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Anisotropic interference of degenerate four-wave mixing in crystalline silicon

R. Buhleier

G. Lüpke

G. Marowsky

Z. Gogolak

J. Kuhl

  • Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, 70506 Stuttgart, Germany

  • Institut für Halbleitertechnik, Rheinisch-Westfälische Technische Hochschule Aachen, 52074 Aachen, Germany

  • Laser-Laboratorium Göttingen e.V., Hans-Adolf-Krebs-Weg 1, 37077 Göttingen, Germany

  • Department of Optics and Quantum Electronics, JATE University, Szeged, Hungary

  • Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, 70506 Stuttgart, Germany

Phys. Rev. B 50, 2425 – Published 15 July, 1994

DOI: https://doi.org/10.1103/PhysRevB.50.2425

Abstract

Degenerate-four-wave-mixing experiments have been performed on crystalline silicon at 620 nm using 100-fs pulses. Symmetry analysis has been applied to monitor the fourfold (bulk) symmetry of the [100] direction. Deviations from orthogonal polarization of the pump-and-probe beam with respect to the diffracted-signal beam have been studied in detail. The rotation patterns exhibit the transformation behavior of the relevant χ(3) tensor. Preliminary time-resolved measurements reveal distinct variations of the signal occurring on a time scale of 10 fs upon excitation with 100-fs pulses, which cannot be detected by standard correlation techniques.

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