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Tailoring ultrathin magnetic multilayers at terraced topologically insulating interfaces for perpendicularly magnetized domains

Benjamin A. Brereton1,2,3, Soumyarup Hait1, Ahmet Yagmur1, Christy J. Kinane2, Francesco Maccherozzi3, Michele Conroy4, Satoshi Sasaki1, Thomas A. Moore1, Sarnjeet S. Dhesi3 et al.

Sean Langridge2 and Christopher H. Marrows1,*

  • *Contact author: c.h.marrows@leeds.ac.uk
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Phys. Rev. Materials 10, 064413 – Published 24 June, 2026

DOI: https://doi.org/10.1103/hp66-tldh

Abstract

Topological insulators and skyrmion-hosting, chiral magnetic multilayers are two well-explored areas of modern condensed matter physics, each offering unique advantages for spintronics applications. In this paper, we demonstrate the optimization process for the growth of a Bi2Se3/buffer/[Pt/CoB/Ru]×N heterostructure that combines these two material classes: the Bi2Se3 epilayer was grown by molecular beam epitaxy before transfer under ultrahigh vacuum to a separate growth chamber where the polycrystalline metallic multilayer was sputter deposited. The structure of the samples was characterized by cofitted x-ray and polarized neutron reflectometry measurements and scanning transmission electron microscopy. Polarized neutron models and standard magnetometry show that a buffer layer exceeding a critical thickness is required to obtain the desired uniform, perpendicular magnetic anisotropy in every magnetic layer in the multilayer. Samples with both Ta and Mo buffers were used requiring thicknesses of 1.5 and 0.9 nm, respectively. In minimizing the Bi2Se3 terracing, buffered samples yield well-defined, out-of-plane, magnetic domains suitable for spin-orbit torque-induced manipulation as determined by x-ray photoemission electron microscopy.

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Phys. Rev. Materials 10, 064413– Published 24 June, 2026
  • Received 10 February 2026
  • Accepted 20 May 2026
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