S. Kim, 1972, J. Chem. Phys. 56, 3122
  40. Grayson, J., and J. G. Aston, 1957, J. Phys. Chem. 61, 610
  41. Hagen, D. E., A. D. Novaco, and F. J. Milford, 1972, in Adsorption Desorption Phenomena, edited by F. Ricca (Academic, London), p. 99
  42. Harvie, C. E., and J. H. Weare, 1978, Phys. Rev. Lett. 40, 187
  43. Hutchison, J., and V. Celli, 1980, Surf. Sci. 93, 263
  44. Landman, U., and G. G. Kleiman, 1977, in Surface and Defect Properties of Solids, Specialist Report of the Chemical Society, London, Vol. 6, p. 1
  45. Lennard-Jones, J. E., and A. F. Devonshire, 1936, Nature 137, 1069
  46. Lennard-Jones, J. E., and A. E. Devonshire, 1937, Proc. R. Soc. London Ser. A 158, 242, 253
  47. Lerner, E., and J. G. Daunt, 1973, J. Low Temp. Phys. 10, 299
  48. Margenau, H., and N. R. Kestner, 1969, Theory of Intermolecular Forces (Pergamon, New York)
  49. McLachlan, A. D., 1964, Mol. Phys. 7, 381
  50. Novaco, A. D., Phys. Rev. B 13, 3194 (1976)
  51. Novaco, A. D., and C. E. Campbell, 1975, Phys. Rev. B 11, 2525
  52. Pendry, J. B., 1974, Low Energy Electron Diffraction (Academic, London)
  53. Polanco, S. E., and M. Bretz, 1980, Surf. Sci. 94, 1
  54. Poshkus, D. P., 1965, Discuss. Faraday Soc. 40, 195
  55. Roth, J. A., G. J. Jelatis, and J. D. Maynard, 1980, Phys. Rev. Lett. 44, 333
  56. Sabisky, E. S., and C. H. Anderson, 1973, Phys. Rev. A 7, 790
  57. Shaw, C. G., and S. C. Fain, Jr., 1979, Surf. Sci. 83, 1
  58. Siddon, R. L., and M. Schick, 1974, Phys. Rev. A 9, 907
  59. Silva-Moreira, A. F., J. Codona, and D. L. Goodstein, 1980, Phys. Lett. A 76, 324
  60. Steele, W. A., 1974, The Interaction of Gases with Solid Surfaces (Pergamon, Oxford)
  61. Steele, W. A., 1980, Surf. Sci. (in press)
  62. Stern, E. A., 1978, Contemp. Phys. 19, 289
  63. Taborek, P., and D. L. Goodstein, 1979, Rev. Sci. Instrum. 50, 227
  64. Thomy, A., and X. Duval, 1969, J. Chim. Phys. Phys.-Chim. Biol. 66, 1966
  65. Thomy, A., and X. Duval, 1970, J. Chim. Phys. Phys.-Chim. Biol. 67, 286 and 1101
  66. van Himbergen, J. E., and R. Silbey, 1977, Solid State Commun. 23, 623
  67. Vidali, G., M. W. Cole, and C. Schwartz, 1979, Surf. Sci. 87, L273
  68. Vidali, G., and M. W. Cole, 1980, Phys. Rev. B 22, 4661
  69. Young, D. M., and A. D. Crowell, 1962, Physical Adsorption of Gases (Butterworth, London)
  70. Zachariasen, W. H., 1945, Theory of X-Ray Diffraction in Crystals (Wiley, New York), p. 85 ff
  71. Zaremba, E., and W. Kohn, 1976, Phys. Rev. B 13, 2270
  72. Zaremba, E., and W. Kohn, 1977, Phys. Rev. B 15, 1769

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