Export citation

Export citation

Choose format for download:

Download Citation
  • Access by Xinjiang University

Pitch-controlled reorientational nonlinearity in chiral nematic liquid crystals: A reduced-order model for self-focusing and soliton formation

Homa Saadatmand1,*, M. Javad Zakeri2,*, Ahmed Sameh Ahmed3, Suraj Bhandari1, Loubna Benkoula1, Ameer B. Batarseh2, Andrea Blanco-Redondo2, Miroslaw Karpierz4, and Pawel S. Jung1,4,†

  • *These authors contributed equally to this work.
  • Contact author: pjung@miami.edu

Phys. Rev. A 113, 033511 – Published 9 March, 2026

DOI: https://doi.org/10.1103/lsbq-lyrt

Abstract

We present a reduced-order semianalytical model for reorientational nonlinearity in chiral nematic liquid crystals, showing that the chiral pitch acts as the dominant physical length scale governing the onset of nonlinear self-focusing and soliton formation. Starting from the full Frank-Oseen equation, we derive a closed-form expression for the optically induced molecular rotation that captures the essential saturable response of the medium while reducing computational cost by more than two orders of magnitude compared with standard relaxation-method solvers. Despite its simplicity, the model reproduces the essential features of the numerically obtained nonlinear refractive index, the onset of self-localization, and the transition from discrete to continuous solitons in one and two dimensions. It further predicts the formation of fully localized astigmatic nematicons with only minor shifts in the self-localization threshold due to the neglect of nonlocal effects. The proposed model provides direct physical insight into light-matter interactions with soft matter media and offers a computationally efficient tool for the design and optimization of nonlinear photonic devices.

Physics Subject Headings (PhySH)

Article Text

References (49)

