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Effects of tampering on rare-gas core-shell clusters irradiated by resonantly tuned soft-x-ray pulses

Rishi Pandit1, Valerie Becker1, Jeremy Thurston1, Kasey Barrington1, Zachary Hartwick1, Nicolas Bigaouette2, Lora Ramunno2, and Edward Ackad1

  • 1Department of Physics, Southern Illinois University Edwardsville, Edwardsville, Illinois 62026, USA
  • 2Department of Physics, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada

Phys. Rev. A 107, 043107 – Published 10 April, 2023

DOI: https://doi.org/10.1103/PhysRevA.107.043107

Abstract

Tampering resonant rare-gas clusters with nonresonant atoms has been shown to significantly decrease in the final ionization of the resonant atoms [J. Phys. B: At., Mol. Opt. Phys. 41, 181001 (2008)], but not their transient ionization [Phys. Rev. Lett. 112, 183401 (2014)]. In this paper, we explain the details of the charge transfer mechanism from the resonant to nonresonant atoms. We have applied our model to the interaction of an ultraintense x-ray laser tuned to the center of xenon's giant 4d resonance with core-shell argon-xenon clusters. Our results are in agreement with previous experimental results of the disintegration products, and the transient states. Also, our model predicts that the resonant xenon is quickly ionized by the laser. The freed electrons then collisionally ionized the outer argon atoms before recombining with the inner xenon ions to reduce their final charge state. We find that unlike homogeneous clusters whose behavior is governed by the number of atoms, the behavior of core-shell heterogeneous clusters is well predicted by the ratio of resonant to nonresonant atoms.

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