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Direct Imaging of the ac Component of Pumped Spin Polarization with Element Specificity

S. Pile1, M. Buchner1, V. Ney1, T. Schaffers1,†, J. Lumetzberger1, K. Lenz2, R. Narkowicz2, J. Lindner2, H. Ohldag3,4,‡ et al.

A. Ney1,*

  • 1Institute of Semiconductor and Solid State Physics, Johannes Kepler University, Altenberger Strasse 69, Linz 4040, Austria
  • 2Helmholtz-Zentrum Dresden-Rossendorf, Institute of Ion Beam Physics and Materials Research, Bautzner Landstrasse 400, Dresden 01328, Germany
  • 3Stanford Synchrotron Radiation Laboratory, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA
  • 4Department of Physics, University of California Santa Cruz, Santa Cruz, California 95064, USA

  • *andreas.ney@jku.at
  • Present address: NanoSpin, Department of Applied Physics, Aalto University School of Science, P.O. Box 15100, FI-00076 Aalto, Finland.
  • Present addresses: Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA and Department of Material Sciences and Engineering, Stanford University, Stanford, CA 94305, USA.

Phys. Rev. Applied 14, 034005 – Published 1 September, 2020

DOI: https://doi.org/10.1103/PhysRevApplied.14.034005

Abstract

Spin pumping in a ferromagnet-nonferromagnet heterostructure is directly imaged with spatial resolution as well as element selectivity. The time-resolved detection in scanning transmission x-ray microscopy allows us to directly probe the spatial extent of the ac spin polarization in Co-doped ZnO, which is generated by spin pumping from an adjacent permalloy microstrip. Comparing the relative phases of the dynamic magnetization component of the two constituents is possible and found to be close to antiphase. The correlation between the distribution of the magnetic excitation in the permalloy and the Co-doped ZnO reveals that laterally there is no one-to-one correlation. The observed distribution is rather complex, but integrating over larger areas demonstrates that the spin polarization in the nonferromagnet extends laterally beyond the region of the ferromagnetic microstrip. Therefore, the observations are better explained by a local spin pumping efficiency and a lateral propagation of the ac spin polarization in the nonferromagnet over the range of a few micrometers.

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References (31)