  1. S. A. Akhmanov, A. P. Sukhorukov, and R. V. Khokhlov, Self-focusing and diffraction of light in a nonlinear medium, Sov. Phys. Usp. 10, 609 (1968).
  2. A. G. Litvak, Self-focusing of electromagnetic waves in a plasma in an intense magnetic field, Sov. Radiophys. 8, 828 (1965).
  3. P. K. Shukla, L. Stenflo, and N. D. Borisov, Nonlinear interaction of powerful radio waves with the plasma in the earth's lower ionosphere, J. Geophys. Res.: Space 97, 12279 (1992).
  4. F. Dalfovo, S. Giorgini, L. P. Pitaevskii, and S. Stringari, Theory of Bose-Einstein condensation in trapped gases, Rev. Mod. Phys. 71, 463 (1999).
  5. L. P. Pitaevskii and S. Stringari, Bose–Einstein Condensation (Oxford University Press, Oxford, 2003).
  6. V. Achilleos, O. Richoux, G. Theocharis, and D. J. Frantzeskakis, Acoustic solitons in waveguides with Helmholtz resonators: Transmission line approach, Phys. Rev. E 91, 023204 (2015).
  7. E. A. Kuznetsov, A. M. Rubenchik, and V. E. Zakharov, Soliton stability in plasmas and hydrodynamics, Phys. Rep. 142, 103 (1986).
  8. P. K. Shukla and L. Stenflo, Nonlinear propagation of electromagnetic waves in magnetized plasmas, Phys. Rev. A 30, 2110 (1984).
  9. Y. S. Kivshar and G. P. Agrawal, Optical Solitons: From Fibers to Photonic Crystals (Academic, San Diego, 2003).
  10. F. K. Abdullaev, A. Gammal, and L. Tomio, Dynamics of bright matter-wave solitons in a Bose–Einstein condensate with inhomogeneous scattering length, J. Phys. B 37, 635 (2004).
  11. S. Wabnitz, Nonlinear Guided Wave Optics (IOP, Bristol, 2017).
  12. A. A. Sukhorukov and Y. S. Kivshar, Nonlinear guided waves and spatial solitons in a periodic layered medium, J. Opt. Soc. Am. B 19, 772 (2002).
  13. O. Bang, D. Edmundson, and W. Krolikowski, Collapse of incoherent light beams in inertial bulk Kerr media, Phys. Rev. Lett. 83, 5479 (1999).
  14. O. Bang, W. Krolikowski, J. Wyller, and J. J. Rasmussen, Collapse arrest and soliton stabilization in nonlocal nonlinear media, Phys. Rev. E 66, 046619 (2002).
  15. A. W. Snyder and D. J. Mitchell, Accessible solitons, Science 276, 1538 (1997).
  16. W. Krolikowski, O. Bang, J. J. Rasmussen, and J. Wyller, Modulational instability in nonlocal nonlinear Kerr media, Phys. Rev. E 64, 016612 (2001).
  17. C. Conti, M. Peccianti, and G. Assanto, Route to nonlocality and observation of accessible solitons, Phys. Rev. Lett. 91, 073901 (2003).
  18. M. Peccianti, A. Dyadyusha, M. Kaczmarek, and G. Assanto, Tunable refraction and reflection of self-confined light beams, Nat. Phys. 2, 737 (2006).
  19. G. Assanto and M. A. Karpierz, Nematicons: self-localised beams in nematic liquid crystals, Liq. Cryst. 36, 1161 (2009).
  20. M. Peccianti and G. Assanto, Nematicons, Phys. Rep. 516, 147 (2012).
  21. E. Braun, L. P. Faucheux, and A. Libchaber, Strong self-focusing in nematic liquid crystals, Phys. Rev. A 48, 611 (1993).
  22. C. Conti, M. Peccianti, and G. Assanto, Observation of optical spatial solitons in a highly nonlocal medium, Phys. Rev. Lett. 92, 113902 (2004).
  23. A. Piccardi and G. Assanto, Nematonics: From physics to photonics of reorientational solitons, Liq. Cryst. 51, 2252 (2024).
  24. X. Hutsebaut, C. Cambournac, M. Haelterman, A. Adamski, and K. Neyts, Single-component higher-order mode solitons in liquid crystals, Opt. Commun. 233, 211 (2004).
  25. U. A. Laudyn, M. Kwasny, A. Piccardi, M. A. Karpierz, R. Dabrowski, O. Chojnowska, A. Alberucci, and G. Assanto, Nonlinear competition in nematicon propagation, Opt. Lett. 40, 5235 (2015).
  26. M. Warenghem, J. F. Blach, and J. F. Henninot, Thermo-nematicon: An unnatural coexistence of solitons in liquid crystals? J. Opt. Soc. Am. B 25, 1882 (2008).
  27. P. S. Jung, W. Krolikowski, U. A. Laudyn, M. Trippenbach, and M. A. Karpierz, Supermode spatial optical solitons in liquid crystals with competing nonlinearities, Phys. Rev. A 95, 023820 (2017).
  28. A. B. Batarseh, M. J. Zakeri, A. Blanco-Redondo, M. Trippenbach, D. Hagan, W. Krolikowski, and P. S. Jung, Crossover from single to two-peak fundamental solitons in nonlocal nonlinear media, Wave Motion 133, 103445 (2025).
  29. P. S. Jung, M. J. Zakeri, A. Ramaniuk, A. Blanco-Redondo, D. J. Hagan, A. Dogariu, D. N. Christodoulides, G. Assanto, W. Krolikowski, and M. Trippenbach, CLEO: Conference on Lasers and Electro-Optics, Charlotte, 2024 (Optica, Washington, DC, 2024), paper JW2A.203.
  30. A. Alberucci, G. Assanto, D. Buccoliero, A. S. Desyatnikov, T. R. Marchant, and N. F. Smyth, Modulation analysis of boundary-induced motion of optical solitary waves in a nematic liquid crystal, Phys. Rev. A 79, 043816 (2009).
  31. P. G. de Gennes and J. Prost, The Physics of Liquid Crystals, 2nd ed. (Oxford University Press, Oxford, 1993).
  32. P. Oswald, P. Pieranski, J. W. Goodby, and G. W. Gray, Nematic and Cholesteric Liquid Crystals (Taylor & Francis, Boca Raton, 2005).
  33. U. A. Laudyn, M. Kwasny, and M. A. Karpierz, Nematicons in chiral nematic liquid crystals, Appl. Phys. Lett. 94, 091110 (2009).
  34. U. A. Laudyn, P. Jung, K. B. Zegadło, M. A. Karpierz, and G. Assanto, Power-induced evolution and increased dimensionality of nonlinear modes in reorientational soft matter, Opt. Lett. 39, 6399 (2014).
  35. U. A. Laudyn, P. Jung, M. A. Karpierz, and G. Assanto, Quasi two-dimensional astigmatic solitons in soft chiral metastructures, Sci. Rep. 6, 22923 (2016).
  36. L.-L. Ma, C.-Y. Li, J.-T. Pan, Y.-E. Ji, C. Jiang, R. Zheng, Z.-Y. Wang, Y. Wang, B.-X. Li, and Y.-Q. Lu, Self-assembled liquid crystal architectures for soft matter photonics, Light: Sci. Appl. 11, 270 (2022).
  37. D. Kang, H. Heo, Y. Yang, J. Seong, H. Kim, J. Kim, and J. Rho, Liquid crystal-integrated metasurfaces for an active photonic platform, Opto-Electron. Adv. 7, 230216 (2024).
  38. R. Zhang, Z. Zhang, J. Han, L. Yang, J. Li, Z. Song, T. Wang, and J. Zhu, Advanced liquid crystal-based switchable optical devices for light protection applications: principles and strategies, Light: Sci. Appl. 12, 11 (2023).
  39. Y. Yang, L. Wang, H. Yang, and Q. Li, 3D chiral photonic nanostructures based on blue-phase liquid crystals, Small Sci. 1, 2100007 (2021).
  40. S. Perumbilavil, M. Kauranen, and G. Assanto, Spatiospectral features of a soliton-assisted random laser in liquid crystals, Opt. Lett. 44, 3574 (2019).
  41. G. Assanto and M. Peccianti, Spatial solitons in nematic liquid crystals, IEEE J. Quantum Electron. 39, 13 (2003).
  42. D. N. Christodoulides, F. Lederer, and Y. Silberberg, Discretizing light behavior in linear and nonlinear waveguide lattices, Nature (London) 424, 817 (2003).
  43. A. Fratalocchi, G. Assanto, K. A. Brzdąkiewicz, and M. A. Karpierz, Discrete propagation and spatial solitons in nematic liquid crystals, Opt. Lett. 29, 1530 (2004).
  44. A. Bregar, M. Štimulak, and M. Ravnik, Photonic properties of heliconical liquid crystals, Opt. Express 26, 23265 (2018).
  45. V. I. Kopp, B. Fan, H. K. M. Vithana, and A. Z. Genack, Low-threshold lasing at the edge of a photonic stop band in cholesteric liquid crystals, Opt. Lett. 23, 1707 (1998).
  46. F. A. Sala and M. A. Karpierz, Modeling of molecular reorientation and beam propagation in chiral and non-chiral nematic liquid crystals, Opt. Express 20, 13923 (2012).
  47. S. Jungling and J. C. Chen, A study and optimization of eigenmode calculations using the imaginary-distance beam-propagation method, IEEE J. Quantum Electron. 30, 2098 (1994).
  48. R. Dabrowski (private communication).
  49. A. Piccardi, A. Alberucci, and G. Assanto, Nematicons and their electro-optic control: Light localization and signal readdressing via reorientation in liquid crystals, Int. J. Mol. Sci. 14, 19932 (2013).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation