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HIGHLIGHTED ARTICLES

Sub-50-mK Electronic Cooling with Large-Area Superconducting Tunnel Junctions

H. Q. Nguyen, M. Meschke, H. Courtois, and J. P. Pekola

Phys. Rev. Applied 2, 054001 (2014) - Published 4 November, 2014

Experiments conducted below 0.1 K require expensive, complicated cryogenic apparatus. What if an integrated solid-state device could be used instead? The authors present just such an on-chip refrigerator, based on a superconductor/normal-metal junction, that chills down to 30 mK with remarkable cooling power. This provides a means to reduce thermal noise in e.g. qubits, SQUIPT magnetometers, or the sensitive detectors required for astronomy experiments.

Platinum-Based Nanowire Networks with Enhanced Oxygen-Reduction Activity

Henning Galinski, Thomas Ryll, Yang Lin, Barbara Scherrer, Anna Evans, Ludwig J. Gauckler, and Max Döbeli

Phys. Rev. Applied 2, 054015 (2014) - Published 26 November, 2014

Platinum is a favorite material for numerous applications, including electrodes for solid oxide fuel cells, but of course it is costly. The authors use dealloying to prepare thin films of spongelike nanoporous Pt-Y-Al, the yttrium being added to engineer the material’s bandstructure and reduce the amount of platinum required. This yields electrodes with enhanced thermal stability and 13 times the electrocatalytic activity of conventional systems.

Conduction at a Ferroelectric Interface

Matthew S. J. Marshall, Andrei Malashevich, Ankit S. Disa, Myung-Geun Han, Hanghui Chen, Yimei Zhu, Sohrab Ismail-Beigi, Frederick J. Walker, and Charles H. Ahn

Phys. Rev. Applied 2, 051001 (2014) - Published 5 November, 2014

A new and surprising property is discovered when a ferroelectric nonvolatile gate is combined with a conductive oxide channel: When the polarization is switched, a single atomic layer in the normally insulating ferroelectric becomes conductive. This layer has a high mobility and becomes the dominant conductive channel in the all-oxide heterostructure. This approach can be extended to control the properties of any single atomic layer at the interface between a ferroelectric and a channel material, and presents a qualitative shift in our understanding of the ferroelectric field effect.

Ultrathin Fibers from Electrospinning Experiments under Driven Fast-Oscillating Perturbations

Ivan Coluzza, Dario Pisignano, Daniele Gentili, Giuseppe Pontrelli, and Sauro Succi

Phys. Rev. Applied 2, 054011 (2014) - Published 19 November, 2014

When it comes to spinning polymer fibers, spiders are much better than scientists. However, the authors have narrowed the gap: Extensive simulations show that for by judiciously oscillating the spinneret, instabilities can be tamed and extremely thin fibers can be extracted. Remarkably, this effect is independent of the rheology of the polymeric solution used. These ultrathin fibers open up a new length scale for applications ranging from photonics and organic field-effect transistors to artificial ligaments and scaffolds used in tissue culture.

Design and Signature Analysis of Remote Trace-Gas Identification Methodology Based on Infrared-Terahertz Double-Resonance Spectroscopy

Elizabeth A. Tanner, Dane J. Phillips, Christopher M. Persons, Frank C. De Lucia, and Henry O. Everitt

Phys. Rev. Applied 2, 054016 (2014) - Published 26 November, 2014

Remote sensing of trace gases in the atmosphere is used to detect toxins, monitor pollution, and verify treaties, but presently is limited when it comes to recognizing and discriminating similar chemicals. The authors quantitatively assess the potential for a technique with high recognition specificity, even among isotopic isomers (isotopomers), at distances up to 1 km.

