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Recoil Studies of Nuclear Reactions Induced by Heavy Ions

John M. Alexander and Lester Winsberg

  • Lawrence Radiation Laboratory, University of California, Berkeley, California

Phys. Rev. 121, 529 – Published 15 January, 1961

DOI: https://doi.org/10.1103/PhysRev.121.529

Abstract

The mechanism of nuclear reactions induced by heavy ions was investigated by measuring the recoil ranges of Tb149, At211 and other alpha-emitting isotopes of At and neighboring elements and by determining the cross sections for the formation of Tb149 and At211.

Recoil ranges were consistent with compound-nucleus formation at all energies studied for the following reactions: Pr141(C12, 4n)Tb149, Ce(N14, xn)Tb149, La139(O16, 6n)Tb149, La139(O18, 8n)Tb149, and Ba(Ne22, pxn)Tb149. A similar result was obtained for the reaction Pr141(O16, 2p6n)Tb149 at 138 and at 146 Mev and for the reactions Au197(O16, 2pxn and 3pxn)At, Po at energies below 100 Mev. The excitation functions of the (HI, xn)Tb149 reactions seem to be characteristic of an evaporation process but have smaller peak cross sections than do the excitation functions of the reactions Ba(Ne22, pxn)Tb149 or Pr141(O16, 2p6n)Tb149. We conclude that most reactions probably involve charged-particle emission. The reaction Ba(Ne22, pxn)Tb149 seems to occur with much greater probability than the reaction Ba(Ne20, pxn)Tb149.

In many cases the compound-nucleus mechanism cannot account for our results. Partial momentum transfer is observed in the reactions Au197(O16, 2pxn and 3pxn)At,Po at energies above 100 Mev. Partial momentum transfer also occurs when Bi is bombarded at energies 1.3 times the barrier energy or greater. Reactions of Bi with heavy ions (Ne20 is possible exception) at energies near the Coulomb barrier produce At211 with greater recoil energy than expected from a compound-nucleus mechanism. Apparently, particles are emitted in the backward direction. Near the barrier the cross section for the production of At211 by C12, O16, and Ne20 bombardment comprises about ¼ the value calculated for compound-nucleus formation. Therefore, the cross section for all noncompound-nucleus reactions must comprise a large fraction of the total interaction cross section. The experiments with Pb as a target are also consistent with this conclusion.

References (12)

  1. L. Winsberg and J. M. Alexander, preceding paper [Phys. Rev. 121, 518 (1961)]
  2. J. Blatt and V. F. Weisskopf, Theoretical Nuclear Physics (John Wiley & Sons, Inc., New York, 1952)
  3. I. Dostrovsky, Z. Fraenkel, and G. Friedlander, Phys. Rev. 116, 683 (1959)
  4. I. Dostrovsky, Z. Fraenkel, and L. Winsberg, Phys. Rev. 118, 781 (1960)
  5. P. F. Donovan, B. G. Harvey, and W. H. Wade, Phys. Rev. 119, 218, 225 (1960)
  6. J. M. Alexander and L. Winsberg, Proceedings of the Second Conference on Reactions between Complex Nuclei, Gatlinburg, Tennessee [John Wiley & Sons, New York (to be published)]
  7. D. Strominger, J. M. Hollander, and G. T. Seaborg, Revs. Modern Phys. 30, No. 2 (1958)
  8. Omitted endnote

  9. L. Winsberg, Bull. Am. Phys. Soc. 3, 406 (1958)
  10. T. D. Thomas, Phys. Rev. 116, 703 (1959)
  11. E. L. Hubbard, R. M. Main, and R. V. Pyle, Phys. Rev. 118, 507 (1960)
  12. P. F. Donovan, Bell Laboratories, Murray Hill, New Jersey (private communication)

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