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  • Access by Xinjiang University

Application of the Statistical Model to Nuclear Magnetic Relaxation in Solid Hydrogen

C. C. Sung*

  • Department of Physics, The Ohio State University, Columbus, Ohio

  • *Research sponsored in part by the Air Force Office of Scientific Research, U.S. Air Force, under AFOSR Grant No. AF-AFOSR-869-65, through the Ohio State University Research Foundation.

Phys. Rev. 167, 271 – Published 10 March, 1968

DOI: https://doi.org/10.1103/PhysRev.167.271

Abstract

The nuclear-spin relaxation of orthohydrogen molecules in solid H2 is due to the intramolecular dipole-dipole interaction modulated by the quadrupole-quadrupole interaction between J=1 molecules. Using the statistical method developed by Margenau and Anderson, we calculate the angular momentum correlation functions. In contrast to Moriya and Motizuki's result, where the Gaussian mode is used and relaxation times are found to be proportional to c12 (c is the concentration of orthohydrogen molecules in the solid), we obtain relaxation times proportional to c53. Our result checks with the experimental data of Hardy and Gaines for c<0.3. In order to fit the experimental data for the entire range of concentration, a crystal field on the orthohydrogen molecules in the range 0.01-0.03°K must be assumed.

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