- Accepted Paper
Magnetic-field–induced Tomonaga-Luttinger liquid and Bose-Einstein condensate phases in an organic Haldane chain
Phys. Rev. Lett. - Accepted 28 July, 2026
DOI: https://doi.org/10.1103/89k5-p261
Phys. Rev. Lett. - Accepted 28 July, 2026
DOI: https://doi.org/10.1103/89k5-p261
We present a comprehensive low-temperature H nuclear magnetic resonance (NMR) study of magnetic field-induced phases and spin fluctuations in an isotropic Haldane chain system -NOPhBNO (BoNO) in fields up to 34~T. NMR spectral and relaxation rate data are used to map out the transition temperature and we show that it defines a complete phase boundary between the field-induced Bose-Einstein condensate (BEC) and Tomonaga-Luttinger liquid (TLL) phases by reproducing its shape via quantum Monte Carlo calculations. We also observe the theoretical critical behavior with and universal quasiparticle scaling in the low-temperature limit close to . The extensive Bayesian inference analysis of the temperature and field dependence of reveals attractive interactions across the TLL phase of a Haldane chain. Our results are further corroborated by magnetostriction measurements in pulsed magnetic fields and density matrix renormalization group calculations.
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