LETTERS

Conduction at a Ferroelectric Interface

Matthew S. J. Marshall, Andrei Malashevich, Ankit S. Disa, Myung-Geun Han, Hanghui Chen, Yimei Zhu, Sohrab Ismail-Beigi, Frederick J. Walker, and Charles H. Ahn

Phys. Rev. Applied 2, 051001 (2014) - Published 5 November, 2014

A new and surprising property is discovered when a ferroelectric nonvolatile gate is combined with a conductive oxide channel: When the polarization is switched, a single atomic layer in the normally insulating ferroelectric becomes conductive. This layer has a high mobility and becomes the dominant conductive channel in the all-oxide heterostructure. This approach can be extended to control the properties of any single atomic layer at the interface between a ferroelectric and a channel material, and presents a qualitative shift in our understanding of the ferroelectric field effect.

ARTICLES

Sub-50-mK Electronic Cooling with Large-Area Superconducting Tunnel Junctions

H. Q. Nguyen, M. Meschke, H. Courtois, and J. P. Pekola

Phys. Rev. Applied 2, 054001 (2014) - Published 4 November, 2014

Experiments conducted below 0.1 K require expensive, complicated cryogenic apparatus. What if an integrated solid-state device could be used instead? The authors present just such an on-chip refrigerator, based on a superconductor/normal-metal junction, that chills down to 30 mK with remarkable cooling power. This provides a means to reduce thermal noise in e.g. qubits, SQUIPT magnetometers, or the sensitive detectors required for astronomy experiments.

High-Cooperativity Cavity QED with Magnons at Microwave Frequencies

Maxim Goryachev, Warrick G. Farr, Daniel L. Creedon, Yaohui Fan, Mikhail Kostylev, and Michael E. Tobar

Phys. Rev. Applied 2, 054002 (2014) - Published 5 November, 2014

Magnons are quantized quasiparticles that can in principle be used in quantum computation. To implement such computations in practice, magnons must be strongly coupled with photons, which transfer information between them. In this work, the authors demonstrate extremely strong couplings using a type of multipost microwave cavity that can focus a magnetic field into submillimeter-sized samples. This ultrastrong coupling of magnons and photons can be a building block in the architecture of high-fidelity hybrid quantum systems for the processors of the future.

Expanding Effective-Medium Theory to Optical Diamagnetic Responses in Magnetoplasmonic Colloids

Ondřej Vlašín, Oana Pascu, Anna Roig, and Gervasi Herranz

Phys. Rev. Applied 2, 054003 (2014) - Published 5 November, 2014

The authors present an effective-medium theory of the optical diamagnetic response of very dilute metal colloids. These dispersions of ferromagnetic metal clusters in diamagnetic hosts show a large, linear response under an applied magnetic field, which is of interest for emerging applications in sensing, integrated optical communications, and magneto-optical current transformers and transducers. This theory could be further extended to describe e.g., metal inclusions in polymers or glasses.

Effect of Surface Termination on the Electronic Properties of LaNiO3 Films

Divine P. Kumah, Andrei Malashevich, Ankit S. Disa, Dario A. Arena, Frederick J. Walker, Sohrab Ismail-Beigi, and Charles H. Ahn

Phys. Rev. Applied 2, 054004 (2014) - Published 6 November, 2014

Tailoring the microscopic structures of oxide interfaces and surfaces to realize desired electronic properties is of intense interest. The authors modulate the conductivity of LaNiO3 films as thin as three unit cells by precisely controlling the composition of the topmost atomic layer. Three-dimensional x-ray imaging combined with first-principles theory exposes the correlation between surface termination and electrical conductivity, which could be widely exploited in logic, memory, or sensor applications.

Electrical Activity of Boron and Phosphorus in Hydrogenated Amorphous Silicon

A. Pandey, B. Cai, N. Podraza, and D. A. Drabold

Phys. Rev. Applied 2, 054005 (2014) - Published 7 November, 2014

Hydrogenated amorphous silicon is a technologically important material, vital to applications as varied as photovoltaics, thin-film transistors, and “night vision” goggles. All of these applications rely on the function of dopants, but, remarkably, our understanding of how the most common dopants infiltrate into a material to perform crucial electronic functions remains largely empirical. The authors provide a comprehensive ab initio study of two key dopants in amorphous silicon, including lattice dynamics and hydrogen hopping and passivation. This insight provides a firm foundation for rational optimization of practical semiconductors.

