- Open Access
Multidimensional phase-space manipulation for attosecond electron bunch compression
Phys. Rev. Accel. Beams 29, 060102 – Published 30 June, 2026
DOI: https://doi.org/10.1103/3t5l-mz61
Abstract
Attosecond electron beams are essential for investigating ultrafast structural and electronic dynamics in matter with atomic-scale resolution. We propose a novel method that enables robust attosecond-level electron bunch compression. This method employs THz-driven linear energy chirping and multidimensional phase-space manipulation, effectively compressing the electron bunch and suppressing its arrival timing jitter. Implemented in an MeV ultrafast electron diffraction beamline, this method compresses a 3.18 MeV electron beam from an initial duration of 747 fs (rms) to 810 as (rms) while retaining 6 fC of charge, with 886 as (rms) arrival-time jitter. This approach enables unprecedented timing resolution in ultrafast sciences and offers significant potential for other accelerator applications involving attosecond-scale electron beams.
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References (23)
- X. Wang, D. Xiang, T. Kim, and H. Ihee, Potential of femtosecond electron diffraction using near-relativistic electrons from a photocathode rf electron gun, J. Korean Phys. Soc. 48, 390 (2006).
- F. Fu, S. Liu, P. Zhu, D. Xiang, J. Zhang, and J. Cao, High quality single shot ultrafast MeV electron diffraction from a photocathode radio-frequency gun, Rev. Sci. Instrum. 85, 083701 (2014).
- S. P. Weathersby , Mega-electron-volt ultrafast electron diffraction at SLAC national accelerator laboratory, Rev. Sci. Instrum. 86, 073702 (2015).
- E. M. Mannebach , Dynamic structural response and deformations of monolayer visualized by femtosecond electron diffraction, Nano Lett. 15, 6889 (2015).
- J. Yang , Diffractive imaging of a rotational wavepacket in nitrogen molecules with femtosecond megaelectronvolt electron pulses, Nat. Commun. 7, 11232 (2016).
- J. Yang, X. Zhu, J. P. F. Nunes, J. K. Yu, R. M. Parrish, T. J. A. Wolf, M. Centurion, M. Gühr, R. Li, Y. Liu, B. Moore, M. Niebuhr, S. Park, X. Shen, S. Weathersby, T. Weinacht, T. J. Martinez, and X. Wang, Simultaneous observation of nuclear and electronic dynamics by ultrafast electron diffraction, Science 368, 885 (2020).
- Y. Morimoto and P. Baum, Diffraction and microscopy with attosecond electron pulse trains, Nat. Phys. 14, 252 (2018).
- R. Srinivasan, V. A. Lobastov, C.-Y. Ruan, and A. H. Zewail, Ultrafast electron diffraction (UED). A new development for the 4D determination of transient molecular structures, ChemInform 34 (2003).
- S. Nie, X. Wang, J. Li, R. Clinite, and J. Cao, Femtosecond electron diffraction: Direct probe of ultrafast structural dynamics in metal films, Microsc. Res. Tech. 72, 131 (2009).
- G. Sciaini, M. Harb, S. G. Kruglik, T. Payer, C. T. Hebeisen, F.-J. M. z. Heringdorf, M. Yamaguchi, M. H.-v.. Hoegen, R. Ernstorfer, and R. J. D. Miller, Electronic acceleration of atomic motions and disordering in bismuth, Nature (London) 458, 56 (2009).
- J. C. Williamson, J. Cao, H. Ihee, H. Frey, and A. H. Zewail, Clocking transient chemical changes by ultrafast electron diffraction, Nature (London) 386, 159
- P. Musumeci, J. T. Moody, C. M. Scoby, M. S. Gutierrez, H. A. Bender, and N. S. Wilcox, High quality single shot diffraction patterns using ultrashort megaelectron volt electron beams from a radio frequency photoinjector, Rev. Sci. Instrum. 81, 013306 (2010).
- J. Maxson, D. Cesar, G. Calmasini, A. Ody, P. Musumeci, and D. Alesini, Direct measurement of sub-10 fs relativistic electron beams with ultralow emittance, Phys. Rev. Lett. 118, 154802 (2017).
- L. Zhao , Terahertz streaking of few-femtosecond relativistic electron beams, Phys. Rev. X 8, 021061 (2018).
- L. Zhao, H. Tang, C. Lu, T. Jiang, P. Zhu, L. Hu, W. Song, H. Wang, J. Qiu, C. Jing, S. Antipov, D. Xiang, and J. Zhang, Femtosecond relativistic electron beam with reduced timing jitter from THz driven beam compression, Phys. Rev. Lett. 124, 054802 (2020).
- E. C. Snively, M. A. K. Othman, M. Kozina, B. K. Ofori-Okai, S. P. Weathersby, S. Park, X. Shen, X. J. Wang, M. C. Hoffmann, R. K. Li, and E. A. Nanni, Femtosecond compression dynamics and timing jitter suppression in a THz-driven electron bunch compressor, Phys. Rev. Lett. 124, 054801 (2020).
- F. Qi, Z. Ma, L. Zhao, Y. Cheng, W. Jiang, C. Lu, T. Jiang, D. Qian, Z. Wang, W. Zhang, P. Zhu, X. Zou, W. Wan, D. Xiang, and J. Zhang, Breaking 50 femtosecond resolution barrier in MeV ultrafast electron diffraction with a double bend achromat compressor, Phys. Rev. Lett. 124, 134803 (2020).
- K.-L. Yeh, M. C. Hoffmann, J. Hebling, and K. A. Nelson, Generation of ultrashort terahertz pulses by optical rectification, Appl. Phys. Lett. 90, 171121 (2007).
- C. Feng and Z. Zhao, A storage ring based free-electron laser for generating ultrashort coherent EUV and x-ray radiation, Sci. Rep. 7, 4724 (2017).
- D. H. Dowell, F. Zhou, and J. Schmerge, Exact cancellation of emittance growth due to coupled transverse dynamics in solenoids and rf couplers, Phys. Rev. Accel. Beams 21, 010101 (2018).
- S. van der Geer and M. de Loos, The general particle tracer code: Design, implementation and application, Ph.D. thesis 1 (research tu/e / graduation tu/e), Applied Physics and Science Education, 2001, 10.6100/IR542912.
- F. Qi, Self-stabilized and self-compressed MeV ultrafast electron diffraction and its application in molecular dynamics, Ph.D. thesis, Shanghai Jiao Tong University, 2023.
- S. Kim, P. Piot, J. Power, W. Liu, E. Wisniewski, D. Doran, G. Chen, and C. Whiteford, Round-to-flat and flat-to-round beam transformations at the Argonne Wakefield Accelerator Facility, in Proceedings of the International Particle Accelerator Conference, IPAC2023, Venice, Italy (JACoW, Geneva, Switzerland, 2023), WEPA037, 10.18429/JACoW-IPAC2023-WEPA037.