Export citation

Export citation

Choose format for download:

Download Citation
  • Access by Xinjiang University

Electrocapillary, thermocapillary, and buoyancy convection driven flows in the Melcher-Taylor experimental setup

Alexander Yu. Gelfgat*

Gerrit Maik Horstmann

  • School of Mechanical Engineering, Faculty of Engineering, Tel-Aviv University, Ramat Aviv, Tel-Aviv 6997801, Israel

  • Helmholtz-Zentrum Dresden-Rossendorf, Bautzner Landstrasse 400, 01328 Dresden, Germany

  • *gelfgat@tau.ac.il
  • g.horstmann@hzdr.de

Phys. Rev. Fluids 9, 044101 – Published 12 April, 2024

DOI: https://doi.org/10.1103/PhysRevFluids.9.044101

Abstract

Electrocapillary driven two-phase flows in a confined configuration of a classical experiment of Melcher and Taylor are studied. The computed streamlines of the flow of the heavier dielectric liquid (corn oil) qualitatively represent the corresponding experimental image. With the increase of electrocapillary forcing, the flow pattern changes, so that the main circulation localizes near a boundary with a larger electric potential. When a dielectric liquid is replaced by a poorly conducting one, the system becomes nonisothermal owing to the Joule heating. Then the flow is driven also by buoyancy and thermocapillary convection, whose effect becomes noticeably stronger than the electrocapillary one. With the increase of electric conductivity, the electrocapillary effect is further weakened compared to the two others, while the electrocapillary and thermocapillary forces remain comparable at the central part of the interface. The results show that consideration of the two-phase model is mandatory for obtaining correct flow patterns in the lower, heavier fluid. The Lippmann equation, connecting electrically induced surface tension with nonuniform surface electric potential, is numerically verified for both isothermal and nonisothermal formulations and is found to hold in both of them.

Physics Subject Headings (PhySH)

Article Text

References (72)