Hot-Electron Transistors for Terahertz Operation Based on Two-Dimensional Crystal Heterostructures

Byoung Don Kong, Zhenghe Jin, and Ki Wook Kim

Phys. Rev. Applied 2, 054006 (2014) - Published 10 November, 2014

The authors explore the feasibility of ultrahigh-frequency devices by utilizing the unique features of two-dimensional (2D) crystals. These materials range from gapless semimetals to wide-band-gap insulators, and a number of them (e.g. hexagonal boron nitride and transition metal dichalcogenides) can be integrated seamlessly with graphene, without causing defects, interfacial scattering centers, or degradation of properties. A detailed theoretical analysis indicates the potential for 2D crystal heterostructures that could process information at rates well over a terahertz–several times the current technological limit.

Pentamode Metamaterials with Independently Tailored Bulk Modulus and Mass Density

Muamer Kadic, Tiemo Bückmann, Robert Schittny, Peter Gumbsch, and Martin Wegener

Phys. Rev. Applied 2, 054007 (2014) - Published 10 November, 2014

Metamaterials can be engineered to control not just light, but also acoustic waves. The authors fabricate a class of three-dimensional, linear elastic metamaterials for which the effective bulk modulus and mass density can be adjusted independently over a large range. This tuning is not possible in ordinary materials, but through geometric design this scheme allows for “acoustic cloaking”, in which an object may be shielded from noise or other sound waves, such as sonar.

All-Optical Blister Test of Suspended Graphene Using Micro-Raman Spectroscopy

Dominik Metten, François Federspiel, Michelangelo Romeo, and Stéphane Berciaud

Phys. Rev. Applied 2, 054008 (2014) - Published 11 November, 2014

Graphene adheres very strongly to solids and is impermeable to many gases, which allows the formation of suspended graphene blisters of controllable shape. The authors use micro-Raman spectroscopy to perform contactless measurement of the topography and stress/strain parameters of these blisters. This unique “all-optical blister test” can be generalized to other systems and invites applications in pressure sensing and nanoelectromechanical systems (NEMS).

Schottky Barrier Formation and Strain at the (011) GdN/GaN Interface from First Principles

Toshiya Kagawa and Hannes Raebiger

Phys. Rev. Applied 2, 054009 (2014) - Published 14 November, 2014

A current motif in physics research is the use of strain to tailor the electronic properties of a material. One well-defined source of strain is the lattice mismatch at the interface of two crystals, such as GdN (a ferromagnetic insulator) and GaN (a direct-band-gap semiconductor). The authors calculate that such an interface under strain should cause GdN to become a half-metal and to form a Schottky barrier with GaN. This could permit strained interfaces to act as rectifiers in spintronics or other applications.

Tunneling Magnetoresistance Devices Based on Topological Insulators: Ferromagnet–Insulator–Topological-Insulator Junctions Employing Bi2Se3

Matthias Götte, Tomi Paananen, Günter Reiss, and Thomas Dahm

Phys. Rev. Applied 2, 054010 (2014) - Published 17 November, 2014

A key feature of a topological insulator is the correlation of spin and propagation direction of electrons at its surface: a potentially valuable property for spintronics applications. The authors show how this feature can be used in tunneling magnetoresistance (TMR) devices that would have similar or better TMR ratios than traditional devices, even at room temperature; that would require only one ferromagnetic layer, not two; and that could be used to measure the spin polarization of the topological surface state.