  1. Y. Tserkovnyak, A. Brataas, and G. E. W. Bauer, Enhanced Gilbert Damping in Thin Ferromagnetic Films, Phys. Rev. Lett. 88, 117601 (2002).
  2. H. Jiao and G. E. W. Bauer, Spin Backflow and ac Voltage Generation by Spin Pumping and the Inverse Spin Hall Effect, Phys. Rev. Lett. 110, 217602 (2013).
  3. D. Wei, M. Obstbaum, M. Ribow, C. H. Back, and G. Woltersdorf, Spin Hall voltages from a.c. and d.c. spin currents, Nat. Commun. 5, 3768 (2014).
  4. M. M. Qaid, T. Richter, A. Müller, C. Hauser, C. Ballani, and G. Schmidt, Radiation damping in ferromagnetic resonance induced by a conducting spin sink, Phys. Rev. B 96, 184405 (2017).
  5. K. Ando, S. Takahashi, J. Ieda, Y. Kajiwara, H. Nakayama, T. Yoshino, K. Harii, Y. Fujikawa, M. Matsuo, S. Maekawa, and E. Saitoh, Inverse spin-Hall effect induced by spin pumping in metallic system, J. Appl. Phys. 109, 103913 (2011).
  6. S. Geprägs, S. Meyer, S. Altmannshofer, M. Opel, F. Wilhelm, A. Rogalev, R. Gross, and S. T. B. Goennenwein, Investigation of induced Pt magnetic polarization in Pt/Y3Fe5O12 bilayers, Appl. Phys. Lett. 101, 262407 (2012).
  7. J.-C. Rojas-Sanchez, M. Cubukcu, A. Jain, C. Vergnaud, C. Portemont, C. Ducruet, A. Barski, A. Marty, L. Vila, J.-P. Attane, E. Augendre, G. Desfonds, S. Gambarelli, H. Jaffres, J.-M. George, and M. Jamet, Spin pumping and inverse spin Hall effect in germanium, Phys. Rev. B 88, 064403 (2013).
  8. T. Richter, M. Paleschke, M. Wahler, F. Heyroth, H. Deniz, D. Hesse, and G. Schmidt, Spin pumping and inverse spin Hall effect in ultrathin SrRuO3 films around the percolation limit, Phys. Rev. B 96, 184407 (2017).
  9. J.-C. Lee, L.-W. Huang, D.-S. Hung, T.-H. Chiang, J. C. A. Huang, J.-Z. Liang, and S.-F. Lee, Inverse spin Hall effect induced by spin pumping into semiconducting ZnO, Appl. Phys. Lett. 104, 052401 (2014).
  10. R. Urban, G. Woltersdorf, and B. Heinrich, Gilbert Damping in Single and Multilayer Ultrathin Films: Role of Interfaces in Nonlocal Spin Dynamics, Phys. Rev. Lett. 87, 217204 (2001).
  11. B. Heinrich, C. Burrowes, E. Montoya, B. Kardasz, E. Girt, Y.-Y. Song, Y. Sun, and M. Wu, Spin Pumping at the Magnetic Insulator (YIG)/Normal Metal (Au) Interfaces, Phys. Rev. Lett. 107, 066604 (2011).
  12. C. Hahn, G. de Loubens, M. Viret, O. Klein, V. V. Naletov, and J. Ben Youssef, Detection of Microwave Spin Pumping Using the Inverse Spin Hall Effect, Phys. Rev. Lett. 111, 217204 (2013).
  13. M. Weiler, J. M. Shaw, H. T. Nembach, and T. J. Silva, Phase-Sensitive Detection of Spin Pumping via the ac Inverse Spin Hall Effect, Phys. Rev. Lett. 113, 157204 (2014).
  14. S. Bonetti, R. Kukreja, Z. Chen, D. Spoddig, K. Ollefs, C. Schöppner, R. Meckenstock, A. Ney, J. Pinto, R. Houanche, J. Frisch, J. Stöhr, H. Dürr, and H. Ohldag, Microwave soft x-ray microscopy for nanoscale magnetization dynamics in the 5–10 GHz frequency range, Rev. Sci. Instrum. 86, 093703 (2015).
  15. R. Kukreja, S. Bonetti, Z. Chen, D. Backes, Y. Acremann, J. A. Katine, A. D. Kent, H. A. Dürr, H. Ohldag, and J. Stöhr, X-Ray Detection of Transient Magnetic Moments Induced by a Spin Current in Cu, Phys. Rev. Lett. 115, 096601 (2015).
  16. J. Ding, W. Zhang, M. B. Jungfleisch, J. E. Pearson, H. Ohldag, V- Novosad, and A. Hoffmann, Direct observation of spin accumulation in Cu induced by spin pumping, Phys. Rev. Res. 2, 013262 (2020).
