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Possible chiral spin-liquid phase in noncentrosymmetric RBaCo4O7

D. D. Khalyavin1, P. Manuel1, and L. C. Chapon2

  • 1ISIS Facility, STFC Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire, OX11 0QX, United Kingdom
  • 2Institut Laue-Langevin, BP 156X, 38042 Grenoble, France

Phys. Rev. B 85, 220401(R) – Published 13 June, 2012

DOI: https://doi.org/10.1103/PhysRevB.85.220401

Abstract

Based on a symmetry approach, we propose a possible explanation of the weak ferromagnetic component recently observed in YBaCo3FeO7 [M. Valldor et al., Phys. Rev. B 84, 224426 (2011)] and other isostructural compounds in the high-temperature spin-liquid phase. Due to the polar nature of their crystal structure, a coupling between time-odd scalar spin chirality which we suggest as the primary order parameter and macroscopic magnetization is possible as follows from the general form of the appropriate free-energy invariant. The deduced pseudoproper coupling between both physical quantities provides a unique possibility to study the critical behavior of the chiral order parameter.

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