Ultrathin Fibers from Electrospinning Experiments under Driven Fast-Oscillating Perturbations

Ivan Coluzza, Dario Pisignano, Daniele Gentili, Giuseppe Pontrelli, and Sauro Succi

Phys. Rev. Applied 2, 054011 (2014) - Published 19 November, 2014

When it comes to spinning polymer fibers, spiders are much better than scientists. However, the authors have narrowed the gap: Extensive simulations show that for by judiciously oscillating the spinneret, instabilities can be tamed and extremely thin fibers can be extracted. Remarkably, this effect is independent of the rheology of the polymeric solution used. These ultrathin fibers open up a new length scale for applications ranging from photonics and organic field-effect transistors to artificial ligaments and scaffolds used in tissue culture.

Dual-Axis High-Data-Rate Atom Interferometer via Cold Ensemble Exchange

Akash V. Rakholia, Hayden J. McGuinness, and Grant W. Biedermann

Phys. Rev. Applied 2, 054012 (2014) - Published 24 November, 2014

Atom interferometers use light to track the Doppler effect as ensembles of cold atoms such as 87Rb travel ballistically in vacuum. These systems are used as ultrasensitive gravimeters and could also be exceptional broadband inertial sensors for vehicle navigation and guidance, but typically they are designed for a static laboratory environment. The authors present a compact atom interferometer that measures acceleration and rotation simultaneously and at a high rate, to be used in a dynamic environment for real-time integration of a vehicle’s equations of motion.

Bilayer Excitons in Two-Dimensional Nanostructures for Greatly Enhanced Thermoelectric Efficiency

Kai Wu, Louk Rademaker, and Jan Zaanen

Phys. Rev. Applied 2, 054013 (2014) - Published 25 November, 2014

Generating electricity from a temperature gradient (due to waste heat from an engine or power plant, say) is seen as a significant aspect of the energy economy. Here the authors propose a thermoelectric device that takes advantage of bilayer excitons, electron-hole bound states that can form at an interface. By enhancing both thermopower and electrical conductivity, the counterflow construction of such bilayer-exciton systems can increase the thermoelectric figure of merit by an order of magnitude, compared to that of a bulk material.

Two-Dimensional Nanoscale Imaging of Gadolinium Spins via Scanning Probe Relaxometry with a Single Spin in Diamond

M. Pelliccione, B. A. Myers, L. M. A. Pascal, A. Das, and A. C. Bleszynski Jayich

Phys. Rev. Applied 2, 054014 (2014) - Published 25 November, 2014

Spin-labeling with paramagnetic ions is important in determining the structures of biomolecules, which are generally large and complex, but current techniques lack the sensitivity to detect a few isolated spins. The authors use a nitrogen-vacancy (NV) center in diamond to image nanoscale volumes of paramagnetic gadolinium compounds on the tip of an atomic force microscope. This is an important step toward imaging isolated spin-labeled molecules.

Platinum-Based Nanowire Networks with Enhanced Oxygen-Reduction Activity

Henning Galinski, Thomas Ryll, Yang Lin, Barbara Scherrer, Anna Evans, Ludwig J. Gauckler, and Max Döbeli

Phys. Rev. Applied 2, 054015 (2014) - Published 26 November, 2014

Platinum is a favorite material for numerous applications, including electrodes for solid oxide fuel cells, but of course it is costly. The authors use dealloying to prepare thin films of spongelike nanoporous Pt-Y-Al, the yttrium being added to engineer the material’s bandstructure and reduce the amount of platinum required. This yields electrodes with enhanced thermal stability and 13 times the electrocatalytic activity of conventional systems.

Design and Signature Analysis of Remote Trace-Gas Identification Methodology Based on Infrared-Terahertz Double-Resonance Spectroscopy

Elizabeth A. Tanner, Dane J. Phillips, Christopher M. Persons, Frank C. De Lucia, and Henry O. Everitt

Phys. Rev. Applied 2, 054016 (2014) - Published 26 November, 2014

Remote sensing of trace gases in the atmosphere is used to detect toxins, monitor pollution, and verify treaties, but presently is limited when it comes to recognizing and discriminating similar chemicals. The authors quantitatively assess the potential for a technique with high recognition specificity, even among isotopic isomers (isotopomers), at distances up to 1 km.

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