  1. J. R. Melcher and G. I. Taylor, Electrodynamics: A review of the role of interfacial shear stresses, Annu. Rev. Fluid Mech. 1, 111 (1969).
  2. A. Y. Gelfgat and I. Tanasawa, Numerical investigation of the thermocapillary drift of a bubble in an electric field, Microgravity Sci. Technol. 8, 16 (1995).
  3. R. Xue, W. Liu, T. Jiang, C. Song, H. Jiang, and T. Ren, Pumping of ionic liquids by liquid metal-enabled electrocapillary flow under dc-biased ac forcing, Adv. Mater. Interfaces 7, 2000345 (2020).
  4. E. Georgiou, D. T. Papageorgiou, C. Maldarelli, and D. S. Rumschitki, The double layer–capillary stability of an annular electrolyte film surrounding a dielelectric–fluid core in a tube, J. Fluid Mech. 226, 149 (1991).
  5. B. S. Tilley, P. G. Petropoulos, and D. T. Papageorgiou, Dynamics and rupture of planar electrified liquid sheets, Phys. Fluids 13, 3547 (2001).
  6. L. F. Pease, III and W. B. Russel, Linear stability analysis of thin leaky dielectric films subjected to electric films, J. Non-Newtonian Fluid Mech. 102, 233 (2002).
  7. D. T. Papageorgiou and J.-M. Vanden-Broeck, Large-amplitude capillary waves in electrified fluid sheets, J. Fluid Mech. 508, 71 (2004).
  8. O. Ozen, D. T. Papageorgiou, and P. G. Petropoulos, Nonlinear stability of a charged electrified liquid sheet under the action of a horizontal electric field, Phys. Fluids 18, 042102 (2006).
  9. J. R. Melcher and W. J. Schwarz, Interfacial relaxation overstability in a tangential electric field, Phys. Fluids 11, 2604 (1968).
  10. R. Aogaki, K. Kitazawa, K. Fueki, and T. Mukaibo, Theory of polarographic maximum current—I. Conditions for the onset of hydrodynamics instability in a liquid metal electrode system, Electrochim. Acta 23, 867 (1978).
  11. R. Aogaki, K. Kitazawa, K. Fueki, and T. Mukaibo, Theory of polarographic maximum current—II. Growth or decay rate of the electrochemical and hydrodynamic instability, Electrochim. Acta 23, 875 (1978).
  12. T. Makino, K. Morioka, and R. Aogaki, Occurrence of cellular convective flow accompanying the polarographic maximum wave of the first kind, J. Electroanal. Chem. Interfacial Electrochem. 190, 261 (1985).
  13. T. Makino and R. Aogaki, Occurrence of regular convection at the liquid-liquid interface of two immiscible electrolyte solutions by resonance with a pulsated potential, J. Electroanal. Chem. Interfacial Electrochem. 198, 209 (1986).
  14. K.-X. Hu, S. Zheng, C.-Z. Zhao, and Q.-S. Chen, Linear stability of electrocapillary convection in an infinite liquid layer, J. Electrost. 114, 103619 (2021).
  15. A. Castellanos and A. Gonzales, Nonlinear electrohydrodynamics of free surfaces, IEEE Trans. Dielectr. Electr. Insul. 5, 334 (1998).
  16. R. M. Thaokar and V. Kumaran, Electrohydrodynamic instability of the interface between two fluids confined in a channel, Phys. Fluids 17, 084104 (2005).
  17. S. Mählmann and D. T. Papageorgiou, Interfacial instability in electric plane Couette flow, J. Fluid Mech. 666, 155 (2011).
  18. H. González, Influence of bounded geometry on electrocapillary instability, Phys. Rev. B 50, 2520 (1994).
  19. A. K. Uguz, O. Ozen, and N. Aubry, Electric field effect on a two-fluid interface instability in channel flow for fast electric times, Phys. Fluids 20, 031702 (2008).
  20. C. L. Burcham and D. A. Saville, Electrohydrodynamic stability: Taylor-Melcher theory for a liquid bridge suspended in a dielectric gas, J. Fluid Mech. 452, 163 (2002).
  21. M. A. Herrada and A. Barrero, Self-rotation in electrocapillary flows, Phys. Rev. E 66, 036311 (2002).
  22. A. B. Petrin, Electrocapillary instability of a conducting liquid cylinder, J. Exp. Theor. Phys. 106, 963 (2008).
  23. M. Lappa, Thermal Convection: Patterns, Evolution and Stability (Wiley & Sons, Chichester, UK, 2009).
  24. O. A. Basaran and L. E. Scriven, The Taylor pump: Viscous-free surface flow driven by electric shear stress, Chem. Eng. Commun. 67, 259 (1988).
  25. A. Yu. Gelfgat, Stability of convective flows in cavities: Solution of benchmark problems by a low-order finite volume method, Int. J. Numer. Methods Fluids 53, 485 (2007).
  26. G. Papeschi, M. Costa, and S. Bordi, Electrochemical behavior of methylene blue and its leucoform at the mercury electrode, J. Electrochem. Sci. Technol. 128, 1518 (1981).
  27. O. E. Godinez-Brizuela, C. Duczek, N. Weber, W. Nash, M. Sarma, and K. E. Einarsrud, A continuous multiphase model for liquid metal batteries, J. Energy Storage 73, 109147 (2023).
  28. A. Y. Gelfgat, Instability of natural convection in a laterally heated cube with perfectly conducting horizontal boundaries, Theor. Comput. Fluid Dyn. 34, 693 (2020).
  29. H. Ferialdi, M. Lappa, and C. Haughey, On the role of thermal boundary conditions in typical problems of buoyancy convection: A combined experimental-numerical analysis, Int. J. Heat Mass Transfer 159, 120012 (2020).
  30. A. Y. Gelfgat, Time-dependent modeling of oscillatory instability of three-dimensional natural convection of air in a laterally heated cubic box, Theor. Comput. Fluid Dyn. 31, 447 (2017).
  31. G. Lippmann, Relations entre les phénomènes électriques et capillaires, Ann. Chim. Phys. 5, 494 (1875).
  32. J. O’M. Bockris and S. U. M. Khan, Surface Electrochemistry (Springer, New York, 1993).
  33. D. A. Saville, Electrodynamics: The Taylor-Melcher leaky dielectric model, Annu. Rev. Fluid Mech. 29, 27 (1997).
  34. D. Johnson, Electrocapillary flows, in Interfacial Fluid Dynamics and Transport Processes, edited by R. Narayanan and D. Schwabe (Springer, Berlin, 2003), pp. 291–304.
  35. T. Köllner, T. Boeck, and J. Schumacher, Thermal Rayleigh-Marangoni convection in a three-layer liquid-metal battery model, Phys. Rev. E 95, 053114 (2017).
  36. L. D. Landau and E. M. Lifshitz, Electrodynamics of Continuous Media (Pergamon Press, New York, 1984).
  37. A. Castellanos, Basic concepts and equations in electrohydrodynamics, in Electrohydrodynamics, edited by A. Castellanos (Springer, New York, 1998), pp. 1–82.
  38. A. I. Zhakin, Electrohydodynamics, Phys.-Usp. 55, 465 (2012).
  39. D. H. Kelley and T. Weier, Fluid mechanics of liquid metal batteries, Appl. Mech. Rev. 70, 020801 (2018).
  40. J. N. Coupland and D. J. McClements, Physical properties of liquid edible oils, J. Am. Oil Chem. Soc. 74, 1559 (1997).
  41. S. N. Sahasrabudheb, V. Rodriguez-Martinez, M. O’Meara, and B. E. Farkas, Density, viscosity, and surface tension of five vegetable oils at elevated temperatures: Measurement and modeling, Int. J. Food Prop. 20, S1965 (2017).
  42. N. Šegatin, T. P. Žontar, and N. P. Ulrih, Dielectric properties and dipole moment of edible oils subjected to ‘frying’ thermal treatment, Foods 9, 9070900 (2020).
  43. The Engineering Toolbox, https://www.engineeringtoolbox.com.
  44. V. S. Kumar, S. Sampath, S. M. Das, and K. V. Kumar, Atmospheric electrical conductivity variations over different environments, Geophys. J. Int. 122, 89 (1995).
  45. D. A. Nissen and R. W. Carlsten, The surface tension of molten binary system, J. Electrochem. Soc. 121, 500 (1974).
  46. A. De Ninno, E. Nikollari, M. Missori, and F. Frezza, Dielectric permittivity of aqueous solutions of electrolytes probed by THz time-domain and FTIR spectroscopy, Phys. Lett. A 384, 126865 (2020).
  47. J. Kestin, H. E. Khalifa, and R. J. Corella, Tables of the dynamic and kinematic viscosity of aqueous NaCl solutions in the temperature range 20–150 °C and the pressure range 0.1–35 MPa, J. Phys. Chem. Ref. Data 10, 71 (1981).
  48. W. Zhang, S. Cheng, Y. Wang, L. Wu, and Y. Hu, Experimental and modeling of conductivity for electrolyte solution systems, ACS Omega 5, 22465 (2020).
  49. S. Seal, K. Doblhoff-Dier, and J. Meyer, Dielectric decrement for aqueous NaCl solutions: Effect of ionic charge scaling in nonpolarizable water force fields, J. Phys. Chem. B 123, 9912 (2019).
  50. A. A. Aleksandrov, E. V. Dzhuraeva, and V. F. Utenkov, Thermal conductivity of sodium chloride aqueous solutions, Therm. Eng. 60, 190 (2013).
  51. D. G. Archer and R. W. Carter, Thermodynamic properties of the NaCl + H2O system. 4. Heat capacities of H2O and NaCl(aq) in cold-stable and supercooled states, J. Phys. Chem. B 104, 8563 (2000).
  52. P. S. Z. Rogers and K. S. Pfitzer, Volumetric properties of aqueous sodium chloride solutions, J. Phys. Chem. Ref. Data 11, 15 (1962).
  53. O. Ozdemir, S. I. Karakashev, A. V. Nguyen, and J. D. Miller, Adsorption and surface tension analysis of concentrated alkali halide brine solutions, Miner. Eng. 22, 263 (2009).
  54. A. Horibe, S. Fukusako, and M. Yamada, Surface tension of low-temperature aqueous solutions, Int. J. Thermophys. 17, 483 (1996).
  55. Advanced Thermodynamics, https://advancedthermo.com/electrolytes/density_NaCl_Jun2021.html.
  56. A. I. Simion, C.-G. Grigoraş, A.-M. Roşu, and L. Gavrilă, Mathematical modelling of density and viscosity of NaCl aqueous solutions, J. Agroaliment. Proc. Technol. 21, 41 (2015).
  57. L. Gao, Y. Wu, J. Chen, Z. Lv, and K. Wu, Comparison of charge mobility in insulating oil and oil-immersed paper, in 2022 IEEE Conference on Electrical Insulation and Dielectric Phenomena (CEIDP) (IEEE, Piscataway, NJ, 2022), pp. 9–12.
  58. M. Rezaei, A. R. Azimian, A. R. Pishevara, and D. J. Bonthuis, Viscous interfacial layer formation causes electroosmotic mobility reversal in monovalent electrolytes, Phys. Chem. Chem. Phys. 20, 22517 (2018).
  59. Y. Matsubara, Measurement of surface conductivity in dielectric liquid, J. Electrostatics 46, 125 (1999).
  60. S. D. James, Electrochemistry of the interface between some aluminosilicate crystals and salt solutions. I. Surface conductivity, J. Phys. Chem. 70, 3447 (1966).
  61. S. Godefroy, J.-P. Korb, M. Fleury, and R. G. Bryant, New ways of probing surface nuclear relaxation and microdynamics of water and oil in porous media, Magn. Reson. Imaging 19, 517 (2001).
  62. Y. F. Zuev, O. I. Gnezdilov, O. S. Zueva, and O. G. Us'yarov, Effective self-diffusion coefficients of ions in sodium dodecyl sulfate micellar solutions, Colloid J. 73, 59 (2011).
  63. A. Nepomnyashchy, I. Simanovskii, and J. C. Legros, Interfacial Convection in Multilayer Systems (Springer, New York, 2006).
  64. A. Y. Gelfgat, Effect of interface dynamic deformations on instabilities of buoyancy-thermocapillary convection in a two-fluid two-layer system, Phys. Rev. Fluids 7, 053503 (2022).
  65. S. V. Patankar, Numerical Heat Transfer and Fluid Flow (McGraw-Hill, New York, 1980).
  66. Y. Feldman, Direct numerical simulation of transitions and supercritical regimes in confined three-dimensional recirculating flows, Ph.D. thesis, Tel-Aviv University, 2010.
  67. Y. Feldman and A. Y. Gelfgat, On pressure–velocity coupled time-integration of incompressible Navier–Stokes equations using direct inversion of Stokes operator or accelerated multigrid technique, Comput. Struct. 87, 710 (2009).
  68. Y. L. Wu, Development of a three-dimensional solver based on the local domain-free discretization and immersed boundary method and its application for incompressible flow problems, Int. J. Numer. Methods Fluids 89, 283 (2019).
  69. J. Kim, D. Kim, and H. Choi, An immersed-boundary finite-volume method for simulations of flow in complex geometries, J. Comput. Phys. 171, 132 (2001).
  70. R. V. Birikh, Thermocapillary convection in a horizontal layer of liquid, J. Appl. Mech. Tech. Phys. 3, 69 (1966).
  71. H. B. Hadid and B. Roux, Thermocapillary convection in long horizontal layers of low-Prandtl-number melts subject to a horizontal temperature gradient, J. Fluid Mech. 221, 77 (1990).
  72. A. Y. Gelfgat, P. Z. Bar-Yoseph, and A. L. Yarin, Stability of multiple steady states of convection in laterally heated cavities, J. Fluid Mech. 388, 315 (1999).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation