Optical and Electron-Spin-Resonance Spectra of <math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><mrow><msup><mrow><mi mathvariant="normal">Yb</mi></mrow><mrow><mn>3</mn><mo>+</mo></mrow></msup></mrow></math>, <math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><mrow><msup><mrow><mi mathvariant="normal">Nd</mi></mrow><mrow><mn>3</mn><mo>+</mo></mrow></msup></mrow></math>, and <math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><mrow><msup><mrow><mi mathvariant="normal">Cr</mi></mrow><mrow><mn>3</mn><mo>+</mo></mrow></msup></mrow></math> in LiNb<math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><mrow><msub><mrow><mi mathvariant="normal">O</mi></mrow><mrow><mn>3</mn></mrow></msub></mrow></math> and LiTa<math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><mrow><msub><mrow><mi mathvariant="normal">O</mi></mrow><mrow><mn>3</mn></mrow></msub></mrow></math>

Gerald Burns; D. F. O'kane; Reuben S. Title

doi:10.1103/PhysRev.167.314

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Optical and Electron-Spin-Resonance Spectra of ${Yb}^{3 +}$ , ${Nd}^{3 +}$ , and ${Cr}^{3 +}$ in LiNb $O_{3}$ and LiTa $O_{3}$

Gerald Burns^*, D. F. O'kane, and Reuben S. Title

IBM, Watson Research Center, Yorktown Heights, New York

^*Partially supported by Army Research Office, Durham, N.C. under Contract DA-31-124-ARO-D-205.

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Phys. Rev. 167, 314 – Published 10 March, 1968

DOI: https://doi.org/10.1103/PhysRev.167.314

Abstract

The results of optical-spectroscopic and electron-spin-resonance (ESR) studies of ${Yb}^{3 +}$ , ${Nd}^{3 +}$ , and ${Cr}^{3 +}$ impurities are presented. The spectra of ${Yb}^{3 +}$ are discussed in detail. Crystal-field parameters are obtained to fit the energy levels and the ESR results on the ground state. These parameters are not obtained by a least-squares fit but rather by physical considerations as to where, on the threefold axis, the ion could be to give crystal-field parameter ratios that can be used to fit the experimental results.

References (14)

(a) K. Nassau, H. J. Levinstein, and G. M. Loiacono, J. Phys. Chem. Solids 27, 983 (1966) (b) ibid. 27, 989 (1966) (c) S. C. Abrahams, J. M. Reddy, and J. L. Bernstein, ibid. 27, 997 (1966) (d) S. C. Abrahams, ibid. 27, 1013 (1966) (e) S. C. Abrahams, H. J. Levinstein, and J. M. Reddy, ibid. 27, 1019 (1966)
G. Burns, D. F. O'Kane, and R. S. Title, Phys. Letters 23, 56 (1966)
A. A. Ballman, J. Am. Ceramic Soc. 48, 112 (1965)
R. A. Buchanan, K. A. Wickersheim, J. J. Pearson, and G. F. Hersmann, Phys. Rev. 159, 245 (1967) ibid. 159, 251 (1967) W. P. Wolf, J. Chem. Phys. 41, 617 (1964) J. A. Koningstein and J. E. Geusic, Phys. Rev. 136, A711 (1965)
K. W. H. Stevens, Proc. Phys. Soc. (London) 65A, 209 (1952)
B. R. Judd, Proc. Roy. Soc. (London) 227A, 552 (1955) ibid.241A, 122 (1957)
A. Misu, J. Phys. Soc. Japan 19, 2260 (1964) P. Kisliuk and C. A. Moore, Phys. Rev. 160, 307 (1967) J. H. Parker, Jr., R. W. Weinert, and J. G. Castle, Jr. (to be published)
B. Welber (private communication)
J. E. Geusic, M. Peter and E. O. Schulz-duBois, Bell System Tech. J. 38, 291 (1959)
E. O. Schulz-duBois, Bell System Tech. J. 38, 271 (1959)
Omitted endnote
G. Burns, Phys. Rev. 128, 2121 (1962) E. Y. Wong and I. Richman, J. Chem. Phys. 36, 1889 (1962) M. T. Hutchings and D. K. Ray, Proc. Roy. Soc. (London) 81, 633 (1963)
M. T. Hutchings and W. P. Wolf, J. Chem. Phys. 41, 617 (1964)
N. F. Evloanova, A. S. Kovalev, V. A. Koptsik, A. M. Prohkorov, and L. N. Rashkovich, Zh. Eksperim. i Teor. Fiz. 5, 251 (1967) [English transl.: Soviet Phys.—JETP 5, 291 (1967)]

