- Open Access
- Access by Xinjiang University
Long-lived fermionic Feshbach molecules with tunable -wave interactions
Phys. Rev. A 107, 053322 – Published 31 May, 2023
DOI: https://doi.org/10.1103/PhysRevA.107.053322
Abstract
Ultracold fermionic Feshbach molecules are promising candidates for exploring quantum matter with strong -wave interactions; however, their lifetimes were measured to be short. Here we characterize the -wave collisions of ultracold fermionic Feshbach molecules for different scattering lengths and temperatures. By increasing the binding energy of the molecules, the two-body loss coefficient reduces by three orders of magnitude, leading to a second-long lifetime 20 times longer than that of ground-state NaK molecules. We exploit the scaling of elastic and inelastic collisions with the scattering length and temperature to identify a regime where the elastic collisions dominate over the inelastic ones, allowing the molecular sample to thermalize. Our results provide a benchmark for four-body calculations of molecular collisions and pave the way for investigating quantum many-body phenomena with fermionic Feshbach molecules.
Physics Subject Headings (PhySH)
Article Text
References (37)
- L. D. Carr, D. DeMille, R. V. Krems, and J. Ye, Cold and ultracold molecules: Science, technology and applications, New J. Phys. 11, 055049 (2009).
- G. Quéméner and P. S. Julienne, Ultracold molecules under control! Chem. Rev. 112, 4949 (2012).
- J. L. Bohn, A. M. Rey, and J. Ye, Cold molecules: Progress in quantum engineering of chemistry and quantum matter, Science 357, 1002 (2017).
- C. Chin, R. Grimm, P. Julienne, and E. Tiesinga, Feshbach resonances in ultracold gases, Rev. Mod. Phys. 82, 1225 (2010).
- F. Ferlaino, S. Knoop, M. Mark, M. Berninger, H. Schöbel, H.-C. Nägerl, and R. Grimm, Collisions between Tunable Halo Dimers: Exploring an Elementary Four-Body Process with Identical Bosons, Phys. Rev. Lett. 101, 023201 (2008).
- B. Marcelis, S. J. J. M. F. Kokkelmans, G. V. Shlyapnikov, and D. S. Petrov, Collisional properties of weakly bound heteronuclear dimers, Phys. Rev. A 77, 032707 (2008).
- F. Ç. Top, Y. Margalit, and W. Ketterle, Spin-polarized fermions with -wave interactions, Phys. Rev. A 104, 043311 (2021).
- K. Maeda, G. Baym, and T. Hatsuda, Simulating Dense QCD Matter with Ultracold Atomic Boson-Fermion Mixtures, Phys. Rev. Lett. 103, 085301 (2009).
- B. Bazak and D. S. Petrov, Stable -Wave Resonant Two-Dimensional Fermi-Bose Dimers, Phys. Rev. Lett. 121, 263001 (2018).
- M. Greiner, C. A. Regal, and D. S. Jin, Emergence of a molecular Bose–Einstein condensate from a Fermi gas, Nature (London) 426, 537 (2003).
- C. A. Regal, M. Greiner, and D. S. Jin, Observation of Resonance Condensation of Fermionic Atom Pairs, Phys. Rev. Lett. 92, 040403 (2004).
- J. J. Zirbel, K.-K. Ni, S. Ospelkaus, J. P. D'Incao, C. E. Wieman, J. Ye, and D. S. Jin, Collisional Stability of Fermionic Feshbach Molecules, Phys. Rev. Lett. 100, 143201 (2008).
- C.-H. Wu, J. W. Park, P. Ahmadi, S. Will, and M. W. Zwierlein, Ultracold Fermionic Feshbach Molecules of , Phys. Rev. Lett. 109, 085301 (2012).
- M.-S. Heo, T. T. Wang, C. A. Christensen, T. M. Rvachov, D. A. Cotta, J.-H. Choi, Y.-R. Lee, and W. Ketterle, Formation of ultracold fermionic NaLi Feshbach molecules, Phys. Rev. A 86, 021602(R) (2012).
- G. Barontini, C. Weber, F. Rabatti, J. Catani, G. Thalhammer, M. Inguscio, and F. Minardi, Observation of Heteronuclear Atomic Efimov Resonances, Phys. Rev. Lett. 103, 043201 (2009).
- D. S. Petrov, Loss process in short range (private communication) (2021).
- G. Quéméner, Ultracold collisions of molecules, arXiv:1703.09174.
- X.-Y. Chen, M. Duda, A. Schindewolf, R. Bause, I. Bloch, and X.-Y. Luo, Suppression of Unitary Three-Body Loss in a Degenerate Bose-Fermi Mixture, Phys. Rev. Lett. 128, 153401 (2022).
- See in Appendixes.
- A. Viel and A. Simoni, Feshbach resonances and weakly bound molecular states of boson-boson and boson-fermion NaK pairs, Phys. Rev. A 93, 042701 (2016).
- R. Bause, A. Schindewolf, R. Tao, M. Duda, X.-Y. Chen, G. Quéméner, T. Karman, A. Christianen, I. Bloch, and X.-Y. Luo, Collisions of ultracold molecules in bright and dark optical dipole traps, Phys. Rev. Res. 3, 033013 (2021).
- Z. Z. Yan, J. W. Park, Y. Ni, H. Loh, S. Will, T. Karman, and M. Zwierlein, Resonant Dipolar Collisions of Ultracold Molecules Induced by Microwave Dressing, Phys. Rev. Lett. 125, 063401 (2020).
- S. Ospelkaus, K.-K. Ni, D. Wang, M. H. G. d. Miranda, B. Neyenhuis, G. Quéméner, P. S. Julienne, J. L. Bohn, D. S. Jin, and J. Ye, Quantum-state controlled chemical reactions of ultracold potassium-rubidium molecules, Science 327, 853 (2010).
- E. R. Hudson, N. B. Gilfoy, S. Kotochigova, J. M. Sage, and D. DeMille, Inelastic Collisions of Ultracold Heteronuclear Molecules in an Optical Trap, Phys. Rev. Lett. 100, 203201 (2008).
- Z. Idziaszek and P. S. Julienne, Universal Rate Constants for Reactive Collisions of Ultracold Molecules, Phys. Rev. Lett. 104, 113202 (2010).
- A. Derevianko, J. F. Babb, and A. Dalgarno, High-precision calculations of van der Waals coefficients for heteronuclear alkali-metal dimers, Phys. Rev. A 63, 052704 (2001).
- J. Mitroy and M. W. J. Bromley, Semiempirical calculation of van der Waals coefficients for alkali-metal and alkaline-earth-metal atoms, Phys. Rev. A 68, 052714 (2003).
- P. S. Julienne, T. M. Hanna, and Z. Idziaszek, Universal ultracold collision rates for polar molecules of two alkali-metal atoms, Phys. Chem. Chem. Phys. 13, 19114 (2011).
- F. Wang, X. Ye, M. Guo, D. Blume, and D. Wang, Observation of resonant scattering between ultracold heteronuclear Feshbach molecules, Phys. Rev. A 100, 042706 (2019).
- K.-K. Ni, S. Ospelkaus, D. Wang, G. Quéméner, B. Neyenhuis, M. H. G. de Miranda, J. L. Bohn, J. Ye, and D. S. Jin, Dipolar collisions of polar molecules in the quantum regime, Nature (London) 464, 1324 (2010).
- B. DeMarco, J. L. Bohn, J. P. Burke, M. Holland, and D. S. Jin, Measurement of -Wave Threshold Law Using Evaporatively Cooled Fermionic Atoms, Phys. Rev. Lett. 82, 4208 (1999).
- Z.-Y. Ma, A. M. Thomas, C. J. Foot, and S. L. Cornish, The evaporative cooling of a gas of caesium atoms in the hydrodynamic regime, J. Phys. B: At. Mol. Opt. Phys. 36, 3533 (2003).
- M. Duda, X.-Y. Chen, A. Schindewolf, R. Bause, J. von Milczewski, R. Schmidt, I. Bloch, and X.-Y. Luo, Transition from a polaronic condensate to a degenerate Fermi gas of heteronuclear molecules, Nat. Phys. 19, 720 (2023).
- A. Schindewolf, R. Bause, X.-Y. Chen, M. Duda, T. Karman, I. Bloch, and X.-Y. Luo, Evaporation of microwave-shielded polar molecules to quantum degeneracy, Nature (London) 607, 677 (2022).
- Z. Zhang, L. Chen, K.-X. Yao, and C. Chin, Transition from an atomic to a molecular Bose–Einstein condensate, Nature (London) 592, 708 (2021).
- G. Durastante, C. Politi, M. Sohmen, P. Ilzhöfer, M. J. Mark, M. A. Norcia, and F. Ferlaino, Feshbach resonances in an erbium-dysprosium dipolar mixture, Phys. Rev. A 102, 033330 (2020).
- A. Frisch, M. Mark, K. Aikawa, S. Baier, R. Grimm, A. Petrov, S. Kotochigova, G. Quéméner, M. Lepers, O. Dulieu, and F. Ferlaino, Ultracold Dipolar Molecules Composed of Strongly Magnetic Atoms, Phys. Rev. Lett. 115, 203201 (2015).