• Accepted Paper

Ultrafast cooperative electronic, structural, and magnetic transition in α-MnTe

Tiangao Lu, Ao Wu, Junxiang Li, Qiyuan Wu, Meng Zeng, Di Cheng, Chang Liu, Jiangbin Gong, and Xinwei Li

Phys. Rev. Lett. - Accepted 10 November, 2026

DOI: https://doi.org/10.1103/mlrq-mm6h

Abstract

Femtosecond laser control of antiferromagnetic order is a cornerstone for future memory and logic devices operating at terahertz clock rates. Here, we demonstrate an ultrafast laser-induced phase transition in α-MnTe that simultaneously engages charge, lattice, and spin degrees of freedom. Using time-resolved reflectivity and birefringence measurements, we reveal that photo-induced demagnetization is accompanied by pronounced structural and electronic instabilities, manifesting as a multistage temporal evolution following photoexcitation. The transition uncovers unique spin-charge and spin-lattice coupling pathways, which we discuss in the context of recently proposed altermagnetic phenomenology.

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