[c1] (a) K. Nassau, H. J. Levinstein, and G. M. Loiacono, J. Phys. Chem. Solids 27, 983 (1966) (b) ibid. 27, 989 (1966) (c) S. C. Abrahams, J. M. Reddy, and J. L. Bernstein, ibid. 27, 997 (1966) (d) S. C. Abrahams, ibid. 27, 1013 (1966) (e) S. C. Abrahams, H. J. Levinstein, and J. M. Reddy, ibid. 27, 1019 (1966)

[c2] G. Burns, D. F. O'Kane, and R. S. Title, Phys. Letters 23, 56 (1966)

[c3] A. A. Ballman, J. Am. Ceramic Soc. 48, 112 (1965)

[c4] R. A. Buchanan, K. A. Wickersheim, J. J. Pearson, and G. F. Hersmann, Phys. Rev. 159, 245 (1967) ibid. 159, 251 (1967) W. P. Wolf, J. Chem. Phys. 41, 617 (1964) J. A. Koningstein and J. E. Geusic, Phys. Rev. 136, A711 (1965)

[c5] K. W. H. Stevens, Proc. Phys. Soc. (London) 65A, 209 (1952)

[c6] B. R. Judd, Proc. Roy. Soc. (London) 227A, 552 (1955) ibid.241A, 122 (1957)

[c7] A. Misu, J. Phys. Soc. Japan 19, 2260 (1964) P. Kisliuk and C. A. Moore, Phys. Rev. 160, 307 (1967) J. H. Parker, Jr., R. W. Weinert, and J. G. Castle, Jr. (to be published)

[c8] B. Welber (private communication)

[c9] J. E. Geusic, M. Peter and E. O. Schulz-duBois, Bell System Tech. J. 38, 291 (1959)

[c10] E. O. Schulz-duBois, Bell System Tech. J. 38, 271 (1959)

[c11] Omitted endnote

[c12] G. Burns, Phys. Rev. 128, 2121 (1962) E. Y. Wong and I. Richman, J. Chem. Phys. 36, 1889 (1962) M. T. Hutchings and D. K. Ray, Proc. Roy. Soc. (London) 81, 633 (1963)

[c13] M. T. Hutchings and W. P. Wolf, J. Chem. Phys. 41, 617 (1964)

[c14] N. F. Evloanova, A. S. Kovalev, V. A. Koptsik, A. M. Prohkorov, and L. N. Rashkovich, Zh. Eksperim. i Teor. Fiz. 5, 251 (1967) [English transl.: Soviet Phys.—JETP 5, 291 (1967)]

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Optical and Electron-Spin-Resonance Spectra of ${Yb}^{3 +}$ , ${Nd}^{3 +}$ , and ${Cr}^{3 +}$ in LiNb $O_{3}$ and LiTa $O_{3}$

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Optical and Electron-Spin-Resonance Spectra of Yb3+, Nd3+, and Cr3+ in LiNbO3 and LiTaO3

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References (14)

Optical and Electron-Spin-Resonance Spectra of ${Yb}^{3 +}$ , ${Nd}^{3 +}$ , and ${Cr}^{3 +}$ in LiNb $O_{3}$ and LiTa $O_{3}$