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Tailoring Superconductivity with Two-Level Systems
Phys. Rev. Lett. 136, 216001 – Published 26 May, 2026
DOI: https://doi.org/10.1103/zdgk-b66f
Abstract
We investigate the impact of two-level systems (TLSs) on superconductivity, treating them as soft modes localized in real space. We show that these defects can either enhance or suppress the superconducting critical temperature, depending on their surface density and average frequency. Using thin-film aluminium as a case study, we quantitatively describe how TLSs modify both the critical temperature and the zero-temperature superconducting gap. Our results thus highlight new opportunities for tailoring material properties through TLS engineering.
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Note that this frequency range corresponds to that of collective vibronic modes resulting from dangling bonds, as discussed in Ref. [70]. While such energies may be directly proportional to the tunnelling amplitudes of TLSs, we do not explicitly incorporate the microscopic specifics of asymmetry energies or tunnelling amplitudes into our study.
Throughout our implementation of Eliashberg theory in the thin-film limit, we note that the Migdal parameter remains small as a consequence of the expected invariance of in the 2D limit [36] and the general anticorrelation between and [73, 90].
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