  17. J. Li, L. R. Shelford, P. Shafer, A. Tan, J. X. Deng, P. S. Keatley, C. Hwang, E. Arenholz, G. van der Laan, R. J. Hicken, and Z. Q. Qiu, Direct detection of pure ac spin current by X-ray pump-probe measurements, Phys. Rev. Lett 117, 076602 (2016).
  18. H. A. Dürr, T. Eimüller, H. J. Elmers, S. Eisebitt, M. Farle, W. Kuch, F. Matthes, M. Martins, H. C. Mertins, P. M. Oppeneer, L. Plucinski, C. M. Schneider, H. Wende, W. Wurth, and H. Zabel, A closer look into magnetism: Opportunities with synchrotron radiation, IEEE Transact. Magn. 45, 15 (2009).
  19. M. Buchner, J. Lumetzberger, V. Ney, T. Schaffers, N. Daffe, and A. Ney, Spin pumping from permalloy into uncompensated antiferromagnetic Co doped zinc oxide, J. Appl. Phys. 127, 043901 (2020).
  20. M. Buchner, B. Henne, V. Ney, and A. Ney, Transition from a hysteresis-like to an exchange-bias-like response of an uncompensated antiferromagnet, Phys. Rev. B 99, 064409 (2019).
  21. R. Narkowicz, D. Suter, and R. Stonies, Planar microresonators for EPR experiments, J. Magn. Reson. 175, 275 (2005).
  22. R. Narkowicz, D. Suter, and I. Niemeyer, Scaling of sensitivity and efficiency in planar microresonators for electron spin resonance, Rev. Sci. Instrum. 79, 084702 (2008).
  23. T. Schaffers, R. Meckenstock, D. Spoddig, T. Feggeler, K. Ollefs, C. Schöppner, S. Bonetti, H. Ohldag, M. Farle, and A. Ney, The combination of micro-resonators with spatially resolved ferromagnetic resonance, Rev. Sci. Instrum. 88, 093703 (2017).
  24. F. M. Römer, M. Möller, K. Wagner, L. Gathmann, R. Narkowicz, H. Zähres, B. R. Salles, P. Torelli, R. Meckenstock, J. Lindner, and M. Farle, In situ multifrequency ferromagnetic resonance and x-ray magnetic circular dichroism investigations on Fe/GaAs(110): Enhanced g-factor, Appl. Phys. Lett. 100, 092402 (2012).
  25. A. Banholzer, R. Narkowicz, C. Hassel, R. Meckenstock, S. Stienen, O. Posth, D. Suter, M. Farle, and J. Lindner, Visualization of spin dynamics in single nanosized magnetic elements, Nanotechnol. 22, 295713 (2011).
  26. V. Ney, B. Henne, J. Lumetzberger, F. Wilhelm, K. Ollefs, A. Rogalev, A. Kovacs, M. Kieschnick, and A. Ney, Coalescence-driven magnetic order of the uncompensated antiferromagnetic Co doped ZnO, Phys. Rev. B 94, 224405 (2016).
  27. T. Schaffers, T. Feggeler, S. Pile, R. Meckenstock, M. Buchner, D. Spoddig, V. Ney, M. Farle, H. Wende, S. Wintz, M. Weigand, H. Ohldag, K. Ollefs, and A. Ney, Extracting the dynamic magnetic contrast in time-resolved X-ray transmission microscopy, Nanomaterials 9, 940 (2019).
  28. S. Pile, T. Feggeler, T. Schaffers, R. Meckenstock, M. Buchner, D. Spoddig, B. Zingsem, V. Ney, M. Farle, H. Wende, H. Ohldag, A. Ney, and K. Ollefs, Non-standing spin-waves in confined micrometer-sized ferromagnetic structures under uniform excitation, Appl. Phys. Lett. 116, 072401 (2020).
  29. F. Groß, N. Träger, J. Förster, M. Weigand, G. Schütz, and J. Gräfe, Nanoscale detection of spin wave deflection angles in permalloy, Appl. Phys. Lett. 114, 012406 (2019).
  30. P. Laczkowski, M. Cosset-Cheneau, W. Savero-Torres, V. T. Pham, G. Zahnd, H. Jaffres, N. Reyren, J.-C. Rojas-Sanchez, A. Marty, L. Vila, J.-M. George, and J.-P. Attane, Spin-dependent transport characterization in metallic lateral spin valves using one-dimensional and three-dimensional modeling, Phys. Rev. B 99, 134436 (2019).
  31. S. Ghosh, V. Sih, W. H. Lau, D. D. Awschalom, S.-Y. Bae, S. Wang, S. Vaidya, and G. Chapline, Room-temperature spin coherence in ZnO, Appl. Phys. Lett. 86, 232507 (2005).

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